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A scene that contains both old and instant events with a clear motion trail is visually intriguing and dynamic, which can convey a sense of change, transition, or evolution. Developing an eco-friendly delay display system offers a powerful tool for fusing old and instant events, which can be used for visualizing motion trails. Herein, we brighten triplet excitons of carbon nanodots (CNDs) and increase their emission yield by a multidimensional confinement strategy, and the CND-based delay display array is demonstrated. The intense confinement effects via multidimensional confinement strategy suppress nonradiative transitions, and 240% enhancement in the phosphorescence efficiency and 260% enhancement in the lifetime of the CNDs are thus realized. Considering their distinctive phosphorescence performances, a delay display array containing a 4 × 4 CND-based delay lighting device is demonstrated, which can provide ultralong phosphorescence over 7 s, and the motion that occurred in different timelines is recorded clearly. This finding will motivate the investigation of phosphorescent CNDs in motion trail recognition.
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Room-temperature phosphorescent materials, renowned for their long luminescence lifetimes, have garnered significant attention in the field of optical materials. However, the challenges posed by thermally induced quenching have significantly hindered the advancement of luminescence efficiency and stability. In this study, thermally enhanced phosphorescent carbon nanodots (CND) are developed by incorporating them into fiber matrices. Remarkably, the phosphorescence lifetime of the thermally enhanced CND exhibits a twofold enhancement, increasing from 326 to 753 ms, while the phosphorescence intensity experienced a tenfold enhancement, increasing from 25 to 245 as the temperature increased to 373 K. Rigid fiber matrices can effectively suppress the non-radiative transition rate of triplet excitons, while high temperatures can desorb oxygen adsorbed on the surface of the CND, disrupting the interaction between the CND and oxygen. Consequently, a thermally enhanced phosphorescence is obtained. In addition, benefiting from the thermally enhanced phosphorescence property of CND, a warning indicator with an anti-counterfeiting function for monitoring cold-chain logistics is demonstrated based on CND.
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The Tavis-Cummings model is intensively investigated in quantum optics and has important applications in generation of multi-atom entanglement. Here, we employ a superconducting circuit quantum electrodynamic system to study a modified Tavis-Cummings model with directly-coupled atoms. In our device, three superconducting artificial atoms are arranged in a chain with direct coupling through fixed capacitors and strongly coupled to a transmission line resonator. By performing transmission spectrum measurements, we observe different anticrossing structures when one or two qubits are resonantly coupled to the resonator. In the case of the two-qubit Tavis-Cummings model without qubit-qubit interaction, we observe two dips at the resonance point of the anticrossing. The splitting of these dips is determined by Δ λ=2g12+g32, where g1 and g3 are the coupling strengths between Qubit 1 and the resonator, and Qubit 3 and the resonator, respectively. The direct coupling J12 between the two qubits results in three dressed states in the two-qubit Tavis-Cummings model at the frequency resonance point, leading to three dips in the transmission spectrum. In this case, the distance between the two farthest and asymmetrical dips, arising from the energy level splitting, is larger than in the previous case. The frequency interval between these two dips is determined by the difference in eigenvalues (Δ λ=ε 1+-ε 1-), obtained through numerical calculations. What we believe as novel and intriguing experimental results may potentially advance quantum optics experiments, providing valuable insights for future research.
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We propose how to achieve nonreciprocal quantum entanglement of light and motion and reveal its counterintuitive robustness against random losses. We find that by splitting the counterpropagating lights of a spinning resonator via the Sagnac effect, photons and phonons can be entangled strongly in a chosen direction but fully uncorrelated in the other. This makes it possible both to realize quantum nonreciprocity even in the absence of any classical nonreciprocity and also to achieve significant entanglement revival against backscattering losses in practical devices. Our work provides a way to protect and engineer quantum resources by utilizing diverse nonreciprocal devices, for building noise-tolerant quantum processors, realizing chiral networks, and backaction-immune quantum sensors.
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We propose a scheme to implement a supersensitive estimation of the coupling strength in a hybrid optomechanical system which consists of a cavity-Bose-Einstein condensate system coupled to an impurity. This method can dramatically improve the estimation precision even when the involved photon number is small. The quantum Fisher information indicates that the Heisenberg scale sensitivity of the coupling rate could be obtained when the photon loss rate is smaller than the corresponding critical value in the input of either coherent state or squeezed state. The critical photon decay rate for the coherent state is larger than that of the squeezed state, and the coherent state input case is more robust against the photon loss than the squeezed state case. We also present the measurement scheme which can saturate the quantum Cramér-Rao bound.
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We propose how to mechanically control photon blockade (PB) and photon-induced tunneling (PIT) in an optomechanical system. We show that single-photon blockade (1PB) and two-photon blockade (2PB) can emerge by tuning mechanical driving parameters. Moreover, by varying the strength of mechanical driving, PIT can be converted into 1PB or 2PB, or vice versa, with the constant optical frequency. We refer to this effect as PIT-1PB or PIT-2PB switch. In addition, the switch between 1PB and 2PB can also be realized with this strategy. This mechanical engineering of quantum optical effects can be understood from the shifts of energy levels induced by external mechanical pumping. Our results not only pave the way towards devising new schemes for quantum light switch but also, on a more fundamental level, could shed light on the nonclassicality of the few-photon states.
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We consider the effects of dipole-dipole interactions on a nonlinear interferometer with spin-1 Bose-Einstein condensates. Compared with the traditional atomic SU(1,1) interferometer, the shot-noise phase sensitivity can be beaten with respect to the input total average number of particles; and the improved sensitivity depends on the effective strength of the dipolar interaction via modifying the trapping geometry. It indicates that the best performance of the interferometer is achieved with highly oblate trap potential. The Bayesian phase estimation strategy is explored to extract the phase information. We show that the Cramér-Rao phase uncertainly bound can saturate, when the ideal dis-entangle scheme is applied. The phase average of the phase sensitivity is also discussed.
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We present a new generalized Dicke model, an impurity-doped Dicke model (IDDM), by the use of an impurity-doped cavity-Bose-Einstein condensate (BEC). It is shown that the impurity atom can induce Dicke quantum phase transition (QPT) from the normal phase to superradiant phase at a critic value of the impurity population. It is found that the impurity-induced Dicke QPT can happen in an arbitrary field-atom coupling regime while the Dicke QPT in the standard Dicke model occurs only in the strong coupling regime of the cavity field and atoms. This opens the possibility to realize the control of quantum properties of a macroscopic-quantum system (BEC) by using a microscopic quantum system (a single impurity atom).
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We investigate the possibility to control quantum evolution speed of a single dephasing qubit for arbitrary initial states by the use of periodic dynamical decoupling (PDD) pulses. It is indicated that the quantum speed limit time (QSLT) is determined by initial and final quantum coherence of the qubit, as well as the non-Markovianity of the system under consideration during the evolution when the qubit is subjected to a zero-temperature Ohmic-like dephasing reservoir. It is shown that final quantum coherence of the qubit and the non-Markovianity of the system can be modulated by PDD pulses. Our results show that for arbitrary initial states of the dephasing qubit with non-vanishing quantum coherence, PDD pulses can be used to induce potential acceleration of the quantum evolution in the short-time regime, while PDD pulses can lead to potential speedup and slow down in the long-time regime. We demonstrate that the effect of PDD on the QSLT for the Ohmic or sub-Ohmic spectrum (Markovian reservoir) is much different from that for the super-Ohmic spectrum (non-Markovian reservoir).
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We study the nonlinear dynamics of collective excitation in an N -site XXZ quantum spin chain, which is manipulated by an oblique magnetic field. We show that, when the tilted field is applied along the magic angle, theta_{0}=+/-arccossqrt[13] , the anisotropic Heisenberg spin chain becomes isotropic and thus an freely propagating spin wave is stimulated. Also, in the regime of tilted angles larger and smaller than the magic angle, two types of nonlinear excitations appear: bright and dark solitons.
