Conditional Dynamics in Heterodyne Detection of Superradiant Lasing with Incoherently Pumped Atoms.

In this Letter, we use quantum trajectory theory to simulate heterodyne detection of narrow bandwidth superradiant lasing from an incoherently excited atomic ensemble. To this end, we describe the system dynamics and account for stochastic measurement backaction by second-order mean-field theory. Our simulations show how heterodyne measurements break the phase symmetry, and initiate the atomic coherence with a random phase and a long temporal phase coherence. More importantly, our theory allows direct simulation of experimental procedures for extraction of spectral information which do not lend themselves to evaluation with the quantum regression theorem.

In situ amplification of spin echoes within a kinetic inductance parametric amplifier.

The use of superconducting microresonators together with quantum-limited Josephson parametric amplifiers has enhanced the sensitivity of pulsed electron spin resonance (ESR) measurements by more than four orders of magnitude. So far, the microwave resonators and amplifiers have been designed as separate components due to the incompatibility of Josephson junction-based devices with magnetic fields. This has produced complex spectrometers and raised technical barriers toward adoption of the technique. Here, we circumvent this issue by coupling an ensemble of spins directly to a weakly nonlinear and magnetic field-resilient superconducting microwave resonator. We perform pulsed ESR measurements with a 1-pL mode volume containing 6 × 107 spins and amplify the resulting signals within the device. When considering only those spins that contribute to the detected signals, we find a sensitivity of [Formula: see text] for a Hahn echo sequence at a temperature of 400 mK. In situ amplification is demonstrated at fields up to 254 mT, highlighting the technique's potential for application under conventional ESR operating conditions.

Quantum Nondemolition Measurements of Moving Target States.

We present a protocol for probing the state of a quantum system by its resonant coupling and entanglement with a meter system. By continuous measurement of a time evolving meter observable, we infer the evolution of the entangled systems and, ultimately, the state and dynamics of the system of interest. The photon number in a cavity field is thus resolved by simulated monitoring of the Rabi oscillations of a resonantly coupled two-level system, and we propose to regard this as a practical extension of quantum nondemolition measurements with applications in quantum metrology and quantum computing.

Cavity Quantum Electrodynamics Effects with Nitrogen Vacancy Center Spins Coupled to Room Temperature Microwave Resonators.

Cavity quantum electrodynamics (CQED) effects, such as Rabi splitting, Rabi oscillations, and superradiance, have been demonstrated with nitrogen vacancy (NV) center spins in diamond coupled to microwave resonators at cryogenic temperature. In this Letter, we explore the possibility to realize strong collective coupling and CQED effects with ensembles of NV spins at room temperature. Our calculations show that thermal excitation of the individual NV spins leads to population of collective Dicke states with low symmetry and a reduced collective coupling to the microwave resonators. Optical pumping can be applied to counteract the thermal excitation of the NV centers and to prepare the spin ensemble in Dicke states with high symmetry. The resulting strong coupling with high-quality resonators enables the study of intriguing CQED effects across the weak-to-strong coupling regime, and may have applications in quantum sensing and quantum information processing.

Deterministic Photon Sorting in Waveguide QED Systems.

Sorting quantum fields into different modes according to their Fock-space quantum numbers is a highly desirable quantum operation. In this Letter, we show that a pair of two-level emitters, chirally coupled to a waveguide, may scatter single- and two-photon components of an input pulse into orthogonal temporal modes with a fidelity ≳0.9997. We develop a general theory to characterize and optimize this process and reveal that such a high fidelity is enabled by an interesting two-photon scattering dynamics: while the first emitter gives rise to a complex multimode field, the second emitter recombines the field amplitudes, and the net two-photon scattering induces a self-time reversal of the input pulse mode. The presented scheme can be employed to construct logic elements for propagating photons, such as a deterministic nonlinear-sign gate with a fidelity ≳0.9995.

Free-Fermion Multiply Excited Eigenstates and Their Experimental Signatures in 1D Arrays of Two-Level Atoms.

One-dimensional (1D) subwavelength atom arrays display multiply excited subradiant eigenstates which are reminiscent of free fermions. So far, these states have been associated with subradiant states with decay rates ∝N^{-3}, with N the number of atoms, which fundamentally prevents detection of their fermionic features by optical means. In this Letter, we show that free-fermion states generally appear whenever the band of singly excited states has a quadratic dispersion relation at the band edge and, hence, may also be obtained with radiant and even superradiant states. 1D arrays have free-fermion multiply excited eigenstates that are typically either subradiant or (super)radiant, and we show that a simple transformation acts between the two families. Based on this correspondence, we propose different means for their preparation and analyze their experimental signature in optical detection.

Active Frequency Measurement on Superradiant Strontium Clock Transitions.

We develop a stochastic mean-field theory to describe active frequency measurements of pulsed superradiant emission, studied in a recent experiment with strontium-87 atoms trapped in an optical lattice inside an optical cavity [M. Norcia et al., Phys. Rev. X 8, 021036 (2018)PRXHAE2160-330810.1103/PhysRevX.8.021036]. Our theory reveals the intriguing dynamics of atomic ensembles with multiple transition frequencies, and it reproduces the superradiant beats signal, noisy power spectra, and frequency uncertainty in remarkable agreement with the experiments. Moreover, using longer superradiant pulses of similar strength and shortening the experimental duty cycle, we predict a short-term frequency uncertainty 7×10^{-17}/sqrt[τ/s], which makes active frequency measurements with superradiant transitions comparable with the record performance of current frequency standards [M. Schioppo et al., Nat. Photonics 11, 48 (2017)NPAHBY1749-488510.1038/nphoton.2016.231]. Our theory combines cavity quantum electrodynamics and quantum measurement theory, and it can be readily applied to explore conditional quantum dynamics and describe frequency measurements for other processes such as steady-state superradiance and superradiant Raman lasing.

Ultranarrow Superradiant Lasing by Dark Atom-Photon Dressed States.

We show that incoherent pumping of an optical lattice clock system with ultracold strontium-88 atoms produces laser light with a ≃10 Hz linewidth when the atoms are exposed to a magnetic field. This linewidth is orders of magnitude smaller than both the cavity linewidth and the incoherent atomic decay and excitation rates. The narrow lasing is due to an interplay of multiatom superradiant effects and the coupling of bright and dark atom-light dressed states by the magnetic field.

Retrodiction beyond the Heisenberg uncertainty relation.

In quantum mechanics, the Heisenberg uncertainty relation presents an ultimate limit to the precision by which one can predict the outcome of position and momentum measurements on a particle. Heisenberg explicitly stated this relation for the prediction of "hypothetical future measurements", and it does not describe the situation where knowledge is available about the system both earlier and later than the time of the measurement. Here, we study what happens under such circumstances with an atomic ensemble containing 1011 rubidium atoms, initiated nearly in the ground state in the presence of a magnetic field. The collective spin observables of the atoms are then well described by canonical position and momentum observables, [Formula: see text] and [Formula: see text] that satisfy [Formula: see text]. Quantum non-demolition measurements of [Formula: see text] before and of [Formula: see text] after time t allow precise estimates of both observables at time t. By means of the past quantum state formalism, we demonstrate that outcomes of measurements of both the [Formula: see text] and [Formula: see text] observables can be inferred with errors below the standard quantum limit. The capability of assigning precise values to multiple observables and to observe their variation during physical processes may have implications in quantum state estimation and sensing.

Self-Stimulated Pulse Echo Trains from Inhomogeneously Broadened Spin Ensembles.

We show experimentally and describe theoretically how a conventional magnetic resonance Hahn echo sequence can lead to a self-stimulated pulse echo train when an inhomogeneously broadened spin ensemble is coupled to a resonator. Effective strong coupling between the subsystems assures that the first Hahn echo can act as a refocusing pulse on the spins, leading to self-stimulated secondary echoes. Within the framework of mean field theory, we show that this process can continue multiple times leading to a train of echoes. We introduce an analytical model that explains the shape of the first echo and numerical results that account well for the experimentally observed shape and strength of the echo train and provides insights into the collective effects involved.

Retraction Note: Exploring the quantum speed limit with computer games.

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

Spin squeezing of 1011 atoms by prediction and retrodiction measurements.

The measurement sensitivity of quantum probes using N uncorrelated particles is restricted by the standard quantum limit1, which is proportional to [Formula: see text]. This limit, however, can be overcome by exploiting quantum entangled states, such as spin-squeezed states2. Here we report the measurement-based generation of a quantum state that exceeds the standard quantum limit for probing the collective spin of 1011 rubidium atoms contained in a macroscopic vapour cell. The state is prepared and verified by sequences of stroboscopic quantum non-demolition (QND) measurements. We then apply the theory of past quantum states3,4 to obtain spin state information from the outcomes of both earlier and later QND measurements. Rather than establishing a physically squeezed state in the laboratory, the past quantum state represents the combined system information from these prediction and retrodiction measurements. This information is equivalent to a noise reduction of 5.6 decibels and a metrologically relevant squeezing of 4.5 decibels relative to the coherent spin state. The past quantum state yields tighter constraints on the spin component than those obtained by conventional QND measurements. Our measurement uses 1,000 times more atoms than previous squeezing experiments5-10, with a corresponding angular variance of the squeezed collective spin of 4.6 × 10-13 radians squared. Although this work is rooted in the foundational theory of quantum measurements, it may find practical use in quantum metrology and quantum parameter estimation, as we demonstrate by applying our protocol to quantum enhanced atomic magnetometry.

Subradiant Emission from Regular Atomic Arrays: Universal Scaling of Decay Rates from the Generalized Bloch Theorem.

The Hermitian part of the field-mediated dipole-dipole interaction in infinite periodic arrays of two-level atoms yields an energy band of the singly excited states. In this Letter, we show that a dispersion relation, ω_{k}-ω_{k_{ex}}∝(k-k_{ex})^{s}, near the band edge of the infinite system leads to the existence of subradiant states of finite one-dimensional arrays of N atoms with decay rates scaling as N^{-(s+1)}. This explains the recently discovered N^{-3} scaling and it leads to the prediction of power law scaling with higher power for special values of the lattice period. For the quantum optical implementation of the Su-Schrieffer-Heeger topological model in a dimerized emitter array, the band gap closing inherent to topological transitions changes the value of s in the dispersion relation and alters the decay rates of the subradiant states by many orders of magnitude.

Input-Output Theory with Quantum Pulses.

We present a formalism that accounts for the interaction of a local quantum system, such as an atom or a cavity, with traveling pulses of quantized radiation. We assume Markovian coupling of the stationary system to the input and output fields and nondispersive asymptotic propagation of the pulses before and after the interaction. This permits derivation of a master equation where the input and output pulses are treated as single oscillator modes that both couple to the local system in a cascaded manner. As examples of our theory, we analyze reflection by an empty cavity with phase noise, stimulated atomic emission by a quantum light pulse, and formation of a Schrödinger-cat state by the dispersive interaction of a coherent pulse and a single atom in a cavity.

Theory of Subradiant States of a One-Dimensional Two-Level Atom Chain.

Recently, the subradiant states of one-dimensional two-level atom chains coupled to light modes were found to have decay rates obeying a universal scaling, and an unexpected fermionic character of the multiply excited subradiant states was discovered. In this Letter, we theoretically obtain the singly excited subradiant states, and by eliminating the superradiant modes, we demonstrate a relation between the multiply excited subradiant states and the Tonks-Girardeau limit of the Lieb-Liniger model which explains the fermionic behavior. In addition, we identify a new family of subradiant states with correlations different from the fermionic ansatz.

Deterministic Free-Space Source of Single Photons Using Rydberg Atoms.

We propose an efficient free-space scheme to create single photons in a well-defined spatiotemporal mode. To that end, we first prepare a single source atom in an excited Rydberg state. The source atom interacts with a large ensemble of ground-state atoms via a laser-mediated dipole-dipole exchange interaction. Using an adiabatic passage with a chirped laser pulse, we produce a spatially extended spin wave of a single Rydberg excitation in the ensemble, accompanied by the transition of the source atom to another Rydberg state. The collective atomic excitation can then be converted to a propagating optical photon via a coherent coupling field. In contrast to previous approaches, our single-photon source does not rely on the strong coupling of a single emitter to a resonant cavity, nor does it require the heralding of collective excitation or complete Rydberg blockade of multiple excitations in the atomic ensemble.

Entangled Quantum Dynamics of Many-Body Systems using Bohmian Trajectories.

Bohmian mechanics is an interpretation of quantum mechanics that describes the motion of quantum particles with an ensemble of deterministic trajectories. Several attempts have been made to utilize Bohmian trajectories as a computational tool to simulate quantum systems consisting of many particles, a very demanding computational task. In this paper, we present a novel ab-initio approach to solve the many-body problem for bosonic systems by evolving a system of one-particle wavefunctions representing pilot waves that guide the Bohmian trajectories of the quantum particles. In this approach, quantum entanglement effects arise due to the interactions between different configurations of Bohmian particles evolving simultaneously. The method is used to study the breathing dynamics and ground state properties in a system of interacting bosons.

Blueprint for a microwave trapped ion quantum computer.

The availability of a universal quantum computer may have a fundamental impact on a vast number of research fields and on society as a whole. An increasingly large scientific and industrial community is working toward the realization of such a device. An arbitrarily large quantum computer may best be constructed using a modular approach. We present a blueprint for a trapped ion-based scalable quantum computer module, making it possible to create a scalable quantum computer architecture based on long-wavelength radiation quantum gates. The modules control all operations as stand-alone units, are constructed using silicon microfabrication techniques, and are within reach of current technology. To perform the required quantum computations, the modules make use of long-wavelength radiation-based quantum gate technology. To scale this microwave quantum computer architecture to a large size, we present a fully scalable design that makes use of ion transport between different modules, thereby allowing arbitrarily many modules to be connected to construct a large-scale device. A high error-threshold surface error correction code can be implemented in the proposed architecture to execute fault-tolerant operations. With appropriate adjustments, the proposed modules are also suitable for alternative trapped ion quantum computer architectures, such as schemes using photonic interconnects.

Hong-Ou-Mandel Interference between Two Deterministic Collective Excitations in an Atomic Ensemble.

We demonstrate deterministic generation of two distinct collective excitations in one atomic ensemble, and we realize the Hong-Ou-Mandel interference between them. Using Rydberg blockade we create single collective excitations in two different Zeeman levels, and we use stimulated Raman transitions to perform a beam-splitter operation between the excited atomic modes. By converting the atomic excitations into photons, the two-excitation interference is measured by photon coincidence detection with a visibility of 0.89(6). The Hong-Ou-Mandel interference witnesses an entangled NOON state of the collective atomic excitations, and we demonstrate its two times enhanced sensitivity to a magnetic field compared with a single excitation. Our work implements a minimal instance of boson sampling and paves the way for further multimode and multiexcitation studies with collective excitations of atomic ensembles.