Observation of the modification of quantum statistics of plasmonic systems.

For almost two decades, researchers have observed the preservation of the quantum statistical properties of bosons in a large variety of plasmonic systems. In addition, the possibility of preserving nonclassical correlations in light-matter interactions mediated by scattering among photons and plasmons stimulated the idea of the conservation of quantum statistics in plasmonic systems. It has also been assumed that similar dynamics underlie the conservation of the quantum fluctuations that define the nature of light sources. So far, plasmonic experiments have been performed in nanoscale systems in which complex multiparticle interactions are restrained. Here, we demonstrate that the quantum statistics of multiparticle systems are not always preserved in plasmonic platforms and report the observation of their modification. Moreover, we show that optical near fields provide additional scattering paths that can induce complex multiparticle interactions. Remarkably, the resulting multiparticle dynamics can, in turn, lead to the modification of the excitation mode of plasmonic systems. These observations are validated through the quantum theory of optical coherence for single- and multi-mode plasmonic systems. Our findings unveil the possibility of using multiparticle scattering to perform exquisite control of quantum plasmonic systems.

Theoretical analysis of quantum random walks with stress-engineered optics.

Quantum random walks (QRWs) are random processes in which the resulting probability density of the "walker" state, whose movement is governed by a "coin" state, is described in a nonclassical manner. Previously, Q-plates have been used to demonstrate QRWs with polarization and orbital angular momentum playing the roles of coin and walker states, respectively. In this theoretical analysis, we show how stress-engineered optics can be used to develop new platforms for complex QRWs through relatively simple optical elements. Our work opens up new paths to speed up classical-to-quantum transitions in robust photonic networks.

Quantum imaging and information.

The maturity of fields such as optical physics and quantum optics has brought with it a new era where the photon represents a promising information resource. In the past few years, scientists and engineers have exploited multiple degrees of freedom of the photon to perform information processing for a wide variety of applications. Of particular importance, the transverse spatial degree of freedom has offered a flexible platform to test complex quantum information protocols in a relatively simple fashion. In this regard, novel imaging techniques that exploit the quantum properties of light have also been investigated. In this review article, we define the fundamental parameters that describe the spatial wavefunction of the photon and establish their importance for applications in quantum information processing. More specifically, we describe the underlying physics behind remarkable protocols in which information is processed through high-dimensional spatial states of photons with sub-shot-noise levels or where quantum images with unique resolution features are formed. We also discuss the fundamental role that certain imaging techniques have played in the development of novel methods for quantum information processing and vice versa.

Measurement of the Photon-Plasmon Coupling Phase Shift.

Scattering processes have played a crucial role in the development of quantum theory. In the field of optics, scattering phase shifts have been utilized to unveil interesting forms of light-matter interactions. Here we investigate the phase shift experienced by a single photon as it scatters into a surface plasmon polariton and vice versa. This coupling phase shift is of particular relevance for quantum plasmonic experiments. Therefore, we demonstrate that the photon-plasmon interaction at a plasmonic slit can be modeled through a quantum-mechanical tritter, a six-port scattering element. We show that the visibilities of a double-slit and a triple-slit interference patterns are convenient observables to characterize the interaction at a slit and determine the coupling phase. Our accurate and simple model of the interaction, validated by simulations and experiments, has important implications not only for quantum plasmonic interference effects, but is also advantageous to classical applications.

Measurement of the radial mode spectrum of photons through a phase-retrieval method.

We propose and demonstrate a simple and easy-to-implement projective-measurement protocol to determine the radial index p of a Laguerre-Gaussian (LGpl) mode. Our method entails converting any specified high-order LGp0 mode into a near-Gaussian distribution that matches the fundamental mode of a single-mode fiber (SMF) through the use of two phase screens (unitary transforms) obtained by applying a phase-retrieval algorithm. The unitary transforms preserve the orthogonality of modes before the SMF and guarantee that our protocol can, in principle, be free of crosstalk. We measure the coupling efficiency of the transformed radial modes to the SMF for different pairs of phase screens. Because of the universality of phase-retrieval methods, we believe that our protocol provides an efficient way of fully characterizing the radial spatial profile of an optical field.

Single-shot measurement of the orbital-angular-momentum spectrum of light.

The existing methods for measuring the orbital-angular-momentum (OAM) spectrum suffer from issues such as poor efficiency, strict interferometric stability requirements, and too much loss. Furthermore, most techniques inevitably discard part of the field and measure only a post-selected portion of the true spectrum. Here, we propose and demonstrate an interferometric technique for measuring the true OAM spectrum of optical fields in a single-shot manner. Our technique directly encodes the OAM-spectrum information in the azimuthal intensity profile of the output interferogram. In the absence of noise, the spectrum can be fully decoded using a single acquisition of the output interferogram, and, in the presence of noise, acquisition of two suitable interferograms is sufficient for the purpose. As an important application of our technique, we demonstrate measurements of the angular Schmidt spectrum of the entangled photons produced by parametric down-conversion and report a broad spectrum with the angular Schmidt number 82.1.

Digital spiral object identification using random light.

Photons that are entangled or correlated in orbital angular momentum have been extensively used for remote sensing, object identification and imaging. It has recently been demonstrated that intensity fluctuations give rise to the formation of correlations in the orbital angular momentum components and angular positions of random light. Here we demonstrate that the spatial signatures and phase information of an object with rotational symmetries can be identified using classical orbital angular momentum correlations in random light. The Fourier components imprinted in the digital spiral spectrum of the object, as measured through intensity correlations, unveil its spatial and phase information. Sharing similarities with conventional compressive sensing protocols that exploit sparsity to reduce the number of measurements required to reconstruct a signal, our technique allows sensing of an object with fewer measurements than other schemes that use pixel-by-pixel imaging. One remarkable advantage of our technique is that it does not require the preparation of fragile quantum states of light and operates at both low- and high-light levels. In addition, our technique is robust against environmental noise, a fundamental feature of any realistic scheme for remote sensing.

Exotic looped trajectories of photons in three-slit interference.

The validity of the superposition principle and of Born's rule are well-accepted tenants of quantum mechanics. Surprisingly, it has been predicted that the intensity pattern formed in a three-slit experiment is seemingly in contradiction with the most conventional form of the superposition principle when exotic looped trajectories are taken into account. However, the probability of observing such paths is typically very small, thus rendering them extremely difficult to measure. Here we confirm the validity of Born's rule and present the first experimental observation of exotic trajectories as additional paths for the light by directly measuring their contribution to the formation of optical interference fringes. We accomplish this by enhancing the electromagnetic near-fields in the vicinity of the slits through the excitation of surface plasmons. This process increases the probability of occurrence of these exotic trajectories, demonstrating that they are related to the near-field component of the photon's wavefunction.

Hanbury Brown and Twiss interferometry with twisted light.

The rich physics exhibited by random optical wave fields permitted Hanbury Brown and Twiss to unveil fundamental aspects of light. Furthermore, it has been recognized that optical vortices are ubiquitous in random light and that the phase distribution around these optical singularities imprints a spectrum of orbital angular momentum onto a light field. We demonstrate that random fluctuations of intensity give rise to the formation of correlations in the orbital angular momentum components and angular positions of pseudothermal light. The presence of these correlations is manifested through distinct interference structures in the orbital angular momentum-mode distribution of random light. These novel forms of interference correspond to the azimuthal analog of the Hanbury Brown and Twiss effect. This family of effects can be of fundamental importance in applications where entanglement is not required and where correlations in angular position and orbital angular momentum suffice. We also suggest that the azimuthal Hanbury Brown and Twiss effect can be useful in the exploration of novel phenomena in other branches of physics and astrophysics.

Enhanced spectral sensitivity of a chip-scale photonic-crystal slow-light interferometer.

We experimentally demonstrate that the spectral sensitivity of a Mach-Zehnder (MZ) interferometer can be enhanced through structural slow light. We observe a 20-fold resolution enhancement by placing a dispersion-engineered, slow-light, photonic-crystal waveguide in one arm of a fiber-based MZ interferometer. The spectral sensitivity of the interferometer increases roughly linearly with the group index, and we have quantified the resolution in terms of the spectral density of interference fringes. These results show promise for the use of slow-light methods for developing novel tools for optical metrology and, specifically, for compact high-resolution spectrometers.

Wigner Distribution of Twisted Photons.

We present the first experimental characterization of the azimuthal Wigner distribution of a photon. Our protocol fully characterizes the transverse structure of a photon in conjugate bases of orbital angular momentum (OAM) and azimuthal angle. We provide a test of our protocol by characterizing pure superpositions and incoherent mixtures of OAM modes in a seven-dimensional space. The time required for performing measurements in our scheme scales only linearly with the dimension size of the state under investigation. This time scaling makes our technique suitable for quantum information applications involving a large number of OAM states.

Light-Drag Enhancement by a Highly Dispersive Rubidium Vapor.

The change in the speed of light as it propagates through a moving material has been a subject of study for almost two centuries. This phenomenon, known as the Fresnel light-drag effect, is quite small and usually requires a large interaction path length and/or a large velocity of the moving medium to be observed. Here, we show experimentally that the observed drag effect can be enhanced by over 2 orders of magnitude when the light beam propagates through a moving slow-light medium. Our results are in good agreement with the theoretical prediction, which indicates that, in the limit of large group indices, the strength of the light-drag effect is proportional to the group index of the moving medium.

Quantum Hilbert Hotel.

In 1924 David Hilbert conceived a paradoxical tale involving a hotel with an infinite number of rooms to illustrate some aspects of the mathematical notion of "infinity." In continuous-variable quantum mechanics we routinely make use of infinite state spaces: here we show that such a theoretical apparatus can accommodate an analog of Hilbert's hotel paradox. We devise a protocol that, mimicking what happens to the guests of the hotel, maps the amplitudes of an infinite eigenbasis to twice their original quantum number in a coherent and deterministic manner, producing infinitely many unoccupied levels in the process. We demonstrate the feasibility of the protocol by experimentally realizing it on the orbital angular momentum of a paraxial field. This new non-Gaussian operation may be exploited, for example, for enhancing the sensitivity of NOON states, for increasing the capacity of a channel, or for multiplexing multiple channels into a single one.

Compressive direct measurement of the quantum wave function.

The direct measurement of a complex wave function has been recently realized by using weak values. In this Letter, we introduce a method that exploits sparsity for the compressive measurement of the transverse spatial wave function of photons. The procedure involves weak measurements of random projection operators in the spatial domain followed by postselection in the momentum basis. Using this method, we experimentally measure a 192-dimensional state with a fidelity of 90% using only 25 percent of the total required measurements. Furthermore, we demonstrate the measurement of a 19,200-dimensional state, a task that would require an unfeasibly large acquiring time with the standard direct measurement technique.

Enhancing entangled-state phase estimation by combining classical and quantum protocols.

Here we describe a laboratory procedure by which we have increased the resolution of a measurement of the position of an optical component by a factor of 16. The factor of 16 arises from a four-fold quantum enhancement through the use of an N = 4 N00N state and a four-fold classical enhancement from a quadruple pass through a prism pair. The possibility of achieving supersensitivity using this method is discussed.

Rapid generation of light beams carrying orbital angular momentum.

We report a technique for encoding both amplitude and phase variations onto a laser beam using a single digital micro-mirror device (DMD). Using this technique, we generate Laguerre-Gaussian and vortex orbital-angular-momentum (OAM) modes, along with modes in a set that is mutually unbiased with respect to the OAM basis. Additionally, we have demonstrated rapid switching among the generated modes at a speed of 4 kHz, which is much faster than the speed regularly achieved by phase-only spatial light modulators (SLMs). The dynamic control of both phase and amplitude of a laser beam is an enabling technology for classical communication and quantum key distribution (QKD) systems that employ spatial mode encoding.