Ultrahigh-Q guided mode resonances in an All-dielectric metasurface.

High quality(Q) factor optical resonators are indispensable for many photonic devices. While very large Q-factors can be obtained theoretically in guided-mode settings, free-space implementations suffer from various limitations on the narrowest linewidth in real experiments. Here, we propose a simple strategy to enable ultrahigh-Q guided-mode resonances by introducing a patterned perturbation layer on top of a multilayer-waveguide system. We demonstrate that the associated Q-factors are inversely proportional to the perturbation squared while the resonant wavelength can be tuned through material or structural parameters. We experimentally demonstrate such high-Q resonances at telecom wavelengths by patterning a low-index layer on top of a 220 nm silicon on insulator substrate. The measurements show Q-factors up to 2.39 × 105, comparable to the largest Q-factor obtained by topological engineering, while the resonant wavelength is tuned by varying the lattice constant of the top perturbation layer. Our results hold great promise for exciting applications like sensors and filters.

Active quasi-BIC metasurfaces assisted by epsilon-near-zero materials.

Active devices play a critical role in modern electromagnetic and photonics systems. To date, the epsilon (ε)-near-zero (ENZ) is usually integrated with the low Q-factor resonant metasurface to achieve active devices, and enhance the light-matter interaction significantly at the nanoscale. However, the low Q-factor resonance may limit the optical modulation. Less work has been focused on the optical modulation in the low-loss and high Q-factor metasurfaces. Recently, the emerging optical bound states in the continuum (BICs) provides an effective way for achieving high Q-factor resonators. In this work, we numerically demonstrate a tunable quasi-BICs (QBICs) by integrating a silicon metasurface with ENZ ITO thin film. Such a metasurface is composed of five square holes in a unit cell, and hosts multiple BICs by engineering the position of centre hole. We also reveal the nature of these QBICs by performing multipole decomposition and calculating near field distribution. Thanks to the large tunability of ITO's permittivity by external bias and high-Q factor enabled by QBICs, we demonstrate an active control on the resonant peak position and intensity of transmission spectrum by integrating ENZ ITO thin films with QBICs supported by silicon metasurfaces. We find that all QBICs show excellent performance on modulating the optical response of such a hybrid structure. The modulation depth can be up to 14.8 dB. We also investigate how the carrier density of ITO film influence the near-field trapping and far-field scattering, which in turn influence the performance of optical modulation based on this structure. Our results may find promising applications in developing active high-performance optical devices.

On-chip low-loss all-optical MoSe2 modulator.

Monolayer transition metal dichalcogenides (TMDCs), like MoS2, MoSe2, WS2, and WSe2, feature direct bandgaps, strong spin-orbit coupling, and exciton-polariton interactions at the atomic scale, which could be harnessed for efficient light emission, valleytronics, and polaritonic lasing, respectively. Nevertheless, to build next-generation photonic devices that make use of these features, it is first essential to model the all-optical control mechanisms in TMDCs. Herein, a simple model is proposed to quantify the performance of a 35-µm-long Si3N4 waveguide-integrated all-optical MoSe2 modulator. Using this model, a switching energy of 14.6 pJ is obtained for a transverse-magnetic (TM) and transverse-electric (TE) polarized pump signals at λ = 480 nm. Moreover, maximal extinction ratios of 20.6 dB and 20.1 dB are achieved for a TM and TE polarized probe signal, respectively, at λ = 500 nm with an ultra-low insertion loss of <0.3 dB. Moreover, the device operates with an ultrafast recovery time of 50 ps, while maintaining a high extinction ratio for practical applications. These findings facilitate modeling and designing novel TMDC-based photonic devices.

Topological Supercavity Resonances in the Finite System.

Acoustic resonant cavities play a vital role in modern acoustical systems. The ultrahigh quality-factor resonances are highly desired for some applications such as high-resolution acoustic sensors and acoustic lasers. Here, a class of supercavity resonances is theoretically proposed and experimentally demonstrated in a coupled acoustic resonator system, arising from the merged bound states in the continuum (BICs) in geometry space. Their topological origin is demonstrated by explicitly calculating their topological charges before and after BIC merging, accompanied by charges annihilation. Compared with other types of BICs, they are robust to the perturbation brought by fabrication imperfection. Moreover, it is found that such supercavity modes can be linked with the Friedrich-Wintgen BICs supported by an entire rectangular (cuboid) resonator sandwiched between two rectangular (or circular) waveguides and thus more supercavity modes are constructed. Then, these coupled resonators are fabricated and such a unique phenomenon-moving, merging, and vanishing of BICs-is experimentally confirmed by measuring their reflection spectra, which show good agreement with the numerical simulation and theoretical prediction of mode evolution. The results may find exciting applications in acoustic and photonics, such as enhanced acoustic emission, filtering, and sensing.

Photonic slide rule with metasurfaces.

As an elementary particle, a photon that carries information in frequency, polarization, phase, and amplitude, plays a crucial role in modern science and technology. However, how to retrieve the full information of unknown photons in an ultracompact manner over broad bandwidth remains a challenging task with growing importance. Here, we demonstrate a versatile photonic slide rule based on an all-silicon metasurface that enables us to reconstruct incident photons' frequency and polarization state. The underlying mechanism relies on the coherent interactions of frequency-driven phase diagrams which rotate at various angular velocities within broad bandwidth. The rotation direction and speed are determined by the topological charge and phase dispersion. Specifically, our metasurface leverages both achromatically focusing and azimuthally evolving phases with topological charges +1 and -1 to ensure the confocal annular intensity distributions. The combination of geometric phase and interference holography allows the joint manipulations of two distinct group delay coverages to realize angle-resolved in-pair spots in a transverse manner- a behavior that would disperse along longitudinal direction in conventional implementations. The spin-orbital coupling between the incident photons and vortex phases provides routing for the simultaneous identification of the photons' frequency and circular polarization state through recognizing the spots' locations. Our work provides an analog of the conventional slide rule to flexibly characterize the photons in an ultracompact and multifunctional way and may find applications in integrated optical circuits or pocketable devices.

Enhanced light-matter interaction in two-dimensional transition metal dichalcogenides.

Two-dimensional (2D) transition metal dichalcogenide (TMDC) materials, such as MoS2, WS2, MoSe2, and WSe2, have received extensive attention in the past decade due to their extraordinary electronic, optical and thermal properties. They evolve from indirect bandgap semiconductors to direct bandgap semiconductors while their layer number is reduced from a few layers to a monolayer limit. Consequently, there is strong photoluminescence in a monolayer (1L) TMDC due to the large quantum yield. Moreover, such monolayer semiconductors have two other exciting properties: large binding energy of excitons and valley polarization. These properties make them become ideal materials for various electronic, photonic and optoelectronic devices. However, their performance is limited by the relatively weak light-matter interactions due to their atomically thin form factor. Resonant nanophotonic structures provide a viable way to address this issue and enhance light-matter interactions in 2D TMDCs. Here, we provide an overview of this research area, showcasing relevant applications, including exotic light emission, absorption and scattering features. We start by overviewing the concept of excitons in 1L-TMDC and the fundamental theory of cavity-enhanced emission, followed by a discussion on the recent progress of enhanced light emission, strong coupling and valleytronics. The atomically thin nature of 1L-TMDC enables a broad range of ways to tune its electric and optical properties. Thus, we continue by reviewing advances in TMDC-based tunable photonic devices. Next, we survey the recent progress in enhanced light absorption over narrow and broad bandwidths using 1L or few-layer TMDCs, and their applications for photovoltaics and photodetectors. We also review recent efforts of engineering light scattering, e.g., inducing Fano resonances, wavefront engineering in 1L or few-layer TMDCs by either integrating resonant structures, such as plasmonic/Mie resonant metasurfaces, or directly patterning monolayer/few layers TMDCs. We then overview the intriguing physical properties of different van der Waals heterostructures, and their applications in optoelectronic and photonic devices. Finally, we draw our opinion on potential opportunities and challenges in this rapidly developing field of research.

Tunable unidirectional nonlinear emission from transition-metal-dichalcogenide metasurfaces.

Nonlinear light sources are central to a myriad of applications, driving a quest for their miniaturisation down to the nanoscale. In this quest, nonlinear metasurfaces hold a great promise, as they enhance nonlinear effects through their resonant photonic environment and high refractive index, such as in high-index dielectric metasurfaces. However, despite the sub-diffractive operation of dielectric metasurfaces at the fundamental wave, this condition is not fulfilled for the nonlinearly generated harmonic waves, thereby all nonlinear metasurfaces to date emit multiple diffractive beams. Here, we demonstrate the enhanced single-beam second- and third-harmonic generation in a metasurface of crystalline transition-metal-dichalcogenide material, offering the highest refractive index. We show that the interplay between the resonances of the metasurface allows for tuning of the unidirectional second-harmonic radiation in forward or backward direction, not possible in any bulk nonlinear crystal. Our results open new opportunities for metasurface-based nonlinear light-sources, including nonlinear mirrors and entangled-photon generation.

Sound trapping in an open resonator.

The ability of sound energy confinement with high-quality factor resonance is of vital importance for acoustic devices requiring high intensity and hypersensitivity in biological ultrasonics, enhanced collimated sound emission (i.e. sound laser) and high-resolution sensing. However, structures reported so far have been experimentally demonstrated with a limited quality factor of acoustic resonances, up to several tens in an open resonator. The emergence of bound states in the continuum makes it possible to realize high quality factor acoustic modes. Here, we report the theoretical design and experimental demonstration of acoustic bound states in the continuum supported by a single open resonator. We predicted that such an open acoustic resonator could simultaneously support three types of bound states in the continuum, including symmetry protected bound states in the continuum, Friedrich-Wintgen bound states in the continuum induced by mode interference, as well as a new type-mirror symmetry induced bound states in the continuum. We also experimentally demonstrated their existence with quality factor up to one order of magnitude greater than the highest quality factor reported in an open resonator.

Infrared all-dielectric Kerker metasurfaces.

The unidirectional scattering of electromagnetic waves in the backward and forward direction, termed Kerkers' first and second conditions, respectively, is a prominent feature of sub-wavelength particles, which also has been found recently in all-dielectric metasurfaces. Here we formulate the exact polarizability requirements necessary to achieve both Kerker conditions simultaneously with dipole terms only and demonstrate its equivalence to so-called "invisible metasurfaces". We further describe the perfect absorption mechanism in all-dielectric metasurfaces through development of an extended Kerker formalism. The phenomena of both invisibility and perfect absorption is shown in a 2D hexagonal array of cylindrical resonators, where only the resonator height is modified to switch between the two states. The developed framework provides critical insight into the range of scattering response possible with all-dielectric metasurfaces, providing a methodology for studying exotic electromagnetic phenomena.

Highly Efficient Near-Infrared Detector Based on Optically Resonant Dielectric Nanodisks.

Fast detection of near-infrared (NIR) photons with high responsivity remains a challenge for photodetectors. Germanium (Ge) photodetectors are widely used for near-infrared wavelengths but suffer from a trade-off between the speed of photodetection and quantum efficiency (or responsivity). To realize a high-speed detector with high quantum efficiency, a small-sized photodetector efficiently absorbing light is required. In this paper, we suggest a realization of a dielectric metasurface made of an array of subwavelength germanium PIN photodetectors. Due to the subwavelength size of each pixel, a high-speed photodetector with a bandwidth of 65 GHz has been achieved. At the same time, high quantum efficiency for near-infrared illumination can be obtained by the engineering of optical resonant modes to localize optical energy inside the intrinsic Ge disks. Furthermore, small junction capacitance and the possibility of zero/low bias operation have been shown. Our results show that all-dielectric metasurfaces can improve the performance of photodetectors.

Mid-infrared polarization-controlled broadband achromatic metadevice.

Metasurfaces provide a compact, flexible, and efficient platform to manipulate the electromagnetic waves. However, chromatic aberration imposes severe restrictions on their applications in broadband polarization control. Here, we propose a broadband achromatic methodology to implement polarization-controlled multifunctional metadevices in mid-wavelength infrared with birefringent meta-atoms. We demonstrate the generation of polarization-controlled and achromatically on-axis focused optical vortex beams with diffraction-limited focal spots and switchable topological charge (L ∥ = 0 and L ⊥ = 2). Besides, we further implement broadband achromatic polarization beamsplitter with high polarization isolation (extinction ratio up to 21). The adoption of all-silicon configuration not only facilitates the integration with CMOS technology but also endows the polarization multiplexing meta-atoms with broad phase dispersion coverage, ensuring the large size and high performance of the metadevices. Compared with the state-of-the-art chromatic aberration-restricted polarization-controlled metadevices, our work represents a substantial advance and a step toward practical applications.

Forward and Backward Switching of Nonlinear Unidirectional Emission from GaAs Nanoantennas.

High-index III-V semiconductor nanoantennas have gained great attention for enhanced nonlinear light-matter interactions, in the past few years. However, the complexity of nonlinear emission profiles imposes severe constraints on practical applications, such as in optical communications and integrated optoelectronic devices. These complexities include the lack of unidirectional nonlinear emission and the severe challenges in switching between forward and backward emissions, due to the structure of the susceptibility tensor of the III-V nanoantennas. Here, we propose a solution to both issues via engineering the nonlinear tensor of the nanoantennas. The special nonlinear tensorial properties of zinc-blende material can be used to engineer the nonlinear characteristics via growing the nanoantennas along different crystalline orientations. Based on the nonlinear multipolar effect, we have designed and fabricated (110)-grown GaAs nanoantennas, with engineered tensorial properties, embedded in a transparent low-index material. Our technique provides an approach not only for unidirectional second-harmonic generation (SHG) forward or backward emission but also for switching from one to another. Importantly, switching the SHG emission directionality is obtained only by rotating the polarization of the incident light, without the need for physical variation of the antennas or the environment. This characteristic is an advantage, as compared to other nonlinear nanoantennas, including (100)- and (111)-grown III-V counterparts or silicon and germanium nanoantennas. Indeed, (110)-GaAs nanoantennas allow for engineering the nonlinear nanophotonic systems including nonlinear "Huygens metasurfaces" and offer exciting opportunities for various nonlinear nanophotonics technologies, such as nanoscale light routing and light sources, as well as multifunctional flat optical elements.

Linear control of light scattering with multiple coherent waves excitation.

With the wave interferometric approach, we study how extrinsically coherent waves excitation can dramatically alter the overall scattering properties, resulting in tailoring the energy assignment between radiation and dissipation, as well as filtering multipolar resonances. As an illustration, we consider cylindrical passive systems encountered by arbitrary configurations of incident waves with various illuminating directions, phases, and intensities. With formulas for dissipation and radiation powers, we demonstrate that a coherent superposition of incident waves extrinsically interferes with the targeted channels in a desirable way. Moreover, the interferometric results can be irrespective of inherent system properties such as size, material, and structure. Our approach paves a non-invasive solution to manipulate wave-obstacle interaction at will.

High Fluence Chromium and Tungsten Bowtie Nano-antennas.

Nano-antennas are replicas of antennas that operate at radio-frequencies, but with considerably smaller dimensions when compared with their radio frequency counterparts. Noble metals based nano-antennas have the ability to enhance photoinduced phenomena such as localized electric fields, therefore-they have been used in various applications ranging from optical sensing and imaging to performance improvement of solar cells. However, such nano-structures can be damaged in high power applications such as heat resisted magnetic recording, solar thermo-photovoltaics and nano-scale heat transfer systems. Having a small footprint, nano-antennas cannot handle high fluences (energy density per unit area) and are subject to being damaged at adequately high power (some antennas can handle just a few milliwatts). In addition, given that nano-antennas are passive devices driven by external light sources, the potential damage of the antennas limits their use with high power lasers: this liability can be overcome by employing materials with high melting points such as chromium (Cr) and tungsten (W). In this article, we fabricate chromium and tungsten nano-antennas and demonstrate that they can handle 110 and 300 times higher fluence than that of gold (Au) counterpart, while the electric field enhancement is not significantly reduced.

Dynamic Nonlinear Image Tuning through Magnetic Dipole Quasi-BIC Ultrathin Resonators.

Dynamical tuning of the nonlinear optical wavefront allows for a specific spectral response of predefined profiles, enabling various applications of nonlinear nanophotonics. This study experimentally demonstrates the dynamical switching of images generated by an ultrathin silicon nonlinear metasurface supporting a high-quality leaky mode, which is formed by partially breaking a bound-state-in-the-continuum (BIC) generated by the collective magnetic dipole (MD) resonance excited in the subdiffractive periodic systems. Such a quasi-BIC MD state can be excited directly under normal plane wave incidence and leads to a strong near-field enhancement to further boost the nonlinear process, resulting in a 500-fold enhancement of the third-harmonic emission experimentally. Due to sharp spectral features and asymmetry of the unit cell, it allows for effective tailoring of the nonlinear emissions over spectral or polarization responses. Dynamical nonlinear image tuning is experimentally demonstarted via polarization and wavelength control. The results pave the way for nanophotonics applications such as tunable displays, nonlinear holograms, tunable nanolaser, and ultrathin nonlinear nanodevices with various functionalities.

Tailoring Second-Harmonic Emission from (111)-GaAs Nanoantennas.

Second-harmonic generation (SHG) in resonant dielectric Mie-scattering nanoparticles has been hailed as a powerful platform for nonlinear light sources. While bulk-SHG is suppressed in elemental semiconductors, for example, silicon and germanium due to their centrosymmetry, the group of zincblende III-V compound semiconductors, especially (100)-grown AlGaAs and GaAs, have recently been presented as promising alternatives. However, major obstacles to push the technology toward practical applications are the limited control over directionality of the SH emission and especially zero forward/backward radiation, resulting from the peculiar nature of the second-order nonlinear susceptibility of this otherwise highly promising group of semiconductors. Furthermore, the generated SH signal for (100)-GaAs nanoparticles depends strongly on the polarization of the pump. In this work, we provide both theoretically and experimentally a solution to these problems by presenting the first SHG nanoantennas made from (111)-GaAs embedded in a low index material. These nanoantennas show superior forward directionality compared to their (100)-counterparts. Most importantly, based on the special symmetry of the crystalline structure, it is possible to manipulate the SHG radiation pattern of the nanoantennas by changing the pump polarization without affecting the linear properties and the total nonlinear conversion efficiency, hence paving the way for efficient and flexible nonlinear beam-shaping devices.

High-Efficiency Visible Light Manipulation Using Dielectric Metasurfaces.

The development of a miniaturised device that provides efficient beam manipulation with high transmittance is extremely desirable for the broad range of applications including holography, metalens, and imaging. Recently, the potential of dielectric metasurfaces has been unleashed to efficiently manipulate the beam with full 2π-phase control by overlapping the electric and magnetic dipole resonances. However, in the visible range for available materials, it comes with the price of higher absorption that reduces efficiency. Here, we have considered dielectric amorphous silicon (a-Si) nanodisk and engineered them in such a way which provides minimal absorption loss in the visible range. We have experimentally demonstrated meta-deflector with high transmittance which operates in the visible wavelengths. The supercell of proposed meta-deflector consists of 15 amorphous silicon nanodisks numerically shows the transmission efficiency of 95% and deflection efficiency of 95% at operating wavelength of 715 nm. However, experimentally measured transmission and deflection efficiencies are 83% and 71%, respectively, having the experimental deflection angle of 8.40°. Nevertheless, by reducing the supercell length, the deflection angle can be controlled, and the value 15.50° was experimentally achieved using eight disks supercell. Our results suggest a new way to realise the highly transmittance metadevice with full 2π-phase control operating with the visible light which could be applicable in the imaging, metalens, holography, and display applications.

Reversible Image Contrast Manipulation with Thermally Tunable Dielectric Metasurfaces.

Increasing demand for higher resolution of miniaturized displays requires techniques achieving high contrast tunability of the images. Employing metasurfaces for image contrast manipulation is a new and rapidly growing field of research aiming to address this need. Here, a new technique to achieve image tuning in a reversible fashion is demonstrated by dielectric metasurfaces composed of subwavelength resonators. It is demonstrated that by controlling the temperature of a metasurface the encoded transmission pattern can be tuned. To this end, two sets of nanoresonators composed of nonconcentric silicon disks with a hole that exhibit spectrally sharp Fano resonances and forming a Yin-Yang pattern are designed and fabricated. Through exploitation of the thermo-optical properties of silicon, full control of the contrast of the Yin-Yang image is demonstrated by altering the metasurface temperature by ΔT ≈ 100 °C. This is the first demonstrated technique to control an image contrast by temperature. Importantly, the turning technique does not require manipulating the external stimulus, such as polarization or angle of the illumination and/or the refractive index of this environment. These results open many opportunities for transparent displays, optical switches, and tunable illumination systems.

Simultaneously nearly zero forward and nearly zero backward scattering objects.

With theoretical analyses and numerical calculations, we show that a passive scatterer at the sub-wavelength scale can simultaneously exhibit both nearly zero forward scattering (NZFS) and nearly zero backward scattering (NZBS). It is related to the interference of dipolar quadrupole modes of different origin, leading to coexistence of Kerker's first and second conditions at the same time. For optical frequencies, we propose two different sets of composited materials in multi-layered nano-structures, i.e., CdTe/Si/TiO2 and TiO2/Au/Si, for the experimental realization.

Lighting up silicon nanoparticles with Mie resonances.

As one of the most important semiconductors, silicon has been used to fabricate electronic devices, waveguides, detectors, solar cells, etc. However, the indirect bandgap and low quantum efficiency (10-7) hinder the use of silicon for making good emitters. For integrated photonic circuits, silicon-based emitters with sizes in the range of 100-300 nm are highly desirable. Here, we show the use of the electric and magnetic resonances in silicon nanoparticles to enhance the quantum efficiency and demonstrate the white-light emission from silicon nanoparticles with feature sizes of ~200 nm. The magnetic and electric dipole resonances are employed to dramatically increase the relaxation time of hot carriers, while the magnetic and electric quadrupole resonances are utilized to reduce the radiative recombination lifetime of hot carriers. This strategy leads to an enhancement in the quantum efficiency of silicon nanoparticles by nearly five orders of magnitude as compared with bulk silicon, taking the three-photon-induced absorption into account.