Measurement of geometric dephasing using a superconducting qubit.

A quantum system interacting with its environment is subject to dephasing, which ultimately destroys the information it holds. Here we use a superconducting qubit to experimentally show that this dephasing has both dynamic and geometric origins. It is found that geometric dephasing, which is present even in the adiabatic limit and when no geometric phase is acquired, can either reduce or restore coherence depending on the orientation of the path the qubit traces out in its projective Hilbert space. It accompanies the evolution of any system in Hilbert space subjected to noise.

Observation of Dicke superradiance for two artificial atoms in a cavity with high decay rate.

An individual excited two-level system decays to its ground state in a process known as spontaneous emission. The probability of detecting the emitted photon decreases exponentially with the time passed since its excitation. In 1954, Dicke first considered the more subtle situation in which two emitters decay in close proximity to each other. He argued that the emission dynamics of a single two-level system is altered by the presence of a second one, even if it is in its ground state. Here, we present a close to ideal realization of Dicke's original two-spin Gedankenexperiment, using a system of two individually controllable superconducting qubits weakly coupled to a fast decaying microwave cavity. The two-emitter case of superradiance is explicitly demonstrated both in time-resolved measurements of the emitted power and by fully reconstructing the density matrix of the emitted field in the photon number basis.

Quantum-limited amplification and entanglement in coupled nonlinear resonators.

We demonstrate a coupled cavity realization of a Bose-Hubbard dimer to achieve quantum-limited amplification and to generate frequency entangled microwave fields with squeezing parameters well below -12 dB. In contrast to previous implementations of parametric amplifiers, our dimer can be operated both as a degenerate and as a nondegenerate amplifier. The large measured gain-bandwidth product of more than 250 MHz for the nondegenerate operation and the saturation at input photon numbers as high as 2000 per µs are both expected to be improvable even further, while maintaining wide frequency tunability of about 2 GHz. Featuring flexible control over all relevant system parameters, the presented Bose-Hubbard dimer based on lumped element circuits has significant potential as an elementary cell in nonlinear cavity arrays for quantum simulations.

Geometric phase and nonadiabatic effects in an electronic harmonic oscillator.

Steering a quantum harmonic oscillator state along cyclic trajectories leads to a path-dependent geometric phase. Here we describe its experimental observation in an electronic harmonic oscillator. We use a superconducting qubit as a nonlinear probe of the phase, which is otherwise unobservable due to the linearity of the oscillator. We show that the geometric phase is, for a variety of cyclic paths, proportional to the area enclosed in the quadrature plane. At the transition to the nonadiabatic regime, we study corrections to the phase and dephasing of the qubit caused by qubit-resonator entanglement. In particular, we identify parameters for which this dephasing mechanism is negligible even in the nonadiabatic regime. The demonstrated controllability makes our system a versatile tool to study geometric phases in open quantum systems and to investigate their potential for quantum information processing.

Quantum-optical catalysis: generating nonclassical states of light by means of linear optics.

We report preparation and characterization of coherent superposition states t[0>+alpha]1> of the electromagnetic field by conditional measurements on a beam splitter. This state is generated in one of the beam splitter output channels if a coherent state [alpha> and a single-photon Fock state [1> are present in the two input ports and a single photon is registered in the other beam splitter output. The single photon thus plays a role of a "catalyst:" it is explicitly present in both the input and the output channels of the interaction yet facilitates generation of a nonclassical state of light.

Tests of relativity using a cryogenic optical resonator.

A 190-day comparison of the optical frequencies defined by an optical cavity and a molecular electronic transition is analyzed for the velocity independence of the speed of light (Kennedy-Thorndike test) and the universality of the gravitational redshift. The modulation of the laboratory velocity and the gravitational potential were provided by Earth's orbital motion around the Sun. We find a velocity-dependence coefficient of (1.9+/-2.1)x10(-5), 3 times lower compared to the best previous test. Alternatively, the data confirm the gravitational redshift for an electronic transition at the 4% level. Prospects for significant improvements of the tests are discussed.

Quantum state reconstruction of the single-photon Fock state.

We have reconstructed the quantum state of optical pulses containing single photons using the method of phase-randomized pulsed optical homodyne tomography. The single-photon Fock state 1> was prepared using conditional measurements on photon pairs born in the process of parametric down-conversion. A probability distribution of the phase-averaged electric field amplitudes with a strongly non-Gaussian shape is obtained with the total detection efficiency of (55+/-1)%. The angle-averaged Wigner function reconstructed from this distribution shows a strong dip reaching classically impossible negative values around the origin of the phase space.

A single gold particle as a probe for apertureless scanning near-field optical microscopy.

We report on the fabrication, characterization and application of a probe consisting of a single gold nanoparticle for apertureless scanning near-field optical microscopy. Particles with diameters of 100 nm have been successfully and reproducibly mounted at the end of sharp glass fibre tips. We present the first optical images taken with such a probe. We have also recorded plasmon resonances of gold particles and discuss schemes for exploiting the wavelength dependence of their scattering cross-section for a novel form of apertureless scanning near-field optical microscopy.

All-solid-state, tunable, single-frequency source of yellow light for high-resolution spectroscopy.

We demonstrate a cw doubly resonant optical parametric oscillator that is frequency doubled in an external resonant cavity to the visible spectral range. We obtained single-frequency radiation in the range 565-590 nm with as much as 3.8 mW of power, which is continuously tunable over an 18-GHz range and step tunable over 160 GHz. The source is well suited for high-resolution spectroscopy in the visible region. As a demonstration, we performed persistent hyperfine spectral hole-burning spectroscopy of Eu(3+): Y(2)SiO(5) . Reliable operation of the source permitted studies of the hole's lifetime over several hours.

High-resolution Doppler-free molecular spectroscopy with a continuous-wave optical parametric oscillator.

We present a reliable, narrow-linewidth (100-kHz) continous-wave optical parametric oscillator (OPO) suitable for high-resolution spectroscopy applications. The singly resonant OPO with a resonated pump is based on periodically poled lithium niobate crystal and features a specially designed intracavity etalon, which permits precise tuning to any desired wavelength in a wide range. We demonstrate Doppler-free spectroscopy of a rovibrational transition of methane at 3.39 mum.

Ultrasensitive pulsed, balanced homodyne detector: application to time-domain quantum measurements.

A pulsed, balanced homodyne detector has been developed for precise measurement of the electric field quadratures of pulsed optical quantum states. A high level of common mode suppression (>85 dB) and low electronic noise (730 electrons per pulse) provide a signal-to-noise ratio of 14 dB for measurement of the quantum noise of individual pulses. Measurements at repetition rates as high as 1 MHz are possible. As a test, quantum tomography of the coherent state was performed, and the Wigner function and the density matrix were reconstructed with 99.5% fidelity. The detection system can be used for ultrarsensitive balanced detection in cw mode, e.g., for weak absorption measurements.

Optical microscopy using a single-molecule light source

Rapid progress in science on nanoscopic scales has promoted increasing interest in techniques of ultrahigh-resolution optical microscopy. The diffraction limit can be surpassed by illuminating an object in the near field through a sub-wavelength aperture at the end of a sharp metallic probe. Proposed modifications of this technique involve replacing the physical aperture by a nanoscopic active light source. Advances in the spatial and spectral detection of individual fluorescent molecules, using near-field and far-field methods, suggest the possibility of using a single molecule as the illumination source. Here we present optical images taken with a single molecule as a point-like source of illumination, by combining fluorescence excitation spectroscopy with shear-force microscopy. Our single-molecule probe has potential for achieving molecular resolution in optical microscopy; it should also facilitate controlled studies of nanometre-scale phenomena (such as resonant energy transfer) with improved lateral and axial spatial resolution.

Nanophase-separated polymer films as high-performance antireflection coatings

Optical surfaces coated with a thin layer to improve light transmission are ubiquitous in everyday optical applications as well as in industrial and scientific instruments. Discovered first in 1817 by Fraunhofer, the coating of lenses became standard practice in the 1930s. In spite of intensive research, broad-band antireflection coatings are still limited by the lack of materials with low refractive indices. A method based on the phase separation of a macromolecular liquid to generate nanoporous polymer films is demonstrated that creates surfaces with high optical transmission.

A novel fabrication method for fluorescence-based apertureless scanning near-field optical microscope probes.

We report a novel method for the fabrication of probes with localized sub-wavelength fluorescing media at their extremities. We present our first results and discuss future plans to extend this technique to the systematic fabrication of fluorescent probes for apertureless scanning near-field optical microscopy.

A single molecule as a probe of optical intensity distribution.

Single terrylene molecules embedded in microscopic p-terphenyl crystals are identified with the technique of fluorescence excitation spectroscopy. By use of the architecture of a scanning-probe microscope at T = 1.4 K , a single molecule is scanned through an excitation laser beam while the fluorescence signal is recorded. In this manner we have mapped the intensity distribution in a one-dimensional optical standing wave, demonstrating the potential of a single molecule as a nanometric probe. We discuss future experiments aimed at combining the high spatial and spectral sensitivity of a single molecule.

Single-frequency continuous-wave radiation from 0.77 to 1.73 microm generated by a green-pumped optical parametric oscillator with periodically poled LiTaO3.

We describe a cw optical parametric oscillator (OPO) with multigrating periodically poled LiTaO(3) . Pumped by a single-frequency 532-nm laser, the OPO emits single-frequency radiation at wavelengths from 0.77 to 1.73 microm with as much as 60 mW of output power. Mode-hop-free operation for as long as 50 min, a low frequency drift (<70 MHz/h), and as much as 700-MHz continuous frequency tuning of signal and idler are demonstrated.

Generation of strongly squeezed continuous-wave light at 1064 nm.

A compact and effcient source of amplitude-squeezed light is described. It employs a semi-monolithic degenerate MgO:LiNbO(3) optical parametric amplifier pumped by a frequency-doubled Nd:YAG laser at 532 nm. Injection-seeding of the amplifier by a 1064 nm wave permits active stabilization of the cavity length and stable operation. At a pump power of 380 mW, a maximum noise reduction of 6.5 dB in the amplitude fluctuations of the 0.2 mW 1064 nm wave was detected. The average detected noise reduction in continuous operation over 14 minutes was 6.2 dB. Taking the detection effciency into account, this corresponds to a squeezing of 7.2 dB in the emitted wave.

Changes in respiratory function after one and three hours of exposure to formaldehyde in non-smoking subjects.

OBJECTIVE: To determine the changes in respiratory function within one hour and three hours of exposure to formaldehyde and investigate the relation between exposure to formaldehyde and acute changes in respiratory function. METHOD: Respiratory function of 50 non-smoking medical students exposed to formaldehyde in a gross anatomy laboratory were compared with respiratory function of 36 non-exposed, non-smoking physiotherapy students. Formaldehyde concentrations were measured in the breathing zone of each exposed subject and in the general work environment. RESULTS: Formaldehyde concentrations in the breathing zone of exposed subjects generally exceeded recommended standards. On average, the variables of respiratory function of both the exposed and the control subjects increased significantly within one hour and from one to three hours after exposure. The increase in respiratory function of the exposed subjects was significantly less than that of the control subjects. There was no meaningful correlation between concentration of formaldehyde in the breathing zone and changes in the respiratory function of exposed subjects. CONCLUSION: As the increase in the respiratory function of the subjects can be attributable to normal diurnal variation, the significantly lower increase in respiratory function of the exposed group than in the control group is probably due to exposure to formaldehyde. The results of this study do not, however, support a dose-response relation.

Toward an optical synthesizer: a single-frequency parametric oscillator using periodically poled LiNbO(3).

We demonstrate single-frequency operation of a cw quasi-phase-matched singly resonant optical parametric oscillator (SRO). We obtained widely tunable output from 1.66 to 1.99 mum (signal) and from 2.29 to 2.96 mum (idler) by employing a periodically poled lithium niobate multigrating chip. Using a single-frequency miniature Nd:YAG ring laser as a pump source results in SRO output with high spectral purity and frequency stability(<10 MHz/min), which can be continuously tuned over 2 GHz without mode hops. We obtain a minimum SRO threshold of 260mW by resonating the pump wave in the SRO cavity.