Dichotomous dynamics of magnetic monopole fluids.

A recent advance in the study of emergent magnetic monopoles was the discovery that monopole motion is restricted to dynamical fractal trajectories [J. N. Hallén et al., Science 378, 1218 (2022)], thus explaining the characteristics of magnetic monopole noise spectra [R. Dusad et al., Nature 571, 234 (2019); A. M. Samarakoon et al., Proc. Natl. Acad. Sci. U.S.A. 119, e2117453119 (2022)]. Here, we apply this novel theory to explore the dynamics of field-driven monopole currents, finding them composed of two quite distinct transport processes: initially swift fractal rearrangements of local monopole configurations followed by conventional monopole diffusion. This theory also predicts a characteristic frequency dependence of the dissipative loss angle for AC field-driven currents. To explore these novel perspectives on monopole transport, we introduce simultaneous monopole current control and measurement techniques using SQUID-based monopole current sensors. For the canonical material Dy2Ti2O7, we measure [Formula: see text], the time dependence of magnetic flux threading the sample when a net monopole current [Formula: see text] is generated by applying an external magnetic field [Formula: see text] These experiments find a sharp dichotomy of monopole currents, separated by their distinct relaxation time constants before and after t ~[Formula: see text] from monopole current initiation. Application of sinusoidal magnetic fields [Formula: see text] generates oscillating monopole currents whose loss angle [Formula: see text] exhibits a characteristic transition at frequency [Formula: see text] over the same temperature range. Finally, the magnetic noise power is also dichotomic, diminishing sharply after t ~[Formula: see text]. This complex phenomenology represents an unprecedented form of dynamical heterogeneity generated by the interplay of fractionalization and local spin configurational symmetry.

Domain Wall Dynamics in Classical Spin Chains: Free Propagation, Subdiffusive Spreading, and Soliton Emission.

The nonequilibrium dynamics of domain wall initial states in a classical anisotropic Heisenberg chain exhibits a striking coexistence of apparently linear and nonlinear behaviors: the propagation and spreading of the domain wall can be captured quantitatively by linear, i.e., noninteracting, spin wave theory absent its usual justifications; while, simultaneously, for a wide range of easy-plane anisotropies, emission can take the place of stable solitons-a process and objects intrinsically associated with interactions and nonlinearities. The easy-axis domain wall only has transient dynamics, the isotropic one broadens diffusively, while the easy-plane one yields a pair of ballistically counterpropagating domain walls which, unusually, broaden subdiffusively, their width scaling as t^{1/3}.

Spectral Response of Disorder-Free Localized Lattice Gauge Theories.

We show that certain lattice gauge theories exhibiting disorder-free localization have a characteristic response in spatially averaged spectral functions: a few sharp peaks combined with vanishing response in the zero frequency limit. This reflects the discrete spectra of small clusters of kinetically active regions formed in such gauge theories when they fragment into spatially finite clusters in the localized phase due to the presence of static charges. We obtain the transverse component of the dynamic structure factor, which is probed by neutron scattering experiments, deep in this phase from a combination of analytical estimates and a numerical cluster expansion. We also show that local spectral functions of large finite clusters host discrete peaks whose positions agree with our analytical estimates. Further, information spreading, diagnosed by an unequal time commutator, halts due to real space fragmentation. Our results can be used to distinguish the disorder-free localized phase from conventional paramagnetic counterparts in those frustrated magnets which might realize such an emergent gauge theory.

Spurious Symmetry Enhancement in Linear Spin Wave Theory and Interaction-Induced Topology in Magnons.

Linear spin wave theory (LSWT) is the standard technique to compute the spectra of magnetic excitations in quantum materials. In this Letter, we show that LSWT, even under ordinary circumstances, may fail to implement the symmetries of the underlying ordered magnetic Hamiltonian leading to spurious degeneracies. In common with pseudo-Goldstone modes in cases of quantum order by disorder these degeneracies tend to be lifted by magnon-magnon interactions. We show how, instead, the correct symmetries may be restored at the level of LSWT. In the process we give examples, supported by nonperturbative matrix product based time evolution calculations, where symmetry dictates topological features but where LSWT fails to implement them. We also comment on possible spin split magnons in MnF_{2} and similar rutiles by analogy to recently proposed altermagnets.

Abundance of Hard-Hexagon Crystals in the Quantum Pyrochlore Antiferromagnet.

We propose a simple family of valence-bond crystals as potential ground states of the S=1/2 and S=1 Heisenberg antiferromagnet on the pyrochlore lattice. Exponentially numerous in the linear size of the system, these can be visualized as hard-hexagon coverings, with each hexagon representing a resonating valence-bond ring. This ensemble spontaneously breaks rotation, inversion, and translation symmetries. A simple, yet accurate, variational wave function allows a precise determination of the energy, confirmed by the density matrix renormalization group and numerical linked cluster expansion, and extended by an analysis of excited states. The identification of the origin of the stability indicates applicability to a broad class of frustrated lattices, which we demonstrate for the checkerboard and ruby lattices. Our work suggests a perspective on such quantum magnets, in which unfrustrated motifs are effectively uncoupled by the frustration of their interactions.

Identifying and Constructing Complex Magnon Band Topology.

Magnetically ordered materials tend to support bands of coherent propagating spin wave, or magnon, excitations. Topologically protected surface states of magnons offer a new path toward coherent spin transport for spintronics applications. In this work we explore the variety of topological magnon band structures and provide insight into how to efficiently identify topological magnon bands in materials. We do this by adapting the topological quantum chemistry approach that has used constraints imposed by time reversal and crystalline symmetries to enumerate a large class of topological electronic bands. We show how to identify physically relevant models of gapped magnon band topology by using so-called decomposable elementary band representations, and in turn discuss how to use symmetry data to infer the presence of exotic symmetry enforced nodal topology.

From Dual Unitarity to Generic Quantum Operator Spreading.

Dual-unitary circuits are paradigmatic examples of exactly solvable yet chaotic quantum many-body systems, but solvability naturally goes along with a degree of nongeneric behavior. By investigating the effect of weakly broken dual unitarity on the spreading of local operators, we study whether, and how, small deviations from dual unitarity recover fully generic many-body dynamics. We present a discrete path-integral formula for the out-of-time-order correlator and recover a butterfly velocity smaller than the light-cone velocity, v_{B}

Dynamical fractal and anomalous noise in a clean magnetic crystal.

Fractals-objects with noninteger dimensions-occur in manifold settings and length scales in nature. In this work, we identify an emergent dynamical fractal in a disorder-free, stoichiometric, and three-dimensional magnetic crystal in thermodynamic equilibrium. The phenomenon is born from constraints on the dynamics of the magnetic monopole excitations in spin ice, which restrict them to move on the fractal. This observation explains the anomalous exponent found in magnetic noise experiments in the spin ice compound Dy2Ti2O7, and it resolves a long-standing puzzle about its rapidly diverging relaxation time. The capacity of spin ice to exhibit such notable phenomena suggests that there will be further unexpected discoveries in the cooperative dynamics of even simple topological many-body systems.

Suppression of Interband Heating for Random Driving.

Heating to high-lying states strongly limits the experimental observation of driving induced nonequilibrium phenomena, particularly when the drive has a broad spectrum. Here we show that, for entire families of structured random drives known as random multipolar drives, particle excitation to higher bands can be well controlled even away from a high-frequency driving regime. This opens a window for observing drive-induced phenomena in a long-lived prethermal regime in the lowest band.

Skin effect as a probe of transport regimes in Weyl semimetals.

SignificanceWeyl semimetals are a class of three-dimensional materials, whose low-energy excitations mimic massless fermions. In consequence they exhibit various unusual transport properties related to the presence of chiral anomalies, a subtle quantum phenomenon that denotes the breaking of the classical chiral symmetry by quantum fluctuations. In this work we present a universal description of transport in weakly disordered Weyl semimetals with several scattering mechanisms taken into account. Our work predicts the existence of a new anomaly-induced transport regime in these materials and gives a crisp experimental signature of a chiral anomaly in optical conductivity measurements. Finally, by also capturing the hydrodynamic regime of quasiparticles, our construction bridges the gap between developments in electronic fluid mechanics and three-dimensional semimetals.

Anomalous magnetic noise in an imperfectly flat landscape in the topological magnet Dy2Ti2O7.

Noise generated by motion of charge and spin provides a unique window into materials at the atomic scale. From temperature of resistors to electrons breaking into fractional quasiparticles, "listening" to the noise spectrum is a powerful way to decode underlying dynamics. Here, we use ultrasensitive superconducting quantum interference device (SQUIDs) to probe the puzzling noise in a frustrated magnet, the spin-ice compound Dy2Ti2O7 (DTO), revealing cooperative and memory effects. DTO is a topological magnet in three dimensions-characterized by emergent magnetostatics and telltale fractionalized magnetic monopole quasiparticles-whose real-time dynamical properties have been an enigma from the very beginning. We show that DTO exhibits highly anomalous noise spectra, differing significantly from the expected Brownian noise of monopole random walks, in three qualitatively different regimes: equilibrium spin ice, a "frozen" regime extending to ultralow temperatures, and a high-temperature "anomalous" paramagnet. We present several distinct mechanisms that give rise to varied colored noise spectra. In addition, we identify the structure of the local spin-flip dynamics as a crucial ingredient for any modeling. Thus, the dynamics of spin ice reflects the interplay of local dynamics with emergent topological degrees of freedom and a frustration-generated imperfectly flat energy landscape, and as such, it points to intriguing cooperative and memory effects for a broad class of magnetic materials.

Long-lived solitons and their signatures in the classical Heisenberg chain.

Motivated by the Kardar-Parisi-Zhang (KPZ) scaling recently observed in the classical ferromagnetic Heisenberg chain, we investigate the role of solitonic excitations in this model. We find that the Heisenberg chain, although well known to be nonintegrable, supports a two-parameter family of long-lived solitons. We connect these to the exact soliton solutions of the integrable Ishimori chain with ln(1+S_{i}·S_{j}) interactions. We explicitly construct infinitely long-lived stationary solitons, and provide an adiabatic construction procedure for moving soliton solutions, which shows that Ishimori solitons have a long-lived Heisenberg counterpart when they are not too narrow and not too fast moving. Finally, we demonstrate their presence in thermal states of the Heisenberg chain, even when the typical soliton width is larger than the spin correlation length, and argue that these excitations likely underlie the KPZ scaling.

Rabi Regime of Current Rectification in Solids.

We investigate rectified currents in response to oscillating electric fields in systems lacking inversion and time-reversal symmetries. These currents, in second-order perturbation theory, are inversely proportional to the relaxation rate, and, therefore, naively diverge in the ideal clean limit. Employing a combination of the nonequilibrium Green function technique and Floquet theory, we show that this is an artifact of perturbation theory, and that there is a well-defined periodic steady state akin to Rabi oscillations leading to finite rectified currents in the limit of weak coupling to a thermal bath. In this Rabi regime the rectified current scales as the square root of the radiation intensity, in contrast with the linear scaling of the perturbative regime, allowing us to readily diagnose it in experiments. More generally, our description provides a smooth interpolation from the ideal periodic Gibbs ensemble describing the Rabi oscillations of a closed system to the perturbative regime of rapid relaxation due to strong coupling to a thermal bath.

Emergent Fine Structure Constant of Quantum Spin Ice Is Large.

Condensed-matter systems provide alternative "vacua" exhibiting emergent low-energy properties drastically different from those of the standard model. A case in point is the emergent quantum electrodynamics (QED) in the fractionalized topological magnet known as quantum spin ice, whose magnetic monopoles set it apart from the familiar QED of the world we live in. Here, we show that the two greatly differ in their fine structure constant α, which parametrizes how strongly matter couples to light: α_{QSI} is more than an order of magnitude greater than α_{QED}≈1/137. Furthermore, α_{QSI}, the emergent speed of light, and all other parameters of the emergent QED, are tunable by engineering the microscopic Hamiltonian. We find that α_{QSI} can be tuned all the way from zero up to what is believed to be the strongest possible coupling beyond which QED confines. In view of the small size of its constrained Hilbert space, this marks out quantum spin ice as an ideal platform for studying exotic quantum field theories and a target for quantum simulation. The large α_{QSI} implies that experiments probing candidate condensed-matter realizations of quantum spin ice should expect to observe phenomena arising due to strong interactions.

Topological Route to New and Unusual Coulomb Spin Liquids.

Coulomb spin liquids are topological magnetic states obeying an emergent Gauss law. Little distinction has been made between different kinds of Coulomb liquids. Here we show how a series of distinct Coulomb liquids can be generated straightforwardly by varying the constraints on a classical spin system. This leads to pair creation, and coalescence, of topological defects of an underlying vector field. The latter makes higher-rank spin liquids, of recent interest in the context of fracton theories, with attendant multifold pinch points in the structure factor, appear naturally. New Coulomb liquids with an abundance of pinch points also arise. We thus establish a new and general route to uncovering exotic Coulomb liquids, via the manipulation of topological defects in momentum space.

Super-Resonant Transport of Topological Surface States Subjected to In-Plane Magnetic Fields.

Magnetic oscillations of Dirac surface states of topological insulators are typically expected to be associated with the formation of Landau levels or the Aharonov-Bohm effect. We instead study the conductance of Dirac surface states subjected to an in-plane magnetic field in the presence of a barrier potential. Strikingly, we find that, in the case of large barrier potentials, the surface states exhibit pronounced oscillations in the conductance when varying the magnetic field, in the absence of Landau levels or the Aharonov-Bohm effect. These novel magnetic oscillations are attributed to the emergence of super-resonant transport by tuning the magnetic field, in which many propagating modes cross the barrier with perfect transmission. In the case of small and moderate barrier potentials, we identify a positive magnetoconductance due to the increase of the Fermi surface by tilting the surface Dirac cone. Moreover, we show that for weak magnetic fields, the conductance displays a shifted sinusoidal dependence on the field direction with period π and phase shift determined by the tilting direction with respect to the field direction. Our predictions can be applied to various topological insulators, such as HgTe and Bi_{2}Se_{3}, and provide important insights into exploring and understanding exotic magnetotransport properties of topological surface states.

Fractonic View of Folding and Tearing Paper: Elasticity of Plates Is Dual to a Gauge Theory with Vector Charges.

We offer a fractonic perspective on a familiar observation-a flat sheet of paper can be folded only along a straight line if one wants to avoid the creation of additional creases or tears. Our core underlying technical result is the establishment of a duality between the theory of elastic plates and a fractonic gauge theory with a second rank symmetric electric field tensor, a scalar magnetic field, a vector charge, and a symmetric tensor current. Bending moment and momentum of the plate are dual to the electric and magnetic fields, respectively. While the flexural waves correspond to the quadratically dispersing photon of the gauge theory, a fold defect is dual to its vector charge. Crucially, the fractonic condition constrains the latter to move only along its direction, i.e., the fold's growth direction. By contrast, fracton motion in the perpendicular direction amounts to tearing the paper.

Rigorous Bounds on the Heating Rate in Thue-Morse Quasiperiodically and Randomly Driven Quantum Many-Body Systems.

The nonequilibrium quantum dynamics of closed many-body systems is a rich yet challenging field. While recent progress for periodically driven (Floquet) systems has yielded a number of rigorous results, our understanding on quantum many-body systems driven by rapidly varying but aperiodic and quasiperiodic driving is still limited. Here, we derive rigorous, nonperturbative, bounds on the heating rate in quantum many-body systems under Thue-Morse quasiperiodic driving and under random multipolar driving, the latter being a tunably randomized variant of the former. In the process, we derive a static effective Hamiltonian that describes the transient prethermal state, including the dynamics of local observables. Our bound for Thue-Morse quasiperiodic driving suggests that the heating time scales like (ω/g)^{-C ln(ω/g)} with a positive constant C and a typical energy scale g of the Hamiltonian, in agreement with our numerical simulations.

Possible Inversion Symmetry Breaking in the S=1/2 Pyrochlore Heisenberg Magnet.

We address the ground-state properties of the long-standing and much-studied three-dimensional quantum spin liquid candidate, the S=1/2 pyrochlore Heisenberg antiferromagnet. By using SU(2) density-matrix renormalization group (DMRG), we are able to access cluster sizes of up to 128 spins. Our most striking finding is a robust spontaneous inversion symmetry breaking, reflected in an energy density difference between the two sublattices of tetrahedra, familiar as a starting point of earlier perturbative treatments. We also determine the ground-state energy, E_{0}/N_{sites}=-0.490(6)J, by combining extrapolations of DMRG with those of a numerical linked cluster expansion. These findings suggest a scenario in which a finite-temperature spin liquid regime gives way to a symmetry-broken state at low temperatures.

Random Multipolar Driving: Tunably Slow Heating through Spectral Engineering.

Driven quantum systems may realize novel phenomena absent in static systems, but driving-induced heating can limit the timescale on which these persist. We study heating in interacting quantum many-body systems driven by random sequences with n-multipolar correlations, corresponding to a polynomially suppressed low-frequency spectrum. For n≥1, we find a prethermal regime, the lifetime of which grows algebraically with the driving rate, with exponent 2n+1. A simple theory based on Fermi's golden rule accounts for this behavior. The quasiperiodic Thue-Morse sequence corresponds to the n→∞ limit and, accordingly, exhibits an exponentially long-lived prethermal regime. Despite the absence of periodicity in the drive, and in spite of its eventual heat death, the prethermal regime can host versatile nonequilibrium phases, which we illustrate with a random multipolar discrete time crystal.