RESUMEN
The distribution and migration of artificial fallout radionuclides in natural soils has been profusely studied for assessing radioecological impacts and predicting their long-term behaviour, among other topics. Despite the standardized use of the analytical solutions of a simplified convection-diffusion equation (CDE), there are still some concerns and open questions. This work is aimed at contributing to the understanding of basic processes governing the distribution of fallout radionuclides in vegetated soils with rhizospheres. It studies 210Pb and 137Cs in soil cores and vegetal samples from Chréa National Park, in Algeria, along with other natural radionuclides and some major and trace elements. Results include surficial and depth distributions of radionuclide concentrations, and site and plant-specific concentration ratios (CR). Inventories of 137Cs (3620 ± 120 Bq m-2) and 210Pbexc (9000 ± 900 Bq m-2) in soils are typical from global fallout in high precipitation areas in the Northern Hemisphere. A simple model of a polyphasic soil, including rhizospheres, provides a realistic description in the studied case, where plant roots occupy about 45% of the volume in the 0-10 cm interval, with a high porosity around rhizomes. This composite soil matrix explains the different patterns observed in the depth distribution of the studied elements. The depth-distributions of 137Cs and 210Pbexc have been modelled with different approaches: i) analytical solution of the CDE with mean annual convection and large observation times; ii) as before, but with convection representing infiltration events and short observation times; iii) numerical modelling of the 137Cs profile in the mineral phase using CDE with fast initial distributions. The three approaches fit the empirical data, but they predict different time evolutions. The approach iii) provides a more realistic description. Results are questioning the common accepted analysis and its predictive use.
Asunto(s)
Monitoreo de Radiación , Suelo , Argelia , Parques Recreativos , RizosferaRESUMEN
The common mussel Mytilus galloprovincialis was selected as unique biomonitor species to implement a regional monitoring programme, the CIESM Mediterranean Mussel Watch (MMW), in the Mediterranean and Black Seas. As of today, and upon standardization of the methodological approach, the MMW Network has been able to quantify (137)Cs levels in mussels from 60 coastal stations and to produce the first distribution map of this artificial radionuclide at the scale of the entire Mediterranean and Black Seas. While measured (137)Cs levels were found to be very low (usually < 1 Bq kg(-1) wet wt) (137)Cs activity concentrations in the Black Sea and North Aegean Sea were up to two orders of magnitude higher than those in the western Mediterranean Basin. Such effects, far from representing a threat to human populations or the environment, reflect a persistent signature of the Chernobyl fallout in this area.