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1.
Environ Sci Technol ; 57(29): 10708-10720, 2023 07 25.
Artículo en Inglés | MEDLINE | ID: mdl-37437161

RESUMEN

Particulate matter air pollution is a leading cause of global mortality, particularly in Asia and Africa. Addressing the high and wide-ranging air pollution levels requires ambient monitoring, but many low- and middle-income countries (LMICs) remain scarcely monitored. To address these data gaps, recent studies have utilized low-cost sensors. These sensors have varied performance, and little literature exists about sensor intercomparison in Africa. By colocating 2 QuantAQ Modulair-PM, 2 PurpleAir PA-II SD, and 16 Clarity Node-S Generation II monitors with a reference-grade Teledyne monitor in Accra, Ghana, we present the first intercomparisons of different brands of low-cost sensors in Africa, demonstrating that each type of low-cost sensor PM2.5 is strongly correlated with reference PM2.5, but biased high for ambient mixture of sources found in Accra. When compared to a reference monitor, the QuantAQ Modulair-PM has the lowest mean absolute error at 3.04 µg/m3, followed by PurpleAir PA-II (4.54 µg/m3) and Clarity Node-S (13.68 µg/m3). We also compare the usage of 4 statistical or machine learning models (Multiple Linear Regression, Random Forest, Gaussian Mixture Regression, and XGBoost) to correct low-cost sensors data, and find that XGBoost performs the best in testing (R2: 0.97, 0.94, 0.96; mean absolute error: 0.56, 0.80, and 0.68 µg/m3 for PurpleAir PA-II, Clarity Node-S, and Modulair-PM, respectively), but tree-based models do not perform well when correcting data outside the range of the colocation training. Therefore, we used Gaussian Mixture Regression to correct data from the network of 17 Clarity Node-S monitors deployed around Accra, Ghana, from 2018 to 2021. We find that the network daily average PM2.5 concentration in Accra is 23.4 µg/m3, which is 1.6 times the World Health Organization Daily PM2.5 guideline of 15 µg/m3. While this level is lower than those seen in some larger African cities (such as Kinshasa, Democratic Republic of the Congo), mitigation strategies should be developed soon to prevent further impairment to air quality as Accra, and Ghana as a whole, rapidly grow.


Asunto(s)
Contaminantes Atmosféricos , Contaminación del Aire , Contaminantes Atmosféricos/análisis , Ghana , Monitoreo del Ambiente , República Democrática del Congo , Material Particulado/análisis , Contaminación del Aire/análisis
2.
ACS Earth Space Chem ; 6(4): 1011-1021, 2022 Apr 21.
Artículo en Inglés | MEDLINE | ID: mdl-35495364

RESUMEN

Air pollution is a leading cause of global premature mortality and is especially prevalent in many low- and middle-income countries (LMICs). In sub-Saharan Africa, preliminary monitoring networks, satellite retrievals of air-quality-relevant species, and air quality models show ambient fine particulate matter (PM2.5) concentrations that far exceed the World Health Organization guidelines, yet many areas remain largely unmonitored and understudied. Deploying a network of five low-cost PurpleAir PM2.5 monitors over 2 years (2019-2021), we present the first multiyear ambient air pollution monitoring data results from Lomé, Togo, a major West African coastal city with a population of about 1.4 million people. The full-study time period network-wide mean measured daily PM2.5 concentration is 23.5 µg m-3 m-3. The strong regional influence of the dry and dusty Harmattan wind increases the local average PM2.5 concentration by up to 58% during December through February, but the diurnal and weekly trends in PM2.5 are largely controlled by local influences. At all sites, more than 87% of measured days exceeded the new WHO Daily PM2.5 guidelines; these first measurements highlight the need for air quality improvement in a rapidly growing urban metropolis.

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