Non-thermal emission in gap-mode plasmon photoluminescence.

Photoluminescence from spatially inhomogeneous plasmonic nanostructures exhibits fascinating wavelength-dependent nonlinear behaviors due to the intraband recombination of hot electrons excited into the conduction band of the metal. The properties of the excited carrier distribution and the role of localized plasmonic modes are subjects of debate. In this work, we use plasmonic gap-mode resonators with precise nanometer-scale confinement to show that the nonlinear photoluminescence behavior can become dominated by non-thermal contributions produced by the excited carrier population that strongly deviates from the Fermi-Dirac distribution due to the confinement-induced large-momentum free carrier absorption beyond the dipole approximation. These findings open new pathways for controllable light conversion using nonequilibrium electron states at the nanoscale.

Nanoscale Transient Magnetization Gratings Created and Probed by Femtosecond Extreme Ultraviolet Pulses.

We utilize coherent femtosecond extreme ultraviolet (EUV) pulses from a free electron laser (FEL) to generate transient periodic magnetization patterns with periods as short as 44 nm. Combining spatially periodic excitation with resonant probing at the M-edge of cobalt allows us to create and probe transient gratings of electronic and magnetic excitations in a CoGd alloy. In a demagnetized sample, we observe an electronic excitation with a rise time close to the FEL pulse duration and ∼0.5 ps decay time indicative of electron-phonon relaxation. When the sample is magnetized to saturation in an external field, we observe a magnetization grating, which appears on a subpicosecond time scale as the sample is demagnetized at the maxima of the EUV intensity and then decays on the time scale of tens of picoseconds via thermal diffusion. The described approach opens multiple avenues for studying dynamics of ultrafast magnetic phenomena on nanometer length scales.

Nonclassical Spin Transfer Effects in an Antiferromagnet.

We simulate scattering of electrons by a chain of antiferromagnetically coupled quantum Heisenberg spins, to analyze spin-transfer effects not described by the classical models of magnetism. Our simulations demonstrate efficient excitation of dynamical states that would be forbidden by the semiclassical symmetries, such as generation of multiple magnetic excitation quanta by a single electron. Furthermore, quantum interference of spin wave functions enables generation of magnetization dynamics with amplitudes exceeding the transferred magnetic moment. The efficiency of excitation is almost independent of the electron spin polarization, and is governed mainly by the transfer of energy. Nonclassical spin transfer may thus enable efficient electronic control of antiferromagnets not limited by the classical constraints.

Controlled nonlinear magnetic damping in spin-Hall nano-devices.

Large-amplitude magnetization dynamics is substantially more complex compared to the low-amplitude linear regime, due to the inevitable emergence of nonlinearities. One of the fundamental nonlinear phenomena is the nonlinear damping enhancement, which imposes strict limitations on the operation and efficiency of magnetic nanodevices. In particular, nonlinear damping prevents excitation of coherent magnetization auto-oscillations driven by the injection of spin current into spatially extended magnetic regions. Here, we propose and experimentally demonstrate that nonlinear damping can be controlled by the ellipticity of magnetization precession. By balancing different contributions to anisotropy, we minimize the ellipticity and achieve coherent magnetization oscillations driven by spatially extended spin current injection into a microscopic magnetic disk. Our results provide a route for the implementation of efficient active spintronic and magnonic devices driven by spin current.

Excitation and Amplification of Spin Waves by Spin-Orbit Torque.

The emerging field of nanomagnonics utilizes high-frequency waves of magnetization-spin waves-for the transmission and processing of information on the nanoscale. The advent of spin-transfer torque has spurred significant advances in nanomagnonics, by enabling highly efficient local spin wave generation in magnonic nanodevices. Furthermore, the recent emergence of spin-orbitronics, which utilizes spin-orbit interaction as the source of spin torque, has provided a unique ability to exert spin torque over spatially extended areas of magnonic structures, enabling enhanced spin wave transmission. Here, it is experimentally demonstrated that these advances can be efficiently combined. The same spin-orbit torque mechanism is utilized for the generation of propagating spin waves, and for the long-range enhancement of their propagation, in a single integrated nanomagnonic device. The demonstrated system exhibits a controllable directional asymmetry of spin wave emission, which is highly beneficial for applications in nonreciprocal magnonic logic and neuromorphic computing.

Evidence for Dyakonov-Perel-like Spin Relaxation in Pt.

We utilize nanoscale spin valves with Pt spacer layers to characterize spin relaxation in Pt. Analysis of the spin lifetime indicates that Elliott-Yafet spin scattering is dominant at room temperature, but an unexpected intrinsic Dyakonov-Perel-like spin relaxation becomes dominant at cryogenic temperatures. We also observe suppression of spin relaxation in a Pt layer interfaced with a ferromagnet, likely caused by the competition between the effective exchange and spin-orbit fields.

Anti-reflection coating design for metallic terahertz meta-materials.

We demonstrate a silicon-based, single-layer anti-reflection coating that suppresses the reflectivity of metals at near-infrared frequencies, enabling optical probing of nano-scale structures embedded in highly reflective surroundings. Our design does not affect the interaction of terahertz radiation with metallic structures that can be used to achieve terahertz near-field enhancement. We have verified the functionality of the design by calculating and measuring the reflectivity of both infrared and terahertz radiation from a silicon/gold double layer as a function of the silicon thickness. We have also fabricated the unit cell of a terahertz meta-material, a dipole antenna comprising two 20-nm thick extended gold plates separated by a 2 µm gap, where the terahertz field is locally enhanced. We used the time-domain finite element method to demonstrate that such near-field enhancement is preserved in the presence of the anti-reflection coating. Finally, we performed magneto-optical Kerr effect measurements on a single 3-nm thick, 1-µm wide magnetic wire placed in the gap of such a dipole antenna. The wire only occupies 2% of the area probed by the laser beam, but its magneto-optical response can be clearly detected. Our design paves the way for ultrafast time-resolved studies, using table-top femtosecond near-infrared lasers, of dynamics in nano-structures driven by strong terahertz radiation.

Spin Transfer due to Quantum Magnetization Fluctuations.

We utilize a nanoscale magnetic spin-valve structure to demonstrate that current-induced magnetization fluctuations at cryogenic temperatures result predominantly from the quantum fluctuations enhanced by the spin transfer effect. The demonstrated spin transfer due to quantum magnetization fluctuations is distinguished from the previously established current-induced effects by a nonsmooth piecewise-linear dependence of the fluctuation intensity on current. It can be driven not only by the directional flows of spin-polarized electrons, but also by their thermal motion and by scattering of unpolarized electrons. This effect is expected to remain non-negligible even at room temperature, and entails a ubiquitous inelastic contribution to spin-polarizing properties of magnetic interfaces.

Excitation of coherent propagating spin waves by pure spin currents.

Utilization of pure spin currents not accompanied by the flow of electrical charge provides unprecedented opportunities for the emerging technologies based on the electron's spin degree of freedom, such as spintronics and magnonics. It was recently shown that pure spin currents can be used to excite coherent magnetization dynamics in magnetic nanostructures. However, because of the intrinsic nonlinear self-localization effects, magnetic auto-oscillations in the demonstrated devices were spatially confined, preventing their applications as sources of propagating spin waves in magnonic circuits using these waves as signal carriers. Here, we experimentally demonstrate efficient excitation and directional propagation of coherent spin waves generated by pure spin current. We show that this can be achieved by using the nonlocal spin injection mechanism, which enables flexible design of magnetic nanosystems and allows one to efficiently control their dynamic characteristics.

Magnetic nano-oscillator driven by pure spin current.

With the advent of pure-spin-current sources, spin-based electronic (spintronic) devices no longer require electrical charge transfer, opening new possibilities for both conducting and insulating spintronic systems. Pure spin currents have been used to suppress noise caused by thermal fluctuations in magnetic nanodevices, amplify propagating magnetization waves, and to reduce the dynamic damping in magnetic films. However, generation of coherent auto-oscillations by pure spin currents has not been achieved so far. Here we demonstrate the generation of single-mode coherent auto-oscillations in a device that combines local injection of a pure spin current with enhanced spin-wave radiation losses. Counterintuitively, radiation losses enable excitation of auto-oscillation, suppressing the nonlinear processes that prevent auto-oscillation by redistributing the energy between different modes. Our devices exhibit auto-oscillations at moderate current densities, at a microwave frequency tunable over a wide range. These findings suggest a new route for the implementation of nanoscale microwave sources for next-generation integrated electronics.

Direct observation and mapping of spin waves emitted by spin-torque nano-oscillators.

Dynamics induced by spin-transfer torque is a quickly developing topic in modern magnetism, which has initiated several new approaches to magnetic nanodevices. It is now well established that a spin-polarized electric current injected into a ferromagnetic layer through a nanocontact exerts a torque on the magnetization, leading to microwave-frequency precession detectable through the magnetoresistance effect. This phenomenon provides a way for the realization of tunable nanometre-size microwave oscillators, the so-called spin-torque nano-oscillators (STNOs). Present theories of STNOs are mainly based on pioneering works predicting emission of spin waves due to the spin torque. Despite intense experimental studies, until now this spin-wave emission has not been observed. Here, we report the first experimental observation and two-dimensional mapping of spin waves emitted by STNOs. We demonstrate that the emission is strongly directional, and the direction of the spin-wave propagation is steerable by the magnetic field. The information about the emitted spin waves obtained in our measurements is of key importance for the understanding of the physics of STNOs, and for the implementation of coupling between individual oscillators mediated by spin waves. Analysis shows that the observed directional emission is a general property inherent to any dynamical system with strongly anisotropic dispersion.

Fractional synchronization of spin-torque nano-oscillators.

We experimentally demonstrate a series of fractional synchronization regimes (Devil's staircase) in a spin-torque nano-oscillator driven by a microwave field. These regimes are characterized by rational relations between the driving frequency and the frequency of the oscillation. An analysis based on the phase model of auto-oscillator indicates that fractional synchronization becomes possible when the driving signal breaks the symmetry of the oscillation, while the synchronization ranges are determined by the geometry of the oscillation orbit. Measurements of fractional synchronization can be utilized to obtain information about the oscillation characteristics in nanoscale systems not accessible to direct imaging techniques.

Parametric excitation of a magnetic nanocontact by a microwave field.

We demonstrate that magnetic oscillations of a current-biased magnetic nanocontact can be parametrically excited by a microwave field applied at twice the resonant frequency of the oscillation. The threshold microwave amplitude for the onset of the oscillation decreases with increasing bias current, and vanishes at the transition to the auto-oscillation regime. Theoretical analysis shows that measurements of parametric excitation provide quantitative information about the relaxation rate, the spin transfer efficiency, and the nonlinearity of the nanomagnetic system.

Effect of polarized current on the magnetic state of an antiferromagnet.

We provide evidence for the effects of spin polarized current on a nanofabricated antiferromagnet incorporated into a spin-valve structure. The signatures of the current-induced effects include bipolar steps in differential resistance, current-induced changes of exchange bias correlated with these steps, and deviations from the statistics expected for thermally activated switching of spin valves. We explain our observations by a combination of spin torque exerted on the interfacial antiferromagnetic moments and electron-magnon scattering in an antiferromagnet.