Two-Dimensional Terahertz Spectroscopy of Nonlinear Phononics in the Topological Insulator MnBi_{2}Te_{4}.

The interaction of a single-cycle terahertz electric field with the topological insulator MnBi_{2}Te_{4} triggers strongly anharmonic lattice dynamics, promoting fully coherent energy transfer between the otherwise noninteracting Raman-active E_{g} and infrared (IR)-active E_{u} phononic modes. Two-dimensional terahertz spectroscopy combined with modeling based on the classical equations of motion and symmetry analysis reveals the multistage process underlying the excitation of the Raman-active E_{g} phonon. In this nonlinear combined photophononic process, the terahertz electric field first prepares a coherent IR-active E_{u} phononic state and subsequently interacts with this state to efficiently excite the E_{g} phonon.

Non-monotonic variation of the Kramers point band gap with increasing magnetic doping in BiTeI.

Polar Rashba-type semiconductor BiTeI doped with magnetic elements constitutes one of the most promising platforms for the future development of spintronics and quantum computing thanks to the combination of strong spin-orbit coupling and internal ferromagnetic ordering. The latter originates from magnetic impurities and is able to open an energy gap at the Kramers point (KP gap) of the Rashba bands. In the current work using angle-resolved photoemission spectroscopy (ARPES) we show that the KP gap depends non-monotonically on the doping level in case of V-doped BiTeI. We observe that the gap increases with V concentration until it reaches 3% and then starts to mitigate. Moreover, we find that the saturation magnetisation of samples under applied magnetic field studied by superconducting quantum interference device (SQUID) magnetometer has a similar behaviour with the doping level. Theoretical analysis shows that the non-monotonic behavior can be explained by the increase of antiferromagnetic coupled atoms of magnetic impurity above a certain doping level. This leads to the reduction of the total magnetic moment in the domains and thus to the mitigation of the KP gap as observed in the experiment. These findings provide further insight in the creation of internal magnetic ordering and consequent KP gap opening in magnetically-doped Rashba-type semiconductors.

Controlling magnetic domain wall velocity by femtosecond laser pulses.

Using the technique of double high-speed photography, we find that a femtosecond laser pulse is able to change the velocity of a moving domain wall in an yttrium iron garnet. The change depends on the light intensity and the domain wall velocity itself. To explain the results we propose a model in which the domain wall velocity is controlled by photo-induced generation of vertical Bloch lines.

Ultrafast spin dynamics in ferrimagnets with compensation point.

We derive an effective Lagrangian that facilitates the modeling of magnetization dynamics in a ferrimagnet with magnetization compensation point. The model is able to explain the earlier reported magnetization dynamics in the noncollinear magnetic phase triggered by a femtosecond laser pulse in GdFeCo amorphous alloy in the vicinity of spin-flop transition. Moreover, the described approach can be easily extended and applied to other cases of ultrafast magnetism in uniaxial f -d (rare-earth-transition metal) ferrimagnet near the magnetization compensation point in high magnetic fields. We assume that the primary effect of the femtosecond laser pulse is the ultrafast demagnetization of the ferrimagnet. We show that in the noncollinear magnetic phase, which can be prepared by applying external magnetic field above the spin-flop transition, such a demagnetization results in a torque acting on the magnetizations of both sublattices. It is shown that, similarly to the experiment, the amplitude and timescales of the dynamics strongly depend on temperature and applied magnetic field. In particular, in the vicinity of the spin-flop phase transition the amplitude dramatically increases while the dynamics exhibit a critical slowdown. We expect that the developed theoretical framework will boost further research of ultrafast magnetism of noncollinear spin systems.

Advanced graphene recording device for spin-orbit torque magnetoresistive random access memory.

The non-volatile spin-orbit torque magnetic random access memory (SOT-MRAM) is a very attractive memory technology for near future computers because it has various advantages such as non-volatility, high density and scalability. In the present work we propose a model of a graphene recording device for the SOT-MRAM unit cell, consisting of a quasi-freestanding graphene intercalated with Au and an ultra-thin Pt layer sandwiched between graphene and a magnetic tunnel junction. As a result of using the claimed graphene recording memory element, a faster operation and lower energy consumption will be achieved under the recording information by reducing the electric current required to record. The efficiency of the graphene recording element was confirmed by the experimental results and the theoretical estimations.

Anomalously Damped Heat-Assisted Route for Precessional Magnetization Reversal in an Iron Garnet.

A heat-assisted route for subnanosecond magnetic recording is discovered for the dielectric bismuth-substituted yttrium iron garnet, known for possessing small magnetic damping. The experiments and simulations reveal that the route involves nonlinear magnetization precession, triggered by a transient thermal modification of the growth-induced crystalline anisotropy in the presence of a fixed perpendicular magnetic field. The pathway is rendered robust by the damping becoming anomalously large during the switching process. Subnanosecond deterministic magnetization reversal was achieved within just one-half of a precessional period, and this mechanism should be possible to implement in any material with suitably engineered dissimilar thermal derivatives of magnetization and anisotropy.

Selection rules for all-optical magnetic recording in iron garnet.

Rapid growth of the area of ultrafast magnetism has allowed to achieve a substantial progress in all-optical magnetic recording with femtosecond laser pulses and triggered intense discussions about microscopic mechanisms responsible for this phenomenon. The typically used metallic medium nevertheless considerably limits the applications because of the unavoidable heat dissipation. In contrast, the recently demonstrated photo-magnetic recording in transparent dielectric garnet for all practical purposes is dissipation-free. This discovery raised question about selection rules, i.e. the optimal wavelength and the polarization of light, for such a recording. Here we report the computationally and experimentally identified workspace of parameters allowing photo-magnetic recording in Co-doped iron garnet using femtosecond laser pulses. The revealed selection rules indicate that the excitations responsible for the coupling of light to spins are d-d electron transitions in octahedral and tetrahedral Co-sublattices, respectively.

Dirac cone intensity asymmetry and surface magnetic field in V-doped and pristine topological insulators generated by synchrotron and laser radiation.

Effect of magnetization generated by synchrotron or laser radiation in magnetically-doped and pristine topological insulators (TIs) is presented and analyzed using angle-resolved photoemission spectroscopy. It was found that non-equal photoexcitation of the Dirac cone (DC) states with opposite momenta and spin orientation indicated by the asymmetry in photoemission intensity of the DC states is accompanied by the k||-shift of the DC states relative to the non-spin-polarized conduction band states located at k|| = 0. We relate the observed k||-shift to the induced surface in-plane magnetic field and corresponding magnetization due to the spin accumulation. The direction of the DC k||-shift and its value are changed with photon energy in correlation with variation of the sign and magnitude of the DC states intensity asymmetry. The theoretical estimations describe well the effect and predict the DC k||-shift values which corroborate the experimental observations. This finding opens new perspectives for effective local magnetization manipulation.

Ferroelectricity of domain walls in rare earth iron garnet films.

In this paper, we report on electric polarization arising in a vicinity of Bloch-like domain walls in rare-earth iron garnet films. The domain walls generate an intrinsic magnetic field that breaks an antiferroelectric structure formed in the garnets due to an exchange interaction between rare earth and iron sublattices. We explore 180° domain walls whose formation is energetically preferable in the films with perpendicular magnetic anisotropy. Magnetic and electric structures of the 180° quasi-Bloch domain walls have been simulated at various relations between system parameters. Singlet, doublet ground states of rare earth ions and strongly anisotropic rare earth Ising ions have been considered. Our results show that electric polarization appears in rare earth garnet films at Bloch domain walls, and the maximum of magnetic inhomogeneity is not always linked to the maximum of electric polarization. A number of factors including the temperature, the state of the rare earth ion and the type of a wall influence magnetically induced electric polarization. We show that the value of polarization can be enhanced by the shrinking of the Bloch domain wall width, decreasing the temperature, and increasing the deviations of magnetization from the Bloch rotation that are regulated by impacts given by magnetic anisotropies of the films.

Large microwave generation from current-driven magnetic vortex oscillators in magnetic tunnel junctions.

Spin-polarized current can excite the magnetization of a ferromagnet through the transfer of spin angular momentum to the local spin system. This pure spin-related transport phenomenon leads to alluring possibilities for the achievement of a nanometer scale, complementary metal oxide semiconductor-compatible, tunable microwave generator that operates at low bias for future wireless communication applications. Microwave emission generated by the persistent motion of magnetic vortices induced by a spin-transfer effect seems to be a unique manner to reach appropriate spectral linewidth. However, in metallic systems, in which such vortex oscillations have been observed, the resulting microwave power is much too small. In this study, we present experimental evidence of spin-transfer-induced vortex precession in MgO-based magnetic tunnel junctions, with an emitted power that is at least one order of magnitude stronger and with similar spectral quality. More importantly and in contrast to other spin-transfer excitations, the thorough comparison between experimental results and analytical predictions provides a clear textbook illustration of the mechanism of spin-transfer-induced vortex precession.

High Domain Wall Velocities due to Spin Currents Perpendicular to the Plane.

We consider long and narrow spin valves composed of a first magnetic layer with a single domain wall (DW), a normal metal spacer, and a second magnetic layer that is a planar or a perpendicular polarizer. For these structures, we study numerically DW dynamics taking into account the spin torques due to the perpendicular spin currents. We obtain high DW velocities: 5 m/s for planar polarizer and 80 m/s for perpendicular polarizer for I=0.01 mA. These values are much larger than those predicted and observed for DW motion due to the in-plane spin currents. The ratio of the magnitudes of the torques, which generate the DW motion in the respective cases, is responsible for these large differences.