Observations of supermicron-sized aerosols originating from biomass burning in southern Central Africa.

During the 3 years of the ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) campaign, the NASA Orion P-3 was equipped with a 2D stereo (2D-S) probe that imaged particles with maximum dimension (D) ranging from 10 < D < 1280 µm. The 2D-S recorded supermicron-sized aerosol particles (SAPs) outside of clouds within biomass burning plumes during flights over the southeastern Atlantic off Africa's coast. Numerous SAPs with 10 < D < 1520 µm were observed in 2017 and 2018 at altitudes between 1230 and 4000 m, 1000 km from the coastline, mostly between 7-11° S. No SAPs were observed in 2016 as flights were conducted further south and further from the coastline. Number concentrations of refractory black carbon (rBC) measured by a single particle soot photometer ranged from 200 to 1200 cm-3 when SAPs were observed. Transmission electron microscopy images of submicron particulates, collected on Holey carbon grid filters, revealed particles with potassium salts, black carbon (BC), and organics. Energy-dispersive X-ray spectroscopy spectra also detected potassium, a tracer for biomass burning. These measurements provided evidence that the submicron particles originated from biomass burning. NOAA Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) 3 d back trajectories show a source in northern Angola for times when large SAPs were observed. Fire Information for Resource Management System (FIRMS) Moderate Resolution Imaging Spectroradiometer (MODIS) 6 active fire maps showed extensive biomass burning at these locations. Given the back trajectories, the high number concentrations of rBC, and the presence of elemental tracers indicative of biomass burning, it is hypothesized that the SAPs imaged by the 2D-S are examples of BC aerosol, ash, or unburned plant material.

Quantifying snowfall from orographic cloud seeding.

Climate change and population growth have increased demand for water in arid regions. For over half a century, cloud seeding has been evaluated as a technology to increase water supply; statistical approaches have compared seeded to nonseeded events through precipitation gauge analyses. Here, a physically based approach to quantify snowfall from cloud seeding in mountain cloud systems is presented. Areas of precipitation unambiguously attributed to cloud seeding are isolated from natural precipitation (<1 mm h-1). Spatial and temporal evolution of precipitation generated by cloud seeding is then quantified using radar observations and snow gauge measurements. This study uses the approach of combining radar technology and precipitation gauge measurements to quantify the spatial and temporal evolution of snowfall generated from glaciogenic cloud seeding of winter mountain cloud systems and its spatial and temporal evolution. The results represent a critical step toward quantifying cloud seeding impact. For the cases presented, precipitation gauges measured increases between 0.05 and 0.3 mm as precipitation generated by cloud seeding passed over the instruments. The total amount of water generated by cloud seeding ranged from 1.2 × 105 m3 (100 ac ft) for 20 min of cloud seeding, 2.4 × 105 m3 (196 ac ft) for 86 min of seeding to 3.4 x 105 m3 (275 ac ft) for 24 min of cloud seeding.

Precipitation formation from orographic cloud seeding.

Throughout the western United States and other semiarid mountainous regions across the globe, water supplies are fed primarily through the melting of snowpack. Growing populations place higher demands on water, while warmer winters and earlier springs reduce its supply. Water managers are tantalized by the prospect of cloud seeding as a way to increase winter snowfall, thereby shifting the balance between water supply and demand. Little direct scientific evidence exists that confirms even the basic physical hypothesis upon which cloud seeding relies. The intent of glaciogenic seeding of orographic clouds is to introduce aerosol into a cloud to alter the natural development of cloud particles and enhance wintertime precipitation in a targeted region. The hypothesized chain of events begins with the introduction of silver iodide aerosol into cloud regions containing supercooled liquid water, leading to the nucleation of ice crystals, followed by ice particle growth to sizes sufficiently large such that snow falls to the ground. Despite numerous experiments spanning several decades, no direct observations of this process exist. Here, measurements from radars and aircraft-mounted cloud physics probes are presented that together show the initiation, growth, and fallout to the mountain surface of ice crystals resulting from glaciogenic seeding. These data, by themselves, do not address the question of cloud seeding efficacy, but rather form a critical set of observations necessary for such investigations. These observations are unambiguous and provide details of the physical chain of events following the introduction of glaciogenic cloud seeding aerosol into supercooled liquid orographic clouds.