As a fundamental property of light, polarization serves as an excellent information encoding carrier, playing significant roles in many optical applications, including liquid crystal displays, polarization imaging, optical computation and encryption. However, conventional polarization information encoding schemes based on Malus' law usually consider 1D polarization projections on a linear basis, implying that their encoding flexibility is largely limited. Here, we propose a Poincaré sphere (PS) trajectory encoding approach with metasurfaces that leverages a generalized form of Malus' law governing universal 2D projections between arbitrary elliptical polarization pairs spanning the entire PS. Arbitrary polarization encodings are realized by engineering PS trajectories governed by either arbitrary analytic functions or aligned modulation grids of interest, leading to versatile polarization image transformation functionalities, including histogram stretching, thresholding and image encryption within non-orthogonal PS loci. Our work significantly expands the encoding dimensionality of polarization information, unveiling new opportunities for metasurfaces in polarization optics for both quantum and classical regimes.
Diffractive nonlocal metasurfaces have recently opened a broad range of exciting developments in nanophotonics research and applications, leveraging spatially extended-yet locally patterned-resonant modes to control light with new degrees of freedom. While conventional grating responses are elegantly captured by temporal coupled mode theory, current approaches are not well equipped to capture the arbitrary spatial response observed in the nascent field of nonlocal metasurfaces. Here, we introduce spatio-temporal coupled mode theory (STCMT), capable of elegantly capturing the key features of the resonant response of wavefront-shaping nonlocal metasurfaces. This framework can quantitatively guide nonlocal metasurface design while maintaining compatibility with local metasurface frameworks, making it a powerful tool to rationally design and optimize a broad class of ultrathin optical components. We validate this STCMT framework against full-wave simulations of various nonlocal metasurfaces, demonstrating that this tool offers a powerful semi-analytical framework to understand and model the physics and functionality of these devices, without the need for computationally intense full-wave simulations. We also discuss how this model may shed physical insights into nonlocal phenomena in photonics and the functionality of the resulting devices. As a relevant example, we showcase STCMT's flexibility by applying it to study and rapidly prototype nonlocal metasurfaces that spatially shape thermal emission.
The emergence of new technological needs in 5 G/6 G networking and broadband satellite internet access amplifies the demand for innovative wireless communication hardware, including high-performance low-profile transceivers. In this context, antennas based on metasurfaces - artificial surfaces engineered to manipulate electromagnetic waves at will - represent highly promising solutions. In this article, we introduce leaky-wave metasurface antennas operating at micro/millimeter-wave frequencies that are designed using the principles of quasi-bound states in the continuum, exploiting judiciously tailored spatial symmetries that enable fully customized radiation. Specifically, we unveil additional degrees of control over leaky-wave radiation by demonstrating pointwise control of the amplitude, phase and polarization state of the metasurface aperture fields by carefully breaking relevant symmetries with tailored perturbations. We design and experimentally demonstrate metasurface antenna prototypes showcasing a variety of functionalities advancing capabilities in wireless communications, including single-input multi-output and multi-input multi-output near-field focusing, as well as far-field beam shaping.
Optical metasurfaces supporting localized resonances have become a versatile platform for shaping the wavefront of light, but their low quality (Q-) factor modes inevitably modify the wavefront over extended momentum and frequency space, resulting in limited spectral and angular control. In contrast, periodic nonlocal metasurfaces have been providing great flexibility for both spectral and angular selectivity but with limited spatial control. Here, we introduce multiresonant nonlocal metasurfaces capable of shaping the spatial properties of light using several resonances with widely disparate Q-factors. In contrast to previous designs, the narrowband resonant transmission punctuates a broadband resonant reflection window enabled by a highly symmetric array, achieving simultaneous spectral filtering and wavefront shaping in the transmission mode. Through rationally designed perturbations, we realize nonlocal flat lenses suitable as compact band-pass imaging devices, ideally suited for microscopy. We further employ modified topology optimization to demonstrate high-quality-factor metagratings for extreme wavefront transformations with large efficiency.
High quality(Q) factor optical resonators are indispensable for many photonic devices. While very large Q-factors can be obtained theoretically in guided-mode settings, free-space implementations suffer from various limitations on the narrowest linewidth in real experiments. Here, we propose a simple strategy to enable ultrahigh-Q guided-mode resonances by introducing a patterned perturbation layer on top of a multilayer-waveguide system. We demonstrate that the associated Q-factors are inversely proportional to the perturbation squared while the resonant wavelength can be tuned through material or structural parameters. We experimentally demonstrate such high-Q resonances at telecom wavelengths by patterning a low-index layer on top of a 220 nm silicon on insulator substrate. The measurements show Q-factors up to 2.39 × 105, comparable to the largest Q-factor obtained by topological engineering, while the resonant wavelength is tuned by varying the lattice constant of the top perturbation layer. Our results hold great promise for exciting applications like sensors and filters.
Engineering , Photons , Silicon , Vibration
Metasurfaces have been rapidly advancing our command over the many degrees of freedom of light; however, so far, they have been mostly limited to manipulating light in free space. Metasurfaces integrated on top of guided-wave photonic systems have been explored to control the scattering of light off-chip with enhanced functionalities-namely, the point-by-point manipulation of amplitude, phase or polarization. However, these efforts have so far been limited to controlling one or two optical degrees of freedom at best, as well as device configurations much more complex compared with conventional grating couplers. Here we introduce leaky-wave metasurfaces, which are based on symmetry-broken photonic crystal slabs that support quasi-bound states in the continuum. This platform has a compact form factor equivalent to the one of grating couplers, but it provides full command over the amplitude, phase and polarization (four optical degrees of freedom) across large apertures. We present devices for phase and amplitude control at a fixed polarization state, and devices controlling all the four optical degrees of freedom for operation at a wavelength of 1.55 µm. Merging the fields of guided and free-space optics through the hybrid nature of quasi-bound states in the continuum, our leaky-wave metasurfaces may find applications in imaging, communications, augmented reality, quantum optics, LIDAR and integrated photonic systems.
Optics and Photonics , Photons
We explore the use of tailored resonant waveguide gratings (RWG) embedded in a glass-like matrix as angularly tolerant tri-band reflection filters under oblique excitation. Through inverse design we optimize 1D grating structures to support multi-frequency narrowband resonances in an otherwise transparent background, ideally suited for augmented reality applications. In particular, we show theoretically and experimentally that a single RWG can be tailored to provide reflection levels larger than 50% under p-polarized excitation at three distinct wavelengths of choice, over a narrow bandwidth and within a substantial angular range around 58° incidence, while simultaneously eliminating ghost reflections from the glass/air interface. Similar performance can be achieved for s-polarization by cascading two RWG's. Moreover, we demonstrate that these metrics of performance are maintained when the devices are fabricated using roll-to-roll techniques, as required for large-area industrial fabrication. Overall, these devices show exciting potential as large-area transparent heads-up displays, due to their ease of fabrication and material compatibility.
Photonic devices rarely provide both elaborate spatial control and sharp spectral control over an incoming wavefront. In optical metasurfaces, for example, the localized modes of individual meta-units govern the wavefront shape over a broad bandwidth, while nonlocal lattice modes extended over many unit cells support high quality-factor resonances. Here, we experimentally demonstrate nonlocal dielectric metasurfaces in the near-infrared that offer both spatial and spectral control of light, realizing metalenses focusing light exclusively over a narrowband resonance while leaving off-resonant frequencies unaffected. Our devices attain this functionality by supporting a quasi-bound state in the continuum encoded with a spatially varying geometric phase. We leverage this capability to experimentally realize a versatile platform for multispectral wavefront shaping where a stack of metasurfaces, each supporting multiple independently controlled quasi-bound states in the continuum, molds the optical wavefront distinctively at multiple wavelengths and yet stay transparent over the rest of the spectrum. Such a platform is scalable to the visible for applications in augmented reality and transparent displays.
Optical metasurfaces with high quality factors (Q-factors) of chiral resonances can boost substantially light-matter interaction for various applications of chiral response in ultrathin, active, and nonlinear metadevices. However, current approaches lack the flexibility to enhance and tune the chirality and Q-factor simultaneously. Here, we suggest a design of chiral metasurface supporting bound state in the continuum (BIC) and demonstrate experimentally chiroptical responses with ultra-high Q-factors and near-perfect circular dichroism (CD = 0.93) at optical frequencies. We employ the symmetry-reduced meta-atoms with high birefringence supporting winding elliptical eigenstate polarizations with opposite helicity. It provides a convenient way for achieving the maximal planar chirality tuned by either breaking in-plane structure symmetry or changing illumination angle. Beyond linear CD, we also achieved strong near-field enhancement CD and near-unitary nonlinear CD in the same planar chiral metasurface design with circular eigen-polarization. Sharply resonant chirality realized in planar metasurfaces promises various practical applications including chiral lasers and chiral nonlinear filters.
Quasi-bound states in the continuum (QBICs) are Fano resonant states with long optical lifetimes controlled by symmetry-breaking perturbations. While conventional Fano responses are limited to linear polarizations and do not support tailored phase control, here we introduce QBICs born of chiral perturbations that encode arbitrary elliptical polarization states and enable geometric phase engineering. We thereby design metasurfaces with ultrasharp spectral features that shape the impinging wave front with near-unity efficiency. Our findings extend Fano resonances beyond their conventional limits, opening opportunities for nanophotonics, classical and quantum optics, and acoustics.
Diffractive photonic devices manipulate light via local and nonlocal optical modes. Local devices, such as metasurfaces, can shape a wave front at multiple selected wavelengths, but inevitably modify light across the spectrum; nonlocal devices, such as grating filters, offer great frequency selectivity but limited spatial control. Here, we introduce a rational design paradigm using quasibound states in the continuum to realize multifunctional nonlocal devices: metasurfaces that produce narrow band spatially tailored wave fronts at multiple selected wavelengths and yet are otherwise transparent.
Metasurfaces are optically thin metamaterials that promise complete control of the wavefront of light but are primarily used to control only the phase of light. Here, we present an approach, simple in concept and in practice, that uses meta-atoms with a varying degree of form birefringence and rotation angles to create high-efficiency dielectric metasurfaces that control both the optical amplitude and phase at one or two frequencies. This opens up applications in computer-generated holography, allowing faithful reproduction of both the phase and amplitude of a target holographic scene without the iterative algorithms required in phase-only holography. We demonstrate all-dielectric metasurface holograms with independent and complete control of the amplitude and phase at up to two optical frequencies simultaneously to generate two- and three-dimensional holographic objects. We show that phase-amplitude metasurfaces enable a few features not attainable in phase-only holography; these include creating artifact-free two-dimensional holographic images, encoding phase and amplitude profiles separately at the object plane, encoding intensity profiles at the metasurface and object planes separately, and controlling the surface textures of three-dimensional holographic objects.
Metasurfaces offer a unique platform to precisely control optical wavefronts and enable the realization of flat lenses, or metalenses, which have the potential to substantially reduce the size and complexity of imaging systems and to realize new imaging modalities. However, it is a major challenge to create achromatic metalenses that produce a single focal length over a broad wavelength range because of the difficulty in simultaneously engineering phase profiles at distinct wavelengths on a single metasurface. For practical applications, there is a further challenge to create broadband achromatic metalenses that work in the transmission mode for incident light waves with any arbitrary polarization state. We developed a design methodology and created libraries of meta-units-building blocks of metasurfaces-with complex cross-sectional geometries to provide diverse phase dispersions (phase as a function of wavelength), which is crucial for creating broadband achromatic metalenses. We elucidated the fundamental limitations of achromatic metalens performance by deriving mathematical equations that govern the tradeoffs between phase dispersion and achievable lens parameters, including the lens diameter, numerical aperture (NA), and bandwidth of achromatic operation. We experimentally demonstrated several dielectric achromatic metalenses reaching the fundamental limitations. These metalenses work in the transmission mode with polarization-independent focusing efficiencies up to 50% and continuously provide a near-constant focal length over λ = 1200-1650 nm. These unprecedented properties represent a major advance compared to the state of the art and a major step toward practical implementations of metalenses.
Passive daytime radiative cooling (PDRC) involves spontaneously cooling a surface by reflecting sunlight and radiating heat to the cold outer space. Current PDRC designs are promising alternatives to electrical cooling but are either inefficient or have limited applicability. We present a simple, inexpensive, and scalable phase inversion-based method for fabricating hierarchically porous poly(vinylidene fluoride-co-hexafluoropropene) [P(VdF-HFP)HP] coatings with excellent PDRC capability. High, substrate-independent hemispherical solar reflectances (0.96 ± 0.03) and long-wave infrared emittances (0.97 ± 0.02) allow for subambient temperature drops of ~6°C and cooling powers of ~96 watts per square meter (W m-2) under solar intensities of 890 and 750 W m-2, respectively. The performance equals or surpasses those of state-of-the-art PDRC designs, and the technique offers a paint-like simplicity.
Broadband high reflectance in nature is often the result of randomly, three-dimensionally structured materials. This study explores unique optical properties associated with one-dimensional nanostructures discovered in silk cocoon fibers of the comet moth, Argema mittrei. The fibers are populated with a high density of air voids randomly distributed across the fiber cross-section but are invariant along the fiber. These filamentary air voids strongly scatter light in the solar spectrum. A single silk fiber measuring ~50 µm thick can reflect 66% of incoming solar radiation, and this, together with the fibers' high emissivity of 0.88 in the mid-infrared range, allows the cocoon to act as an efficient radiative-cooling device. Drawing inspiration from these natural radiative-cooling fibers, biomimetic nanostructured fibers based on both regenerated silk fibroin and polyvinylidene difluoride are fabricated through wet spinning. Optical characterization shows that these fibers exhibit exceptional optical properties for radiative-cooling applications: nanostructured regenerated silk fibers provide a solar reflectivity of 0.73 and a thermal emissivity of 0.90, and nanostructured polyvinylidene difluoride fibers provide a solar reflectivity of 0.93 and a thermal emissivity of 0.91. The filamentary air voids lead to highly directional scattering, giving the fibers a highly reflective sheen, but more interestingly, they enable guided optical modes to propagate along the fibers through transverse Anderson localization. This discovery opens up the possibility of using wild silkmoth fibers as a biocompatible and bioresorbable material for optical signal and image transport.
A galvanic-displacement-reaction-based, room-temperature "dip-and-dry" technique is demonstrated for fabricating selectively solar-absorbing plasmonic-nanoparticle-coated foils (PNFs). The technique, which allows for facile tuning of the PNFs' spectral reflectance to suit different radiative and thermal environments, yields PNFs which exhibit excellent, wide-angle solar absorptance (0.96 at 15°, to 0.97 at 35°, to 0.79 at 80°), and low hemispherical thermal emittance (0.10) without the aid of antireflection coatings. The thermal emittance is on par with those of notable selective solar absorbers (SSAs) in the literature, while the wide-angle solar absorptance surpasses those of previously reported SSAs with comparable optical selectivities. In addition, the PNFs show promising mechanical and thermal stabilities at temperatures of up to 200 °C. Along with the performance of the PNFs, the simplicity, inexpensiveness, and environmental friendliness of the "dip-and-dry" technique makes it an appealing alternative to current methods for fabricating selective solar absorbers.
Research on two-dimensional designer optical structures, or metasurfaces, has mainly focused on controlling the wavefronts of light propagating in free space. Here, we show that gradient metasurface structures consisting of phased arrays of plasmonic or dielectric nanoantennas can be used to control guided waves via strong optical scattering at subwavelength intervals. Based on this design principle, we experimentally demonstrate waveguide mode converters, polarization rotators and waveguide devices supporting asymmetric optical power transmission. We also demonstrate all-dielectric on-chip polarization rotators based on phased arrays of Mie resonators with negligible insertion losses. Our gradient metasurfaces can enable small-footprint, broadband and low-loss photonic integrated devices.
