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1.
Nat Commun ; 12(1): 6027, 2021 Oct 15.
Article in English | MEDLINE | ID: mdl-34654828

ABSTRACT

The paradigm of Landau's Fermi liquid theory has been challenged with the finding of a strongly interacting Fermi liquid that cannot be adiabatically connected to a non-interacting system. A spin-1 two-channel Kondo impurity with anisotropy D has a quantum phase transition between two topologically different Fermi liquids with a peak (dip) in the Fermi level for D < Dc (D > Dc). Extending this theory to general multi-orbital problems with finite magnetic field, we reinterpret in a unified and consistent fashion several experimental studies of iron phthalocyanine molecules on Au(111) that were previously described in disconnected and conflicting ways. The differential conductance shows a zero-bias dip that widens when the molecule is lifted from the surface (reducing the Kondo couplings) and is transformed continuously into a peak under an applied magnetic field. We reproduce all features and propose an experiment to induce the topological transition.

2.
Phys Rev Lett ; 123(3): 036601, 2019 Jul 19.
Article in English | MEDLINE | ID: mdl-31386456

ABSTRACT

Recent experiments on cold atoms in optical lattices allow for a quantitative comparison of the measurements to the conductivity calculations in the square lattice Hubbard model. However, the available calculations do not give consistent results, and the question of the exact solution for the conductivity in the Hubbard model remained open. In this Letter, we employ several complementary state-of-the-art numerical methods to disentangle various contributions to conductivity and identify the best available result to be compared to experiment. We find that, at relevant (high) temperatures, the self-energy is practically local, yet the vertex corrections remain rather important, contrary to expectations. The finite-size effects are small even at the lattice size 4×4, and the corresponding Lanczos diagonalization result is, therefore, close to the exact result in the thermodynamic limit.

3.
Sci Adv ; 5(7): eaav1235, 2019 Jul.
Article in English | MEDLINE | ID: mdl-31281880

ABSTRACT

A semiconductor nanowire with strong spin-orbit coupling in proximity to a superconductor is predicted to display Majorana edge states emerging under a properly oriented magnetic field. The experimental investigation of these exotic states requires assessing the one-dimensional (1D) character of the nanowire and understanding the superconducting proximity effect in the presence of a magnetic field. Here, we explore the quasi-ballistic 1D transport regime of an InAs nanowire with Ta contacts. Fine-tuned by means of local gates, the observed plateaus of approximately quantized conductance hide the presence of a localized electron, giving rise to a lurking Coulomb blockade effect and Kondo physics. When Ta becomes superconducting, this local charge causes an unusual, reentrant magnetic field dependence of the supercurrent, which we ascribe to a 0 - π transition. Our results underline the relevant role of unintentional charge localization in the few-channel regime where helical subbands and Majorana quasi-particles are expected to arise.

4.
Nat Commun ; 9(1): 2376, 2018 06 18.
Article in English | MEDLINE | ID: mdl-29915280

ABSTRACT

A magnetic impurity coupled to a superconductor gives rise to a Yu-Shiba-Rusinov (YSR) state inside the superconducting energy gap. With increasing exchange coupling the excitation energy of this state eventually crosses zero and the system switches to a YSR ground state with bound quasiparticles screening the impurity spin by h/2. Here we explore indium arsenide (InAs) nanowire double quantum dots tunnel coupled to a superconductor and demonstrate YSR screening of spin-1/2 and spin-1 states. Gating the double dot through nine different charge states, we show that the honeycomb pattern of zero-bias conductance peaks, archetypal of double dots coupled to normal leads, is replaced by lines of zero-energy YSR states. These enclose regions of YSR-screened dot spins displaying distinctive spectral features, and their characteristic shape and topology change markedly with tunnel coupling strengths. We find excellent agreement with a simple zero-bandwidth approximation, and with numerical renormalization group calculations for the two-orbital Anderson model.

5.
Phys Rev Lett ; 121(25): 257701, 2018 Dec 21.
Article in English | MEDLINE | ID: mdl-30608792

ABSTRACT

We demonstrate the Josephson effect in a serial double quantum dot defined in a nanowire with epitaxial superconducting leads. The supercurrent stability diagram adopts a honeycomb pattern. We observe sharp discontinuities in the magnitude of the critical current, I_{c}, as a function of dot occupation, related to doublet to singlet ground state transitions. Detuning of the energy levels offers a tuning knob for I_{c}, which attains a maximum at zero detuning. The consistency between experiment and theory indicates that our device is a faithful realization of the two-impurity Anderson model.

6.
Phys Rev Lett ; 119(13): 137205, 2017 Sep 29.
Article in English | MEDLINE | ID: mdl-29341713

ABSTRACT

The ground state of the quantum kagome antiferromagnet Zn-brochantite, ZnCu_{3}(OH)_{6}SO_{4}, which is one of only a few known spin-liquid (SL) realizations in two or three dimensions, has been described as a gapless SL with a spinon Fermi surface. Employing nuclear magnetic resonance in a broad magnetic-field range down to millikelvin temperatures, we show that in applied magnetic fields this enigmatic state is intrinsically unstable against a SL with a full or a partial gap. A similar instability of the gapless Fermi-surface SL was previously encountered in an organic triangular-lattice antiferromagnet, suggesting a common destabilization mechanism that most likely arises from spinon pairing. A salient property of this instability is that an infinitesimal field suffices to induce it, as predicted theoretically for some other types of gapless SLs.

7.
J Phys Condens Matter ; 23(9): 094212, 2011 Mar 09.
Article in English | MEDLINE | ID: mdl-21339565

ABSTRACT

We study the zero-temperature properties of the Kondo lattice model within the dynamical mean-field theory. As an impurity solver we use the numerical renormalization group. We present results for the paramagnetic case showing the anticipated heavy-fermion physics, including direct evidence for the appearance of a large Fermi surface for antiferromagnetic exchange interaction. Allowing for the formation of a Néel state, we observe at finite doping an antiferromagnetic metal below a critical exchange interaction, which shows a crossover from a local moment antiferromagnet with a small Fermi surface for weak exchange coupling to a heavy-fermion antiferromagnet with a large Fermi surface for increasing exchange. Including lattice degrees of freedom via an additional Holstein term we observe a significant suppression of the Kondo effect, leading to a strongly reduced low-energy scale. For too large electron-phonon coupling we find a complete collapse of the heavy Fermi liquid and the formation of polarons.

8.
J Phys Condens Matter ; 22(2): 026002, 2010 Jan 20.
Article in English | MEDLINE | ID: mdl-21386266

ABSTRACT

We study the system of two magnetic impurities described by a two-impurity Kondo model where only the first impurity couples directly to the conduction band, while the second impurity interacts with the first through Heisenberg exchange coupling in a 'side-coupled' configuration. We consider various choices of the impurity spins (S(1)S(2)) and we contrast the regimes where the inter-impurity exchange coupling J is either lower or higher than the Kondo temperature T(K)((0)) of the first impurity in the absence of the second. This model is a high-spin generalization of the two-impurity model for side-coupled double quantum dots which corresponds to the simplest S(1)=S(2)=1/2 case, where the moments are Kondo-screened successively in two stages for JS(2), there is no second stage of screening for JT(K)((0)) the Kondo screening of the effective spin S(1)-S(2) is found.

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