Up-converted photorefractive optical transient detection with femtosecond laser pulses.

We report on experimental demonstration of optical transient detection (OTD) based on photorefractive two-wave mixing of femtosecond pulses. The demonstrated technique also combines nonlinear-crystal-based OTD with up-conversion from infrared into the visible range. The approach enables measurement of phase changes of a dynamic signal in the infrared using GaP- or Si-based detectors while suppressing stationary background. Experimental results reveal existence of the relation between input phases in the infrared and output phases in the visible wavelength range. We further present experimental evidence of additional merits of up-converted transient phase analysis under noisy conditions, such as residual continuous-wave emission affecting the ultrashort pulses from the laser.

Yb-fiber-pumped high-average-power picosecond optical parametric oscillator tunable across 1.3-1.5†µm.

We report the generation of high-repetition-rate picosecond pulses in the 1.3-1.5 µm spectral range by internal second harmonic generation (SHG) of an idler-resonant optical parametric oscillator (OPO) based on MgO-doped periodically-poled LiNbO3 (MgO:PPLN), synchronously pumped by ∼20 ps pulses at 80 MHz using an Yb-fiber laser at 1.064 µm. By taking advantage of the high spatial quality of the resonant idler beam in the 2503-3030 nm wavelength range and using a second MgO:PPLN crystal with fanout grating structure for intracavity SHG, we have achieved spectral coverage across 1272-1515 nm with up to 1.23 W average power. The second harmonic output exhibits a power stability of 3% rms over 1 hour in pulses of 8.3 ps with Gaussian beam profile. The described approach overcomes the spectral limitation of 1.064 µm-pumped OPOs based on MgO:PPLN and other oxide-based nonlinear crystals, where signal generation below ∼1.45 µm is precluded by multi-phonon absorption of idler radiation above ∼4 µm.

Tunable, high-power, high-order optical vortex beam generation in the mid-infrared.

We report the generation of tunable high-order optical vortices in the mid-infrared (mid-IR) using a picosecond optical parametric oscillator (OPO). The OPO is based on MgO:PPLN as the nonlinear gain medium and synchronously pumped by a mode-locked Yb-fiber laser at 1064 nm. Using a singly-resonant oscillator configuration for the OPO, we have achieved direct transfer of pump optical vortices to the non-resonant idler beam, with the resonant signal in the Gaussian cavity mode. We demonstrate the successful transfer of pump optical vortices of order, lp = 1 to 5, to the idler beam of the same order across the mid-IR, with an output power of 630 mW to 130 mW across 2538 nm to 4035 nm for the highest idler vortex order, li = 5. To the best of our knowledge, this is the first report of an OPO pumped by a vortex beam of order as high as lp = 5 and generating idler vortices of high order in the mid-IR.

Broadly tunable, intracavity injection-seeded, hybrid optical parametric oscillator.

We report a novel, to the best of our knowledge, approach for injection seeding of pulsed optical parametric oscillators (OPOs), which can provide spectral control over the full tuning range. Bandwidth reduction down to single-mode operation is realized across the pulsed tuning range by deploying a hybrid design, where a continuous-wave (cw) OPO injection seeds the pulsed OPO in a single composite cavity. By exploiting two identical MgO-doped periodically poled lithium niobate crystals, the hybrid OPO provides signal pulses with a single-frequency linewidth as narrow as 7.2 MHz across 1510-1677 nm. The effect of cw injection seeding on pulsed OPO operation is also confirmed by reduced rise time, increased pump depletion, major reduction in threshold, and substantial enhancement in output power and extraction efficiency.

Green-pumped continuous-wave parametric oscillator based on fanout-grating MgO:PPLN: publisher's note.

This publisher's note contains corrections to Opt. Lett.45, 6486 (2020)OPLEDP0146-959210.1364/OL.404979.

Performance studies of high-average-power picosecond optical parametric generation and amplification in MgO:PPLN at 80†MHz.

We report on performance studies of high-average-power single-pass picosecond optical parametric generation (OPG) and amplification (OPA) tunable near 2 µm in MgO:PPLN pumped by an Yb-fiber laser at 1.064 µm and 80 MHz pulse repetition rate. The simple setup based on two identical crystals, and without the need for an intermediate delay line for synchronization, delivers up to 6.3 W of average power at an overall conversion efficiency of ∼50% and is tunable across 1902-2415 nm. We present systematic characterization of OPG and OPA stages to compare their performance and investigate the effect of parametric generation in the high-gain limit, enabling high output power and full-width-half-maximum (FWHM) spectral bandwidths as large as 189 nm. The OPG-OPA output exhibits excellent passive power stability better than 0.3% rms and central wavelength stability better than 0.03% rms over 1 hour, in high spatial beam quality with M2<2. The OPG output pulses have duration of 5.2 ps with a FWHM spectral bandwidth of 117 nm at 2123 nm, resulting in a time-bandwidth product of ΔτΔν∼40, indicating ∼4 times temporal compression compared to the input pump pulses. Theoretical simulations confirm the effect of pump beam divergence on the observed shift in wavelength tuning with respect to temperature, while the exponential gain in the parametric process is identified as playing a key role in the resulting pulse compression.

Fiber-laser-pumped high-repetition-rate picosecond optical parametric generation and amplification in MgO:PPLN.

We report the generation of tunable high-repetition-rate picosecond pulses in the near-infrared at high average power with record conversion efficiency using single-pass optical parametric generation (OPG) and amplification (OPA) in MgO:PPLN, for the first time, to the best of our knowledge. By deploying a mode-locked Yb-fiber laser at 1064 nm providing 21 ps pump pulses at 80 MHz, and a cascade of two 50-mm-long MgO:PPLN crystals, we generate up to 8.3 W of total average output power at a conversion efficiency of 59% over a tunable range of 513 nm, across 1902-2415 nm, with a record threshold as low as 600 mW (7.5 nJ). The two-stage OPG-OPA scheme provides control over fine wavelength tuning and output spectral bandwidths, enabled by the independent control of phase-matching in each crystal. The OPG-OPA output exhibits high spatial beam quality and excellent passive power and central wavelength stability better than 0.9% rms and 0.1% rms, respectively, over 1 hour. The output pulses have a duration of ∼11ps, with a 10 dB bandwidth of ∼350nm at 2107 nm.

Phase-locked picosecond optical parametric oscillator.

We report a degenerate self-phase-locked picosecond optical parametric oscillator (OPO) synchronously pumped by a mode-locked Yb-fiber laser at 1064 nm, delivering broadband output near 2 µm with 2.8 W of average power at ∼80MHz repetition rate. By exploiting a 50-mm-long MgO:PPLN crystal providing high gain and low group velocity dispersion under type-0 (e→ee) phase matching, the OPO generates a phase-locked degenerate output spectrum with a bandwidth of ∼202nm centered at 2128 nm in pulses of ∼21ps duration with excellent passive long-term power and spectral stability in high spatial beam quality. Phase-locked operation results in spectral and power stabilization at exact degeneracy and is further validated by f-2f interferometry and radio frequency measurements of OPO output. To the best of our knowledge, this is the first degenerate self-phase-locked OPO in picosecond time scale, and the highest average power reported for a phase-locked ultrafast OPO to date.

Green-pumped optical parametric oscillator based on fan-out grating periodically-poled MgO-doped congruent LiTaO3.

We report a green-pumped optical parametric oscillator (OPO) based on periodically poled MgO-doped congruent lithium tantalate (MgO:cPPLT). Pumped at 532 nm by a frequency-doubled Q-switched Nd:YAG laser, and using a fan-out grating structure, the singly-resonant OPO provides continuous tuning across 689-1025 nm in the signal and 1106-2336 nm in the idler at room temperature by simple mechanical translation of the crystal. The tuning range can be further extended to 677 nm and 2479 nm in the signal and idler, respectively, by temperature tuning the crystal to 200°C. With a 29-mm-long crystal, the OPO generates 131 mW of average idler power at 1476.5 nm for an input pump power of 1.8 W at 25 kHz repetition rate, with a slope efficiency of 11.3%. Bulk damage in the MgO:cPPLT crystal has been observed for pump powers above ∼1.8 W, and at pump powers beyond ∼1.4 W under long-term operation. The passive power stability of the generated idler is 3.9% over 30 min, in a Gaussian spatial profile.

Tunable ultraviolet vortex source based on a continuous-wave optical parametric oscillator.

We report a continuous-wave (cw) optical parametric oscillator (OPO) generating optical vortices tunable in the ultraviolet (UV). Based on MgO:sPPLT as the nonlinear crystal, the singly resonant OPO is pumped by a cw vortex beam in the green, and deploying intracavity sum-frequency generation (SFG) between the undepleted pump and the Gaussian resonant signal in the crystal of BiB3O6, it can generate optical vortices of order, luv=1 and 2, tunable across 332-344 nm in the UV with a maximum power of 12 mW. Due to conservation of orbital angular momentum in the parametric process, the OPO also produces a non-resonant idler output beam in a vortex spatial profile of order li=1 and 2, identical to the pump vortex, with the signal beam in Gaussian distribution. The idler vortex is tunable across 1172-1338 nm with maximum output power of 1.3 W.

Femtosecond optical parametric oscillator continuously tunable across 3.6-8 µm based on orientation-patterned gallium phosphide.

We report a synchronously-pumped femtosecond optical parametric oscillator (OPO) based on orientation-patterned gallium phosphide (OP-GaP), providing continuously tunable mid-infrared (mid-IR) idler radiation across 3570-7892 nm (2801-1267 cm-1), by exploiting pump wavelength tuning. We generate up to 54 mW of output average power at 80 MHz, and quantum conversion efficiencies up to 28.9% are achieved by use of synchronized pump retroreflection. With the inclusion of intracavity dispersion compensation in an OP-GaP OPO, near-transform-limited signal pulse durations of 112 fs at 1288 nm are measured, and peak powers up to 3 kW in the mid-IR are inferred. Finally, evidence of three-photon absorption is observed and characterized near the pump wavelength.

Orbital angular momentum exchange in a picosecond optical parametric oscillator.

We report on the orbital angular momentum (OAM) exchange among the interacting beams in an ultrafast optical parametric oscillator (OPO). The singly-resonant OPO is synchronously pumped by a picosecond vortex beam from a frequency-doubled Yb-fiber laser at 532 nm in the green. We demonstrate successful transfer of the pump OAM mode to the non-resonant idler beam tunable across 1109-1209 nm, with OAM as high as lp=3. Controlling the cavity loss and spatial overlap between the resonant signal and the pump beam in the nonlinear crystal, we have generated signal and idler OAM mode combinations, (ls,li) of (0,2) and (1,1), and (0,3) and (1,2) for pump OAM mode lp=2 and 3, respectively. Using a pump power of 1 W, we have generated idler OAM mode of orders, li=1, 2, and 3, with maximum output powers of 202, 113, and 57 mW, respectively. To the best of our knowledge, this is the first report on controlled generation of OAM modes from an ultrafast OPO.

High-repetition-rate, deep-infrared, picosecond optical parametric oscillator based on CdSiP2.

We report a high-repetition-rate picosecond optical parametric oscillator (OPO) based on CdSiP2 (CSP) that is synchronously pumped by an Yb-fiber laser at 1064 nm and provides high average power in the deep-infrared (deep-IR) at 79.5 MHz. The OPO is tunable across 6205-6710 nm in the idler, providing as much as 105 mW of average power at 6205 nm and >55 mW over nearly the entire tuning range. The deep-IR idler output exhibits passive power stability better than 2.3% rms over 12 h in good beam quality. The near-IR signal pulses from the OPO have a Gaussian pulse duration of ∼19 ps, measured at 1284 nm. We have investigated the temperature tuning characteristics of the OPO and compared the data with the theoretical calculations using the most recent Sellmeier equations and thermo-optic coefficients for the crystal. To the best of our knowledge, this is the first picosecond OPO based on CSP operating at MHz repetition rates.

Optical parametric generation in orientation-patterned gallium phosphide.

We report an optical parametric generator (OPG) based on the new nonlinear material, orientation-patterned gallium phosphide (OP-GaP). Pumped by a Q-switched nanosecond Nd:YAG laser at 1064 nm with 25 kHz pulse repetition rate, the OPG can be tuned across 1721-1850 nm in the signal and 2504-2787 nm in the idler. Using a 40-mm-long crystal in single-pass configuration, we have generated a total average output power of up to ∼18 mW, with ∼5 mW of idler power at 2670 nm, for 2 W of input pump power. The OPG exhibits a passive stability in total output power better than 0.87% rms over 1 h, at a crystal temperature of 120°C, compared to 0.14% rms for the input pump. The output signal pulses, recorded at 1769 nm, have duration of 5.9 ns for input pump pulses of 9 ns. Temperature-dependent loss measurements for the pump polarization along the [100] axis in the OP-GaP crystal have also been performed, for the first time, indicating a drop in transmission from 28.8% at 50°C to 19.4% at 160°C.

Nanosecond difference-frequency generation in orientation-patterned gallium phosphide.

We report a tunable, single-pass, pulsed nanosecond difference-frequency generation (DFG) source based on the new semiconductor nonlinear material, orientation-patterned gallium phosphide (OP-GaP). The DFG source is realized by mixing the output signal of a nanosecond OPO tunable over 1723-1827 nm with the input pump pulses of the same OPO at 1064 nm in an OP-GaP crystal, resulting in tunable generation over 233 nm in the mid-infrared from 2548 to 2781 nm. Using a 40-mm-long crystal, we have produced ∼14 mW of average DFG output power at 2719 nm for a pump power of 5 W and signal power of 1 W at 80 kHz repetition rate. To the best of our knowledge, this is the first single-pass nanosecond DFG source based on OP-GaP. The DFG output beam has a TEM00 spatial mode profile and exhibits passive power stability better than 1.7% rms over 1.4 h at 2774 nm, compared to 1.6% and 0.1% rms for the signal and pump, respectively. The OP-GaP crystal is recorded to have a temperature acceptance bandwidth of 17.7°C.

Fiber-laser-based, high-repetition-rate, picosecond ultraviolet source tunable across 329-348 nm.

We report a compact, fiber-laser-based, high-repetition-rate picosecond source for the ultraviolet (UV), providing multi-tens of milliwatt of average power across 329-348 nm. The source is based on internal sum-frequency-generation (SFG) in a singly resonant optical parametric oscillator (OPO), synchronously pumped at 532 nm by the second harmonic of a picosecond Yb-fiber laser at 80 MHz repetition rate. Using a 30-mm-long single-grating MgO:sPPLT crystal for the OPO and a 5-mm-long BiB3O6 crystal for intracavity SFG, we generate up to 115 mW of average UV power at 339.9 nm, with >50 mW over 73% of the tuning range, for 1.6 W of input pump power. The UV output exhibits a passive rms power stability of ∼2.9% rms over 1 min and 6.5% rms over 2 h in high beam quality. Angular acceptance bandwidth and cavity detuning effects have also been studied.

Pump-tuned deep-infrared femtosecond optical parametric oscillator across 6-7 µm based on CdSiP2.

We report on a high-power femtosecond optical parametric oscillator (OPO) at 80 MHz repetition rate, tunable across 6318-7061 nm in the deep-infrared (deep-IR) using pump wavelength tuning. The OPO, based on CdSiP2 (CSP), is synchronously pumped by a commercial Ti:sapphire-pumped femtosecond OPO in the near-IR, enabling rapid static tuning of the CSP OPO with minimal adjustments to its cavity length. The deep-IR CSP OPO provides as much as 32 mW of average idler power at 6808 nm with spectral bandwidth >1000 nm (at -10 dB level) across the tuning range. By implementing intracavity dispersion control, near-transform-limited signal pulses of ∼100 fs duration with smooth single-peak spectrum are achieved at 1264 nm, corresponding to an idler wavelength at 6440 nm. To the best of our knowledge, this is the first time such practical idler powers in the deep-IR have been generated from a dispersion-compensated CSP femtosecond OPO at sub-100 MHz repetition rate.

Ultrafast optical vortex beam generation in the ultraviolet.

We report on the generation of ultrafast vortex beams in the deep ultraviolet (DUV) wavelength range at 266 nm, for the first time to our knowledge. Using a Yb-fiber-based green source in combination with two spiral phase plates of orders 1 and 2, we were able to generate picosecond Laguerre-Gaussian (LG) beams at 532 nm. Subsequently, these LG beams were frequency doubled by single-pass, second-harmonic generation in a 10 mm-long ß-BaB2O4 crystal to generate ultrafast vortex beams at 266 nm with a vortex order as high as 12, providing up to 383 mW of DUV power at a single-pass, green-to-DUV conversion efficiency of 5.2%. The generated picosecond UV vortex beam has a spectral width of 1.02 nm with a passive power stability better than 1.2% rms over >1.5 h.

Ti:sapphire-pumped deep-infrared femtosecond optical parametric oscillator based on CdSiP2.

We report on a femtosecond optical parametric oscillator (OPO) for the deep-infrared (deep-IR) based on the Kerr-lens-mode-locked Ti:sapphire laser as the pump source. By deploying a novel cascaded intracavity arrangement, comprising a femtosecond OPO based on the nonlinear crystal, CdSiP2, synchronously pumped internal to a MgO:PPLN femtosecond OPO, we have generated broadly tunable radiation across 5958-8117 nm using rapid static cavity delay tuning, with a maximum power of 64 µW at 6791 nm, limited by the absorption in mirror substrates as well as polarization-dependent intracavity losses. The deep-IR idler power exhibits excellent passive stability of better than 1.1% rms over 2 h, with a spectral bandwidth as large as ∼650 nm at ∼6800 nm. The demonstrated concept is generic and can be similarly deployed in other operating time scales and wavelength regions, also using different laser pump sources and nonlinear materials.

Fiber-laser-based, green-pumped, picosecond optical parametric oscillator using fan-out grating PPKTP.

We report a stable, Yb-fiber-laser-based, green-pumped, picosecond optical parametric oscillator (OPO) for the near-infrared based on periodically poled potassium titanyl phosphate (PPKTP) nonlinear crystal, using fan-out grating design and operating near room temperature. The OPO is continuously tunable across 726-955 nm in the signal and 1201-1998 nm in the idler, resulting in a total signal plus idler wavelength coverage of 1026 nm by grating tuning at a fixed temperature. The device generates up to 580 mW of average power in the signal at 765 nm and 300 mW in the idler at 1338 nm, with an overall extraction efficiency of up to 52% and a pump depletion >76%. The extracted signal at 765 nm and idler at 1746 nm exhibit excellent passive power stability better than 0.5% and 0.8% rms, respectively, over 1 h with good beam quality in TEM00 mode profile. The output signal pulses have a Gaussian temporal duration of 13.2 ps, with a FWHM spectral bandwidth of 3.4 nm at 79.5 MHz repetition rate. Power scaling limitations of the OPO due to the material properties of PPKTP are studied.