Highly birefringent vaterite microspheres: production, characterization and applications for optical micromanipulation.

This paper reports on a simple synthesis and characterization of highly birefringent vaterite microspheres, which are composed of 20-30 nm sized nanocrystalls. Scanning electron microscopy shows a quite disordered assembly of nanocrystals within the microspheres. However, using optical tweezers, the effective birefringence of the microspheres was measured to be Deltan = 0.06, which compares to Deltan = 0.1 of vaterite single crystals. This suggests a very high orientation of the nanocrystals within the microspheres. A hyperbolic model of the direction of the optical axis throughout the vaterite spherulite best fits the experimental data. Results from polarized light microscopy further confirm the hyperbolic model.

Constant power optical tweezers with controllable torque.

We describe a means for controlling the spin angular-momentum flux of a laser beam at constant power, without introducing any elliptical or linear polarization. This allows a controllable torque, acting to spin the particle uniformly, to be exerted on a birefringent particle in optical tweezers. The constant power means that transverse and axial trapping, and heating due to absorption, are unaffected by changing the torque. The torque can be computer controlled and rapidly changed. In addition, the lateral trapping is kept constant. Very low torques can be obtained such that rotational Brownian motion of birefringent particles can be observed. This has the potential to greatly extend the quantitative applications of the rotation of birefringent objects in optical tweezers.