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Sci Total Environ ; 626: 887-898, 2018 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-29898557


Despite the implementation of strict air pollution control measures in recent years, severe haze events were still encountered in the Beijing-Tianjin-Hebei (Jing-Jin-Ji) region during the winter 2016. In this work, seasonal differences in correlations between air pollution and geographic terrain, atmospheric dynamical and thermal structures, and PBL height over the Jing-Jin-Ji region in history and recent years were investigated and a comprehensive model of atmospheric factors affecting winter air pollution formation was proposed. We found that the distribution of PM2.5 concentration closely correlated with the topography feature of China and the difference in haze pollution intensity between winter and other seasons was the most significant in the Jing-Jin-Ji region. The "semi-enclosed" terrain along with the enhanced winter "downdraft" strongly inhibited the diffusion and convection of air pollutants in this region. Meanwhile, seasonal variations of the vertical thermal structure over the Jing-Jin-Ji region, i.e., the anomalous pattern of "upper warming and bottom cooling" structure in the middle troposphere, and the "weak wind zone" were more distinct in winter 2016 than historical record, providing an important precondition for the frequent occurrence of thermal inversion layers and severe pollution episodes in the lower troposphere. In addition, abnormally low PBL heights occurred in the Jing-Jin-Ji region during severe pollutant episodes in winter 2016, with mean postmeridian PBL height in December of only 869.4 m, the minimum value since 2013. PM2.5 concentration was not only closely related to PBL height but also the "warm cover" structure in the middle troposphere. The stronger the structure was, the lower the PBL height became, and severer the pollution event was encountered, accompanying water vapor accumulation and intensification of the thermal inversion layer in the lower troposphere. All above observations revealed the mutual feedback correlations between air pollutants concentration and meteorological factors.

Poluentes Atmosféricos/análise , Monitoramento Ambiental , Conceitos Meteorológicos , Material Particulado/análise , Poluição do Ar/estatística & dados numéricos , Pequim , Estações do Ano