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Environ Sci Technol ; 53(24): 14212-14221, 2019 Dec 17.
Artigo em Inglês | MEDLINE | ID: mdl-31722174


The hygroscopic properties of BC-containing particles (BCc) are important to determine their wet scavenging, atmospheric lifetime, and interactions with clouds. Such information is still lacking in the real world because of the challenges in isolating BCc from other aerosols to be directly characterized. In this study, the size-resolved chemical components of BCc including the refractory BC core and associated coatings were measured by a soot particle-aerosol mass spectrometer in suburban Nanjing. The size-resolved hygroscopicity parameter of BCc (κBCc) was obtained based on this full chemical characterization of BCc. We found increased inorganic fraction and more oxidized organic coatings with thicker coatings, which modified κBCc besides the determinant of particle size. The bulk κBCc was observed to range from 0.11 to 0.34. The size-resolved κBCc consistently showed minima at coated diameter (Dcoated) of 100 nm, parametrized as κ(x) = 0.28-0.35 × exp(-0.004 × x), x = Dcoated. Under critical supersaturations (SS) of 0.1% and 0.2%, the D50 values of BCc were 200 ± 20 and 135 ± 18 nm, respectively. On average 33 ± 16% and 59 ± 20% of BCc in number could be activated at SS = 0.1% and 0.2%, respectively. These results provide constraints on surface CCN sources for the light-absorbing BC-containing particles.

Huan Jing Ke Xue ; 37(1): 280-7, 2016 Jan 15.
Artigo em Chinês | MEDLINE | ID: mdl-27078968


Field experiments were conducted in winter wheat-growing season to investigate the effect of reduced water and diurnal warming on wheat biomass and soil respiration. The experimental treatments included the control (CK), 30% reduced water (W), diurnal warming (T, enhanced 2 degrees C), and the combined treatment (TW, 30% reduced water plus diurnal warming 2 degrees C). Soil respiration rate was measured using a static chamber-gas chromatograph technique. The results showed that in the winter wheat-growing season, compared to CK, T and TW treatments significantly increased shoot biomass by 46.0% (P = 0.002) and 19.8% (P = 0.032) during the elongation-booting stage, respectively. T and TW treatments also significantly increased the harvested shoot biomass by 19.8% (P = 0.050) and 34.6% (P = 0.028), respectively. On the other hand, W treatment had no significant effect on shoot biomass, and W, T, and TW treatments didn't significantly change the root biomass. T and W treatments had no significant effect on the mean respiration rate (MRR) of soil (P > 0.05). TW treatment significantly decreased soil MRR by 22.4% (P = 0.049). We also found T treatment decreased the temperature sensitivity coefficients of soil respiration (Q10). The results of our study suggested that compared to the single treatment (reduced water or diurnal warming), the combined treatment (reduced water plus diurnal warming) may have different effects on agroecosystem.

Irrigação Agrícola , Solo/química , Temperatura Ambiente , Triticum/crescimento & desenvolvimento , Biomassa , Dióxido de Carbono , Periodicidade , Raízes de Plantas/crescimento & desenvolvimento , Água
Huan Jing Ke Xue ; 36(2): 636-43, 2015 Feb.
Artigo em Chinês | MEDLINE | ID: mdl-26031093


To investigate the impact of elevated surface ozone (O3) concentration on nitrous oxide (N2O) emission from arid farmland, field experiments were carried out during winter-wheat and soybean growing seasons under the condition of simulating O3 concentrations, including free air (CK), 100 nL x L(-1) O3 concentration (T1), and 150 nL x L(-1) O3 concentration (T2). N2O emission fluxes were measured by static dark chamber-gas chromatograph method. The results showed that the accumulative amount of N2O (AAN) were decreased by 37.8% (P = 0.000 ) and 8.8% (P = 0.903 ) under T1 and T2 treatments, respectively, in the turning-green stage of winter wheat. In the elongation-booting stage, ANN were decreased by 15.0% (P = 0.217) and 39.1% (P = 0.000) under T1 and T2 treatments, respectively. ANN were decreased by 18.9% (P = 0.138) and 25.6% (P = 0.000) under T1 and T2 treatments, respectively, during the whole winter-wheat growing season. No significant impact of elevated O3 concentration on N2O emission from soil-soybean system was found due to the less rainfall during the soybean growing season, drought had a stronger stress on soybean than O3 concentration. The results of this study suggested that elevated O3 concentration could reduce N2O emission from arid farmland.

Poluentes Atmosféricos/análise , Óxido Nitroso/análise , Ozônio/química , Solo/química , Agricultura , Monitoramento Ambiental , Soja , Triticum
Huan Jing Ke Xue ; 35(7): 2771-6, 2014 Jul.
Artigo em Chinês | MEDLINE | ID: mdl-25244867


In order to study the effect of conservation tillage on soil CO2 and N2O emissions in the following crop-growing season, field experiments were conducted in the winter wheat-growing season. Four treatments were conventional tillage (T), no-tillage with no straw cover (NT), no-tillage with straw cover (NTS), and conventional tillage with straw incorporation (TS), respectively. The CO2 and N2O fluxes were measured using a static chamber-gas chromatograph technique. The results showed that in the following winter wheat-growing season, conservation tillage did not change the seasonal pattern of CO2 and N2O emission fluxes from soil, and had no significant effect on crop biomass. Conservation tillage significantly reduced the accumulative amount of CO2 and N2O. Compared with the T treatment, the accumulative amount of CO2 under TS, NT, and NTS treatments were reduced by 5.95% (P = 0.132), 12.94% (P = 0.007), and 13.91% (P = 0.004), respectively, and the accumulative amount of N2O were significantly reduced by 31.23% (P = 0.000), 61.29% (P = 0.000), and 33.08% (P = 0.000), respectively. Our findings suggest that conservation tillage significantly reduced CO2 and N2O emission from soil in the following winter wheat-growing season.

Agricultura/métodos , Dióxido de Carbono/análise , Óxido Nitroso/análise , Solo/química , Estações do Ano , Triticum/crescimento & desenvolvimento