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Advances in the Stability of Catalysts for Electroreduction of CO2 to Formic Acid.
Song, Dewen; Zhang, Shipeng; Zhou, Minjun; Wang, Mingwang; Zhu, Ruirui; Ning, Hui; Wu, Mingbo.
Affiliation
  • Song D; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
  • Zhang S; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
  • Zhou M; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
  • Wang M; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
  • Zhu R; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
  • Ning H; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
  • Wu M; State Key Laboratory of Heavy Oil Processing, College of Chemical Engineering, College of New Energy, Institute of New Energy, China University of Petroleum, East China, Qingdao, 266580.
ChemSusChem ; 17(14): e202301719, 2024 Jul 22.
Article in En | MEDLINE | ID: mdl-38411399
ABSTRACT
The electroreduction of CO2 to high-value products is a promising approach for achieving carbon neutrality. Among these products, formic acid stands out as having the most potential for industrialization due to its optimal economic value in terms of consumption and output. In recent years, the Faraday efficiency of formic acid from CO2 electroreduction has reached 90~100 %. However, this high selectivity cannot be maintained for extended periods under high currents to meet industrial requirements. This paper reviews excellent work from the perspective of catalyst stability, summarizing and discussing the performance of typical catalysts. Strategies for preparing stable and highly active catalysts are also briefly described. This review may offer a useful data reference and valuable guidance for the future design of long-stability catalysts.

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: ChemSusChem / ChemSusChem (Weinh., Internet) / ChemSusChem (Weinheim. Internet) Journal subject: QUIMICA / TOXICOLOGIA Year: 2024 Document type: Article Country of publication:

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: ChemSusChem / ChemSusChem (Weinh., Internet) / ChemSusChem (Weinheim. Internet) Journal subject: QUIMICA / TOXICOLOGIA Year: 2024 Document type: Article Country of publication: