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Laser-induced transient magnons in Sr3Ir2O7 throughout the Brillouin zone.
Mazzone, Daniel G; Meyers, Derek; Cao, Yue; Vale, James G; Dashwood, Cameron D; Shi, Youguo; James, Andrew J A; Robinson, Neil J; Lin, Jiaqi; Thampy, Vivek; Tanaka, Yoshikazu; Johnson, Allan S; Miao, Hu; Wang, Ruitang; Assefa, Tadesse A; Kim, Jungho; Casa, Diego; Mankowsky, Roman; Zhu, Diling; Alonso-Mori, Roberto; Song, Sanghoon; Yavas, Hasan; Katayama, Tetsuo; Yabashi, Makina; Kubota, Yuya; Owada, Shigeki; Liu, Jian; Yang, Junji; Konik, Robert M; Robinson, Ian K; Hill, John P; McMorrow, Desmond F; Först, Michael; Wall, Simon; Liu, Xuerong; Dean, Mark P M.
Affiliation
  • Mazzone DG; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Meyers D; Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232 Villigen, Switzerland.
  • Cao Y; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Vale JG; Department of Physics, Oklahoma State University, Stillwater, OK 74078.
  • Dashwood CD; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Shi Y; Materials Science Division, Argonne National Laboratory, Argonne, IL 60439.
  • James AJA; London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.
  • Robinson NJ; London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.
  • Lin J; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
  • Thampy V; School of Physical Sciences, The Open University, Milton Keynes MK7 6AA, United Kingdom.
  • Tanaka Y; Institute for Theoretical Physics, University of Amsterdam, 1098 XH Amsterdam, The Netherlands.
  • Johnson AS; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Miao H; School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.
  • Wang R; Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.
  • Assefa TA; RIKEN SPring-8 Center, Sayo 679-5148, Japan.
  • Kim J; ICFO - The Institute of Photonics Sciences, The Barcelona Institute of Science and Technology, 08860, Castelldefels, Barcelona, Spain.
  • Casa D; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Mankowsky R; School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.
  • Zhu D; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Alonso-Mori R; Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439.
  • Song S; Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439.
  • Yavas H; Max Planck Institute for the Structure and Dynamics of Matter, D-22761 Hamburg, Germany.
  • Katayama T; Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.
  • Yabashi M; Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.
  • Kubota Y; Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.
  • Owada S; Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.
  • Liu J; RIKEN SPring-8 Center, Sayo 679-5148, Japan.
  • Yang J; RIKEN SPring-8 Center, Sayo 679-5148, Japan.
  • Konik RM; RIKEN SPring-8 Center, Sayo 679-5148, Japan.
  • Robinson IK; RIKEN SPring-8 Center, Sayo 679-5148, Japan.
  • Hill JP; Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996.
  • McMorrow DF; Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996.
  • Först M; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Wall S; Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
  • Liu X; London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.
  • Dean MPM; National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY 11973.
Proc Natl Acad Sci U S A ; 118(22)2021 Jun 01.
Article in En | MEDLINE | ID: mdl-34039712
ABSTRACT
Although ultrafast manipulation of magnetism holds great promise for new physical phenomena and applications, targeting specific states is held back by our limited understanding of how magnetic correlations evolve on ultrafast timescales. Using ultrafast resonant inelastic X-ray scattering we demonstrate that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets and that they persist for several picoseconds, which is opposite to what is observed in nearly gapless magnets. Our work suggests that materials with isotropic magnetic interactions are preferred to achieve rapid manipulation of magnetism.
Key words

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Proc Natl Acad Sci U S A Year: 2021 Document type: Article

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Proc Natl Acad Sci U S A Year: 2021 Document type: Article