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Picosecond Spin Current Generation from Vicinal Metal-Antiferromagnetic Insulator Interfaces.
Yang, B; Ji, Qing; Huang, F Z; Li, Jiacong; Tian, Y Z; Xue, B; Zhu, Ruxian; Wu, Hui; Yang, Hanyue; Yang, Y B; Tang, Shaolong; Zhao, H B; Cao, Y; Du, J; Wang, B G; Zhang, Chunfeng; Wu, D.
Affiliation
  • Yang B; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Ji Q; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Huang FZ; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Li J; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Tian YZ; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Xue B; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Zhu R; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Wu H; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Yang H; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Yang YB; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Tang S; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Zhao HB; Key Laboratory of Micro and Nano Photonic Structures (Ministry of Education), Department of Optical Science and Engineering, Fudan University, Shanghai 200433, People's Republic of China.
  • Cao Y; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Du J; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Wang BG; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Zhang C; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
  • Wu D; National Laboratory of Solid State Microstructures, Jiangsu Provincial Key Laboratory for Nanotechnology, Collaborative Innovation Center of Advanced Microstructures and Department of Physics, Nanjing University, Nanjing 210093, People's Republic of China.
Phys Rev Lett ; 132(17): 176703, 2024 Apr 26.
Article in En | MEDLINE | ID: mdl-38728713
ABSTRACT
We report the picosecond spin current generation from the interface between a heavy metal and a vicinal antiferromagnet insulator Cr_{2}O_{3} by laser pulses at room temperature and zero magnetic field. It is converted into a detectable terahertz emission in the heavy metal via the inverse spin Hall effect. The vicinal interfaces are apparently the source of the picosecond spin current, as evidenced by the proportional terahertz signals to the vicinal angle. We attribute the origin of the spin current to the transient magnetic moment generated by an interfacial nonlinear magnetic-dipole difference-frequency generation. We propose a model based on the in-plane inversion symmetry breaking to quantitatively explain the terahertz intensity with respect to the angles of the laser polarization and the film azimuth. Our work opens new opportunities in antiferromagnetic and ultrafast spintronics by considering symmetry breaking.

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Phys Rev Lett Year: 2024 Document type: Article

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Phys Rev Lett Year: 2024 Document type: Article