Interface Structure Strengthening of a Mesoporous Silicon/Expanded Perlite Microevaporator for Efficient Solar-Driven Interfacial Evaporation.

ABSTRACT

Solar-driven interfacial evaporation is one of the cutting-edge technologies for seawater desalination and wastewater purification. Herein, a floating carbon-coated silica microsphere/expanded perlite integrated interfacial microevaporator (HEPCL) is reported. The carbon nanolayer allows the HEPCL to have better broadband light absorption performance than natural graphite and graphene oxide. Through the low density of expanded perlite, HEPCL particles can self-float on the water surface and self-aggregate into an integrated whole under surface tension, which enhances the heat collection capacity. The hierarchical porous structure of the HEPCL has a continuous water absorption capacity. Notably, water molecules adsorbed in the HEPCL have a high desorption energy, which reduces the water evaporation enthalpy (1621 kJ/kg), making it easy to remove with external energy. Thanks to the design merits, the HEPCL achieves a water evaporation rate of 1.551 kg m-2 h-1 (efficiency of 94.85%) under 1 sun irradiation and may inspire a practicable solution of water scarcity.