High-resolution Doppler-free molecular spectroscopy with a continuous-wave optical parametric oscillator.

ABSTRACT

We present a reliable, narrow-linewidth (100-kHz) continous-wave optical parametric oscillator (OPO) suitable for high-resolution spectroscopy applications. The singly resonant OPO with a resonated pump is based on periodically poled lithium niobate crystal and features a specially designed intracavity etalon, which permits precise tuning to any desired wavelength in a wide range. We demonstrate Doppler-free spectroscopy of a rovibrational transition of methane at 3.39 mum.