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Catalytic enantioselective intermolecular hydroacylation: rhodium-catalyzed combination of beta-S-aldehydes and 1,3-disubstituted allenes.
Osborne, James D; Randell-Sly, Helen E; Currie, Gordon S; Cowley, Andrew R; Willis, Michael C.
Affiliation
  • Osborne JD; Department of Chemistry, University of Oxford, Chemical Research Laboratory, Mansfield Road, Oxford, UK.
J Am Chem Soc ; 130(51): 17232-3, 2008 Dec 24.
Article in En | MEDLINE | ID: mdl-19053453
ABSTRACT
A rhodium(I) catalyst incorporating the Me-DuPhos ligand promotes enantioselective intermolecular hydroacylation between beta-S-aldehydes and 1,3-disubstituted allenes. The nonconjugated enone products are obtained in good yields and with high enantioselectivities.
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Full text: 1 Collection: 01-internacional Database: MEDLINE Main subject: Rhodium / Chemistry / Aldehydes / Alkenes Language: En Journal: J Am Chem Soc Year: 2008 Document type: Article Affiliation country: United kingdom
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Full text: 1 Collection: 01-internacional Database: MEDLINE Main subject: Rhodium / Chemistry / Aldehydes / Alkenes Language: En Journal: J Am Chem Soc Year: 2008 Document type: Article Affiliation country: United kingdom