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On-Surface Synthesis of Novel Kagome Lattices Coordinated via Four-Fold N-Ag Bonding.
Xiong, Juanjuan; Qin, Tianchen; Hu, Lei; Yang, Weishan; Chen, Zijie; Ding, Honghe; Hu, Jun; Xu, Qian; Zhu, Junfa.
Affiliation
  • Xiong J; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Qin T; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Hu L; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Yang W; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Chen Z; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Ding H; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Hu J; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Xu Q; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
  • Zhu J; National Synchrotron Radiation Laboratory, Department of Chemical Physics and Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China.
J Phys Chem Lett ; 14(43): 9787-9792, 2023 Nov 02.
Article in En | MEDLINE | ID: mdl-37883195
The Kagome lattice structures based on metal-organic coordination have garnered widespread interest because of their topologically Dirac/flat bands and other exotic electronic structures. However, the experimental fabrication of large-area two-dimensional (2D) Kagome lattice structures of metal-organic frameworks (MOFs) via on-surface synthesis remains limited. Herein, we successfully construct two kinds of large-scale 2D Kagome-type lattices stabilized by 4-fold N-Ag coordination on the Ag(111) surface. With the aid of scanning tunneling microscopy (STM) and synchrotron radiation photoemission spectroscopy (SRPES), we clearly elucidate the reaction pathway and mechanism of fabrication of the two Kagome lattices. This work provides a novel platform for investigating related intriguing physical properties.
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Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: J Phys Chem Lett Year: 2023 Document type: Article Country of publication: United States
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Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: J Phys Chem Lett Year: 2023 Document type: Article Country of publication: United States