Time-resolved ARPES with probe energy of 6.0/7.2 eV and switchable resolution configuration.
Rev Sci Instrum
; 95(1)2024 Jan 01.
Article
in En
| MEDLINE
| ID: mdl-38165821
ABSTRACT
We present a detailed exposition of the design for time- and angle-resolved photoemission spectroscopy using a UV probe laser source that combines the nonlinear effects of ß-BaB2O4 and KBe2BO3F2 optical crystals. The photon energy of the probe laser can be switched between 6.0 and 7.2 eV, with the flexibility to operate each photon energy setting under two distinct resolution configurations. Under the fully optimized energy resolution configuration, we achieve an energy resolution of 8.5 meV at 6.0 eV and 10 meV at 7.2 eV. Alternatively, switching to the other configuration enhances the temporal resolution, yielding a temporal resolution of 72 fs for 6.0 eV and 185 fs for 7.2 eV. We validated the performance and reliability of our system by applying it to measuring two typical materials the topological insulator MnBi2Te4 and the excitonic insulator candidate Ta2NiSe5.
Full text:
1
Collection:
01-internacional
Database:
MEDLINE
Language:
En
Journal:
Rev Sci Instrum
Year:
2024
Document type:
Article
Affiliation country:
China