Coherent Phonon Assisted Ultrafast Order-Parameter Reversal and Hidden Metallic State in Ta_{2}NiSe_{5}.
Phys Rev Lett
; 131(25): 256503, 2023 Dec 22.
Article
in En
| MEDLINE
| ID: mdl-38181365
ABSTRACT
The nonequilibrium dynamics during photoinduced insulator-to-metal transition (IMT) in the excitonic insulator (EI) candidate Ta_{2}NiSe_{5} have been investigated, which reproduce the timescale and spectral features of the ultrafast switch and reveal intricate many-body interactions involving multidegrees of freedom. The key role of lattice order parameter (OP) reversal, occurring on a timescale comparable to that of purely electronic processes (<100 fs), is identified. This reversal is enabled by the anharmonic interactions between EI-OP-coupled phonons and the conventional coherent phonons, leading to a modified potential energy landscape and a high-frequency mode up-conversion. The phonon excitation depends on the dynamics of photocarriers distributed around the Fermi level, and thus intertwines with the excitonic quenching and the complete gap collapse. These findings provide a comprehensive understanding of exciton-phonon dynamics in correlated quantum materials.
Full text:
1
Collection:
01-internacional
Database:
MEDLINE
Type of study:
Prognostic_studies
Language:
En
Journal:
Phys Rev Lett
Year:
2023
Document type:
Article
Affiliation country:
China