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Controlling the Polarization of Nitrogen Ion Lasing.
Gao, Jingsong; Zhang, Xiang; Wang, Yang; Dong, Jiahao; Lei, Mingwei; Liu, Yi; Wu, Chengyin; Gong, Qihuang; Jiang, Hongbing.
Affiliation
  • Gao J; State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.
  • Zhang X; Shanghai Key Lab of Modern Optical System, University of Shanghai for Science and Technology, Shanghai 200093, China.
  • Wang Y; State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.
  • Dong J; Shanghai Key Lab of Modern Optical System, University of Shanghai for Science and Technology, Shanghai 200093, China.
  • Lei M; State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.
  • Liu Y; Shanghai Key Lab of Modern Optical System, University of Shanghai for Science and Technology, Shanghai 200093, China.
  • Wu C; CAS Center for Excellence in Ultra-intense Laser Science, Shanghai 201800, China.
  • Gong Q; State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.
  • Jiang H; State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.
J Phys Chem Lett ; 15(14): 3805-3811, 2024 Apr 11.
Article in En | MEDLINE | ID: mdl-38557052
ABSTRACT
Air lasing provides a promising technique to remotely produce coherent radiation in the atmosphere and has attracted continuous attention. However, the polarization properties of N2+ lasing with seeding have not been understood since it was discovered 10 years ago, in which the polarization behaviors appear disordered and confusing. Here, we performed an experimental and theoretical investigation of the polarization properties of N2+ lasing and successfully revealed its underlying physical mechanism. We found that the optical gain is anisotropic, owing to the permanent alignment of N2+ induced by the preferential ionization of the pump light. As a result, the polarization of the N2+ lasing tends to align with that of the pump light after amplification, which becomes more pronounced as the amplification factor increases. Based on the permanent alignment of N2+, we built a theoretical model that analytically interpreted and numerically reproduced the experimental observations, which points out the key factors for controlling the polarization of N2+ lasing.

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: J Phys Chem Lett / J. phys. chem. lett / The journal of physical chemistry letters Year: 2024 Document type: Article Affiliation country: China Country of publication: United States

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: J Phys Chem Lett / J. phys. chem. lett / The journal of physical chemistry letters Year: 2024 Document type: Article Affiliation country: China Country of publication: United States