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Engineering the Optical Properties of CsPbBr3 Nanoplatelets through Cd2+ Doping.
Skurlov, Ivan D; Sokolova, Anastasiia V; Tatarinov, Danila A; Parfenov, Peter S; Kurshanov, Danil A; Ismagilov, Azat O; Koroleva, Aleksandra V; Danilov, Denis V; Zhizhin, Evgeniy V; Mikushev, Sergey V; Tcypkin, Anton N; Fedorov, Anatoly V; Litvin, Aleksandr P.
Afiliación
  • Skurlov ID; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
  • Sokolova AV; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
  • Tatarinov DA; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
  • Parfenov PS; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
  • Kurshanov DA; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
  • Ismagilov AO; Laboratory of Quantum Processes and Measurements, ITMO University, 197101 Saint Petersburg, Russia.
  • Koroleva AV; Research Park, Saint Petersburg State University, 199034 Saint Petersburg, Russia.
  • Danilov DV; Research Park, Saint Petersburg State University, 199034 Saint Petersburg, Russia.
  • Zhizhin EV; Research Park, Saint Petersburg State University, 199034 Saint Petersburg, Russia.
  • Mikushev SV; Research Park, Saint Petersburg State University, 199034 Saint Petersburg, Russia.
  • Tcypkin AN; Laboratory of Quantum Processes and Measurements, ITMO University, 197101 Saint Petersburg, Russia.
  • Fedorov AV; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
  • Litvin AP; PhysNano Department, ITMO University, 197101 Saint Petersburg, Russia.
Materials (Basel) ; 15(21)2022 Nov 01.
Article en En | MEDLINE | ID: mdl-36363269
ABSTRACT
Lead halide perovskite nanoplatelets (NPls) attract significant attention due to their exceptional and tunable optical properties. Doping is a versatile strategy for modifying and improving the optical properties of colloidal nanostructures. However, the protocols for B-site doping have been rarely reported for 2D perovskite NPls. In this work, we investigated the post-synthetic treatment of CsPbBr3 NPls with different Cd2+ sources. We show that the interplay between Cd2+ precursor, NPl concentrations, and ligands determines the kinetics of the doping process. Optimization of the treatment allows for the boosting of linear and nonlinear optical properties of CsPbBr3 NPls via doping or/and surface passivation. At a moderate doping level, both the photoluminescence quantum yield and two-photon absorption cross section increase dramatically. The developed protocols of post-synthetic treatment with Cd2+ facilitate further utilization of perovskite NPls in nonlinear optics, photonics, and lightning.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Guideline Idioma: En Revista: Materials (Basel) Año: 2022 Tipo del documento: Article País de afiliación: Rusia

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Guideline Idioma: En Revista: Materials (Basel) Año: 2022 Tipo del documento: Article País de afiliación: Rusia
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