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A non-centrosymmetric chalcohalide synthesized through the combination of chemical tailoring with aliovalent substitution.
Song, Yufei; Qian, Zhen; Zhou, Boru; Yu, Hongwei; Hu, Zhanggui; Wang, Jiyang; Wu, Yicheng; Wu, Hongping.
Afiliación
  • Song Y; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Qian Z; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Zhou B; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Yu H; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Hu Z; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Wang J; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Wu Y; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
  • Wu H; Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystal, Tianjin University of Technology, Tianjin 300384, China. wuhp@ms.xjb.ac.cn.
Chem Commun (Camb) ; 59(22): 3309-3312, 2023 Mar 14.
Article en En | MEDLINE | ID: mdl-36847600
A new non-centrosymmetric (NCS) chalcohalide, [Sr4Cl2][Ge3S9], was successfully designed and synthesized through combining chemical tailoring with aliovalent substitution strategies from the maternal [NaSr4Cl][Ge3S10]. It can exhibit a large SHG effect (0.97 × AgGaS2), a wide band gap of 3.71 eV, and a high LDT (∼16 × AgGaS2). These results indicate that [Sr4Cl2][Ge3S9] may be a potential infrared nonlinear optical crystal.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2023 Tipo del documento: Article País de afiliación: China Pais de publicación: Reino Unido
Texto completo
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XML
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2023 Tipo del documento: Article País de afiliación: China Pais de publicación: Reino Unido