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Solar Hydrocarbons: Single-Step, Atmospheric-Pressure Synthesis of C2 -C4 Alkanes and Alkenes from CO2.
Song, Rui; Li, Zhao; Guo, Jiuli; Duchesne, Paul N; Qiu, Chenyue; Mao, Chengliang; Jia, Jia; Tang, Sanli; Xu, Yang-Fan; Zhou, Wenzhe; Wang, Lu; Sun, Wei; Yan, Xiaoliang; Guo, Liejin; Jing, Dengwei; Ozin, Geoffrey A.
Afiliación
  • Song R; International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China.
  • Li Z; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Guo J; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Duchesne PN; School of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan, 455000, P. R. China.
  • Qiu C; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Mao C; Department of Materials Science and Engineering, University of Toronto, Toronto, Ontario, M5S 3E4, Canada.
  • Jia J; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Tang S; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Xu YF; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Zhou W; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Wang L; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Sun W; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Yan X; State Key Laboratory of Silicon Materials and School of Materials Science and Engineering, Zhejiang University, Hangzhou, Zhejiang, 310058, China.
  • Guo L; Solar Fuels Group, Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6, Canada.
  • Jing D; International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China.
  • Ozin GA; International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China.
Angew Chem Int Ed Engl ; 62(27): e202304470, 2023 Jul 03.
Article en En | MEDLINE | ID: mdl-37137871
ABSTRACT
Cobalt ferrite (CoFe2 O4 ) spinel has been found to produce C2 -C4 hydrocarbons in a single-step, ambient-pressure, photocatalytic hydrogenation of CO2 with a rate of 1.1 mmol g-1 h-1 , selectivity of 29.8 % and conversion yield of 12.9 %. On stream the CoFe2 O4 reconstructs to a CoFe-CoFe2 O4 alloy-spinel nanocomposite which facilitates the light-assisted transformation of CO2 to CO and hydrogenation of the CO to C2 -C4 hydrocarbons. Promising results obtained from a laboratory demonstrator bode well for the development of a solar hydrocarbon pilot refinery.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Angew Chem Int Ed Engl Año: 2023 Tipo del documento: Article País de afiliación: China
Texto completo
Añadir a Mi BVS
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Angew Chem Int Ed Engl Año: 2023 Tipo del documento: Article País de afiliación: China