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Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavity.
Zhang, Hongbo; Wen, Wen; Du, Bowen; Zhou, Lei; Chen, Yu; Feng, Shun; Zou, Chenji; Wu, Lishu; Fan, Hong Jin; Gao, Weibo; Sun, Handong; Shang, Jingzhi; Yu, Ting.
Afiliación
  • Zhang H; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Wen W; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Du B; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Zhou L; College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China.
  • Chen Y; School of Chemical Engineering and Technology, Sun Yat-Sen University, Zhuhai 519082, PR China.
  • Feng S; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Zou C; Commonwealth Scientific and Industrial Research Organisation (CSIRO) Manufacturing, Clayton, Victoria 3168, Australia.
  • Wu L; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Fan HJ; Institute of Photonics and Quantum Sciences, SUPA, Heriot-Watt University, Edinburgh EH14 4AS, UK.
  • Gao W; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Sun H; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Shang J; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
  • Yu T; Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore. hdsun@ntu.edu.sg.
Nanoscale Horiz ; 8(10): 1403-1410, 2023 Sep 26.
Article en En | MEDLINE | ID: mdl-37482887
All-inorganic cesium lead bromide (CsPbBr3) quantum dots (QDs) with high photoluminescence (PL) quantum efficiency have been reported as ideal gain materials for high-performance lasers. Nevertheless, isolated CsPbBr3 QDs have not achieved lasing emission (LE) due to finite absorption cross-section. Here, we demonstrate continuous-wave lasing of isolated CsPbBr3 QDs embedded in a microcavity. Distributed Bragg reflectors (DBRs), together with isolated CsPbBr3 QDs in a polymer matrix, are introduced to construct a vertical-cavity surface-emitting laser (VCSEL), which exhibits stable single-mode lasing emissions with an ultra-low threshold of 8.8 W cm-2 and a high Q factor of 1787. Such perovskite-based microcavity structures sustain highly stable excitons at room temperature and can provide an excellent experimental platform to further study the single-particle nano-lasers and quantum physics frontiers such as exciton-polariton condensation, single-photon emission, and optical quantum communication.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nanoscale Horiz Año: 2023 Tipo del documento: Article País de afiliación: Singapur Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nanoscale Horiz Año: 2023 Tipo del documento: Article País de afiliación: Singapur Pais de publicación: Reino Unido