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Unexpected and divergent mechanosynthesis of furanoid-bridged fullerene dimers C120O and C120O2.
Shao, Gang; Liu, Yuan-Yuan; Niu, Chuang; Yin, Zheng-Chun; Ye, Shi-Qi; Yao, Yang-Rong; Chen, Muqing; Chen, Jun-Shen; Xia, Xu-Ling; Yang, Shangfeng; Wang, Guan-Wu.
Afiliación
  • Shao G; Hefei National Research Center for Physical Sciences at Microscale and Department of Chemistry, University of Science and Technology of China Hefei Anhui 230026 P. R. China gwang@ustc.edu.cn.
  • Liu YY; Hefei National Research Center for Physical Sciences at Microscale and Department of Chemistry, University of Science and Technology of China Hefei Anhui 230026 P. R. China gwang@ustc.edu.cn.
  • Niu C; Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecule-Based Materials, and School of Chemistry and Materials Science, Anhui Normal University Wuhu Anhui 241002 P. R. China.
  • Yin ZC; Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecule-Based Materials, and School of Chemistry and Materials Science, Anhui Normal University Wuhu Anhui 241002 P. R. China.
  • Ye SQ; Hefei National Research Center for Physical Sciences at Microscale and Department of Chemistry, University of Science and Technology of China Hefei Anhui 230026 P. R. China gwang@ustc.edu.cn.
  • Yao YR; Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, and Department of Materials Science and Engineering, University of Science and Technology of China Hefei Anhui 230026 P. R. China sfyang@ustc.edu.cn.
  • Chen M; School of Environment and Civil Engineering, Dongguan University of Technology Dongguan Guangdong 523808 P. R. China.
  • Chen JS; Hefei National Research Center for Physical Sciences at Microscale and Department of Chemistry, University of Science and Technology of China Hefei Anhui 230026 P. R. China gwang@ustc.edu.cn.
  • Xia XL; Hefei National Research Center for Physical Sciences at Microscale and Department of Chemistry, University of Science and Technology of China Hefei Anhui 230026 P. R. China gwang@ustc.edu.cn.
  • Yang S; Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, and Department of Materials Science and Engineering, University of Science and Technology of China Hefei Anhui 230026 P. R. China sfyang@ustc.edu.cn.
  • Wang GW; Hefei National Research Center for Physical Sciences at Microscale and Department of Chemistry, University of Science and Technology of China Hefei Anhui 230026 P. R. China gwang@ustc.edu.cn.
Chem Sci ; 2024 Aug 16.
Article en En | MEDLINE | ID: mdl-39246362
ABSTRACT
An unexpected, divergent and efficient approach toward furanoid-bridged fullerene dimers C120O and C120O2 was established under different solvent-free ball-milling conditions by simply using pristine C60 as the starting material, water as the oxygen source and FeCl3 as the mediator. The structures of C120O and C120O2 were unambiguously established by single-crystal X-ray crystallography. A plausible reaction mechanism is proposed on the basis of control experiments. Furthermore, C120O2 has been applied in organic solar cells as the third component and exhibits good performance.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Sci Año: 2024 Tipo del documento: Article Pais de publicación: Reino Unido
Texto completo
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Sci Año: 2024 Tipo del documento: Article Pais de publicación: Reino Unido