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Nuclei engineering for even halide distribution in stable perovskite/silicon tandem solar cells.
Chen, Yihua; Yang, Ning; Zheng, Guanhaojie; Pei, Fengtao; Zhou, Wentao; Zhang, Yu; Li, Liang; Huang, Zijian; Liu, Guilin; Yin, Ruiyang; Zhou, Huanping; Zhu, Cheng; Song, Tinglu; Hu, Chun; Zheng, Dezhi; Bai, Yang; Duan, Ye; Ye, Yakuan; Wu, Yiliang; Chen, Qi.
Affiliation
  • Chen Y; School of Materials Science and Engineering, Beijing Institute of Technology (Zhuhai), Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Yang N; School of Materials Science and Engineering, Beijing Institute of Technology (Zhuhai), Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Zheng G; Shanghai Synchrotron Radiation Facility (SSRF), Zhangjiang Laboratory, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201204, P. R. China.
  • Pei F; School of Materials Science and Engineering, Beijing Institute of Technology (Zhuhai), Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Zhou W; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Zhang Y; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Li L; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Huang Z; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Liu G; School of Science, Jiangnan University, Wuxi 214122, P. R. China.
  • Yin R; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Zhou H; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Zhu C; School of Materials Science and Engineering, Beijing Institute of Technology (Zhuhai), Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Song T; Advanced Research Institute of Multidisciplinary Sciences, MIIT Key Laboratory of Complex-field Intelligent Exploration, State Key Laboratory of CNS/ATM, Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Hu C; School of Materials Science and Engineering, Beijing Institute of Technology (Zhuhai), Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Zheng D; Advanced Research Institute of Multidisciplinary Sciences, MIIT Key Laboratory of Complex-field Intelligent Exploration, State Key Laboratory of CNS/ATM, Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Bai Y; Advanced Research Institute of Multidisciplinary Sciences, MIIT Key Laboratory of Complex-field Intelligent Exploration, State Key Laboratory of CNS/ATM, Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Duan Y; School of Materials Science and Engineering, Beijing Institute of Technology (Zhuhai), Beijing Institute of Technology, Beijing 100081, P. R. China.
  • Ye Y; Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, School of Materials Science and Engineering, Peking University, Beijing 100871, P. R. China.
  • Wu Y; Auner Technology Co., Ltd., Beijing 100081, China.
  • Chen Q; Auner Technology Co., Ltd., Beijing 100081, China.
Science ; 385(6708): 554-560, 2024 Aug 02.
Article in En | MEDLINE | ID: mdl-39088618
ABSTRACT
Wide-bandgap (WBG) absorbers in tandem configurations suffer from poor crystallinity and weak texture, which leads to severe mixed halide-cation ion migration and phase segregation during practical operation. We control WBG film growth insensitive to compositions by nucleating the 3C phase before any formation of bromine-rich aggregates and 2H phases. The resultant WBG absorbers show improved crystallinity and strong texture with suppressed nonradiative recombination and enhanced resistance to various aging stresses. Perovskite/silicon tandem solar cells achieve power conversion efficiencies of 29.4% (28.8% assessed by a third party) in a 25-square centimeter active area and 32.5% in a 1-square centimeter active area. These solar cells retained 98.3 and 90% of the original efficiency after 1301 and 800 hours of operation at 25° and 50°C, respectively, at the maximum power point (AM 1.5G illumination, full spectrum, 1-sun) when encapsulated.
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Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Science Year: 2024 Document type: Article Country of publication:
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Add to My VHL
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Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Science Year: 2024 Document type: Article Country of publication: