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Controlled Homoepitaxial Growth of Hybrid Perovskites.
Lei, Yusheng; Chen, Yimu; Gu, Yue; Wang, Chunfeng; Huang, Zhenlong; Qian, Haoliang; Nie, Jiuyuan; Hollett, Geoff; Choi, Woojin; Yu, Yugang; Kim, NamHeon; Wang, Chonghe; Zhang, Tianjiao; Hu, Hongjie; Zhang, Yunxi; Li, Xiaoshi; Li, Yang; Shi, Wanjun; Liu, Zhaowei; Sailor, Michael J; Dong, Lin; Lo, Yu-Hwa; Luo, Jian; Xu, Sheng.
Affiliation
  • Lei Y; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Chen Y; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Gu Y; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Wang C; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Huang Z; The Key Laboratory of Materials Processing and Mold of Ministry of Education, School of Materials Science and Engineering, Zhengzhou University, Zhengzhou, Henan, 450001, P. R. China.
  • Qian H; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Nie J; School of Microelectronics and Solid State Electronics, University of Electronic Science and Technology of China, Chengdu, Sichuan, 611731, P. R. China.
  • Hollett G; Department of Electrical and Computer Engineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Choi W; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Yu Y; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Kim N; Department of Electrical and Computer Engineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Wang C; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Zhang T; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Hu H; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Zhang Y; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Li X; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Li Y; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Shi W; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Liu Z; Department of Nanoengineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Sailor MJ; Zhejiang Research Institute of Chemical Industry, Hangzhou, Zhejiang, 310023, P. R. China.
  • Dong L; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Lo YH; Department of Electrical and Computer Engineering, University of California San Diego, La Jolla, CA, 92093, USA.
  • Luo J; Materials Science and Engineering Program, University of California San Diego, La Jolla, CA, 92093, USA.
  • Xu S; Department of Chemistry and Biochemistry, University of California San Diego, La Jolla, CA, 92093, USA.
Adv Mater ; 30(20): e1705992, 2018 May.
Article in En | MEDLINE | ID: mdl-29611280
Organic-inorganic hybrid perovskites have demonstrated tremendous potential for the next-generation electronic and optoelectronic devices due to their remarkable carrier dynamics. Current studies are focusing on polycrystals, since controlled growth of device compatible single crystals is extremely challenging. Here, the first chemical epitaxial growth of single crystal CH3 NH3 PbBr3 with controlled locations, morphologies, and orientations, using combined strategies of advanced microfabrication, homoepitaxy, and low temperature solution method is reported. The growth is found to follow a layer-by-layer model. A light emitting diode array, with each CH3 NH3 PbBr3 crystal as a single pixel, with enhanced quantum efficiencies than its polycrystalline counterparts is demonstrated.
Key words

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Adv Mater Journal subject: BIOFISICA / QUIMICA Year: 2018 Document type: Article Affiliation country: Country of publication:

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Adv Mater Journal subject: BIOFISICA / QUIMICA Year: 2018 Document type: Article Affiliation country: Country of publication: