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Coexistence of long-range antiferromagnetic order and slow relaxation of the magnetization in the first lanthanide complex of a 1,2,4-benzotriazinyl radical.
Morgan, Ian S; Mansikkamäki, Akseli; Rouzières, Mathieu; Clérac, Rodolphe; Tuononen, Heikki M.
Afiliação
  • Morgan IS; Department of Chemistry, Nanoscience Centre, University of Jyväskylä, P.O. Box 35, FI-40014, Finland. ian.s.morgan@jyu.fi heikki.m.tuononen@jyu.fi.
Dalton Trans ; 46(38): 12790-12793, 2017 Oct 14.
Artigo em Inglês | MEDLINE | ID: mdl-28932832
ABSTRACT
The first lanthanide complex of a 1,2,4-benzotriazinyl radical (1), Dy(1)(tbacac)3 (2, tbacac = 2,2,6,6-tetramethyl-3,5-heptane-dionato), was synthesised and found to have an antiferromagnetically ordered ground state with a metamagnetic phase diagram and a critical field of 0.91 T at 1.85 K. The application of a small dc field revealed the single-molecule magnet behaviour of 2, illustrating the coexistence of long-range antiferromagnetic order and slow relaxation of the magnetization.

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Texto completo: Disponível Coleções: Bases de dados internacionais Base de dados: MEDLINE Idioma: Inglês Revista: Dalton Trans Assunto da revista: Química Ano de publicação: 2017 Tipo de documento: Artigo