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Does the thermal evolution of molecular structures critically affect the magnetic anisotropy?
Chem Sci ; 6(8): 4587-4593, 2015 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-29568416
ABSTRACT
A dysprosium based single-ion magnet is synthesized and characterized by the angular dependence of the single-crystal magnetic susceptibility. Ab initio and effective electrostatic analyses are performed using the molecular structures determined from single crystal X-ray diffraction at 20 K, 100 K and 300 K. Contrary to the common assumption, the results reveal that the structural thermal effects that may affect the energy level scheme and magnetic anisotropy below 100 K are negligible.

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Texto completo: Disponível Coleções: Bases de dados internacionais Base de dados: MEDLINE Idioma: Inglês Revista: Chem Sci Ano de publicação: 2015 Tipo de documento: Artigo