Observation of chiral state transfer without encircling an exceptional point.

The adiabatic theorem, a corollary of the Schrödinger equation, manifests itself in a profoundly different way in non-Hermitian arrangements, resulting in counterintuitive state transfer schemes that have no counterpart in closed quantum systems. In particular, the dynamical encirclement of exceptional points (EPs) in parameter space has been shown to lead to a chiral phase accumulation, non-adiabatic jumps and topological mode conversion1-8. Recent theoretical studies, however, have shown that contrary to previously established demonstrations, this behaviour is not strictly a result of winding around a non-Hermitian degeneracy9. Instead, it seems to be mostly attributed to the non-trivial landscape of the Riemann surfaces, sometimes because of the presence of an EP in the vicinity9-11. Here, in an effort to bring this counterintuitive aspect of non-Hermitian systems to light and confirm this hypothesis, we provide a set of experiments to directly observe the field evolution and chiral state conversion in an EP-excluding cycle in a slowly varying non-Hermitian system. To do so, a versatile yet unique fibre-based photonic emulator is realized that utilizes the polarization degrees of freedom in a quasi-common-path single-ring arrangement. Our observations may open up new avenues for light manipulation and state conversion, as well as providing a foundation for understanding the intricacies of the adiabatic theorem in non-Hermitian systems.

Video-rate Raman-based metabolic imaging by Airy light-sheet illumination and photon-sparse detection.

Despite its massive potential, Raman imaging represents just a modest fraction of all research and clinical microscopy to date. This is due to the ultralow Raman scattering cross-sections of most biomolecules that impose low-light or photon-sparse conditions. Bioimaging under such conditions is suboptimal, as it either results in ultralow frame rates or requires increased levels of irradiance. Here, we overcome this tradeoff by introducing Raman imaging that operates at both video rates and 1,000-fold lower irradiance than state-of-the-art methods. To accomplish this, we deployed a judicially designed Airy light-sheet microscope to efficiently image large specimen regions. Further, we implemented subphoton per pixel image acquisition and reconstruction to confront issues arising from photon sparsity at just millisecond integrations. We demonstrate the versatility of our approach by imaging a variety of samples, including the three-dimensional (3D) metabolic activity of single microbial cells and the underlying cell-to-cell variability. To image such small-scale targets, we again harnessed photon sparsity to increase magnification without a field-of-view penalty, thus, overcoming another key limitation in modern light-sheet microscopy.

Non-Hermitian ring laser gyroscopes with enhanced Sagnac sensitivity.

Gyroscopes are essential to many diverse applications associated with navigation, positioning and inertial sensing1. In general, most optical gyroscopes rely on the Sagnac effect-a relativistically induced phase shift that scales linearly with the rotational velocity2,3. In ring laser gyroscopes (RLGs), this shift manifests as a resonance splitting in the emission spectrum, which can be detected as a beat frequency4. The need for ever more precise RLGs has fuelled research activities aimed at boosting the sensitivity of RLGs beyond the limits dictated by geometrical constraints, including attempts to use either dispersive or nonlinear effects5-8. Here we establish and experimentally demonstrate a method using non-Hermitian singularities, or exceptional points, to enhance the Sagnac scale factor9-13. By exploiting the increased rotational sensitivity of RLGs in the vicinity of an exceptional point, we enhance the resonance splitting by up to a factor of 20. Our results pave the way towards the next generation of ultrasensitive and compact RLGs and provide a practical approach for the development of other classes of integrated sensor.

Observation of Weyl exceptional rings in thermal diffusion.

SignificanceThermal diffusion is dissipative and strongly related to non-Hermitian physics. At the same time, non-Hermitian Weyl systems have spurred tremendous interest across photonics and acoustics. This correlation has been long ignored and hence shed little light upon the question of whether the Weyl exceptional ring (WER) in thermal diffusion could exist. Intuitively, thermal diffusion provides no real parameter dimensions, thus prohibiting a topological nature and WER. This work breaks this perception by imitating synthetic dimensions via two spatiotemporal advection pairs. The WER is achieved in thermal diffusive systems. Both surface-like and bulk states are demonstrated by coupling two WERs with opposite topological charges. These findings extend topological notions to diffusions and motivate investigation of non-Hermitian diffusive and dissipative control.

Statistical mechanics and pressure of composite multimoded weakly nonlinear optical systems.

Statistical mechanics can provide a versatile theoretical framework for investigating the collective dynamics of weakly nonlinear-wave settings that can be utterly complex to describe otherwise. In optics, composite systems arise due to interactions between different frequencies and polarizations. The purpose of this work is to develop a thermodynamic theory that takes into account the synergistic action of multiple components. We find that the type of the nonlinearity involved can have important implications in the thermalization process and, hence, can lead to different thermal equilibrium conditions. Importantly, we derive closed-form expressions for the actual optomechanical pressure that is exerted on the system. In particular, the total optomechanical pressure is the sum of the partial pressures due to each component. Our results can be applied to a variety of weakly nonlinear optical settings such as multimode fibers, bulk waveguides, photonic lattices, and coupled microresonators. We present two specific examples, where two colors interact in a one-waveguide array with either a cubic or quadratic nonlinearity.

Dalton's law of partial optical thermodynamic pressures in highly multimoded nonlinear photonic systems.

We show that in highly multimoded nonlinear photonic systems, the optical thermodynamic pressures emerging from different species of the optical field obey Dalton's law of partial pressures. In multimode settings, the optical thermodynamic pressure is defined as the conjugate to the extensive variable associated with the system's total number of modes and is directly related to the actual electrodynamic radiation forces exerted at the physical boundaries of the system. Here, we extend this notion to photonic configuration supporting different species of the optical field. Under thermal equilibrium conditions, we formally derive an equation that establishes a direct link between the partial thermodynamic pressures and the electrodynamic radiation pressures exerted by each polarization species. Our theoretical framework provides a straightforward approach for quantifying the total radiation pressures through the system's thermodynamic variables without invoking the Maxwell stress tensor formalism. In essence, we show that the total electrodynamic pressure in such arrangements can be obtained in an effortless manner from initial excitation conditions, thus avoiding time-consuming simulations of the utterly complex multimode dynamics. To illustrate the validity of our results, we carry out numerical simulations in multimoded nonlinear optical structures supporting two polarization species and demonstrate excellent agreement with the Maxwell stress tensor method.

Spatiotemporal Single-Photon Airy Bullets.

Uninhibited control of the complex spatiotemporal quantum wave function of a single photon has so far remained elusive even though it can dramatically increase the encoding flexibility and thus the information capacity of a photonic quantum link. By fusing temporal waveform generation in an atomic ensemble and spatial single-photon shaping, we hereby demonstrate for the first time complete spatiotemporal control of a propagation invariant (2+1)D Airy single-photon optical bullet. These correlated photons are not only self-accelerating and impervious to spreading as their classical counterparts, but can be concealed and revealed in the presence of strong classical stray light.

Flying couplers above spinning resonators generate irreversible refraction.

Creating optical components that allow light to propagate in only one direction-that is, that allow non-reciprocal propagation or 'isolation' of light-is important for a range of applications. Non-reciprocal propagation of sound can be achieved simply by using mechanical components that spin1,2. Spinning also affects de Broglie waves 3 , so a similar idea could be applied in optics. However, the extreme rotation rates that would be required, owing to light travelling much faster than sound, lead to unwanted wobbling. This wobbling makes it difficult to maintain the separation between the spinning devices and the couplers to within tolerance ranges of several nanometres, which is essential for critical coupling4,5. Consequently, previous applications of optical6-17 and optomechanical10,17-20 isolation have used alternative methods. In hard-drive technology, the magnetic read heads of a hard-disk drive fly aerodynamically above the rapidly rotating disk with nanometre precision, separated by a thin film of air with near-zero drag that acts as a lubrication layer 21 . Inspired by this, here we report the fabrication of photonic couplers (tapered fibres that couple light into the resonators) that similarly fly above spherical resonators with a separation of only a few nanometres. The resonators spin fast enough to split their counter-circulating optical modes, making the fibre coupler transparent from one side while simultaneously opaque from the other-that is, generating irreversible transmission. Our setup provides 99.6 per cent isolation of light in standard telecommunication fibres, of the type used for fibre-based quantum interconnects 22 . Unlike flat geometries, such as between a magnetic head and spinning disk, the saddle-like, convex geometry of the fibre and sphere in our setup makes it relatively easy to bring the two closer together, which could enable surface-science studies at nanometre-scale separations.

Bimorphic Floquet topological insulators.

Topological theories have established a unique set of rules that govern the transport properties in a wide variety of wave-mechanical settings. In a marked departure from the established approaches that induce Floquet topological phases by specifically tailored discrete coupling protocols or helical lattice motions, we introduce a class of bimorphic Floquet topological insulators that leverage connective chains with periodically modulated on-site potentials to reveal rich topological features in the system. In exploring a 'chain-driven' generalization of the archetypical Floquet honeycomb lattice, we identify a rich phase structure that can host multiple non-trivial topological phases associated simultaneously with both Chern-type and anomalous chiral states. Experiments carried out in photonic waveguide lattices reveal a strongly confined helical edge state that, owing to its origin in bulk flat bands, can be set into motion in a topologically protected fashion, or halted at will, without compromising its adherence to individual lattice sites.

Nature of Optical Thermodynamic Pressure Exerted in Highly Multimoded Nonlinear Systems.

The theory of optical thermodynamics provides a comprehensive framework that enables a self-consistent description of the intricate dynamics of nonlinear multimoded photonic systems. This theory, among others, predicts a pressurelike intensive quantity (p[over ^]) that is conjugate to the system's total number of modes (M)-its corresponding extensive variable. Yet at this point, the nature of this intensive quantity is still nebulous. In this Letter, we elucidate the physical origin of the optical thermodynamic pressure and demonstrate its dual essence. In this context, we rigorously derive an expression that splits p[over ^] into two distinct components, a term that is explicitly tied to the electrodynamic radiation pressure and a second entropic part that is responsible for the entropy change. We utilize this result to establish a formalism that simplifies the quantification of radiation pressure under nonlinear equilibrium conditions, thus eliminating the need for a tedious evaluation of the Maxwell stress tensor. Our theoretical analysis is corroborated by numerical simulations carried out in highly multimoded nonlinear optical structures. These results may provide a novel way in predicting and controlling radiation pressure processes in a variety of nonlinear electromagnetic settings.

Enhanced sensitivity at higher-order exceptional points.

Non-Hermitian degeneracies, also known as exceptional points, have recently emerged as a new way to engineer the response of open physical systems, that is, those that interact with the environment. They correspond to points in parameter space at which the eigenvalues of the underlying system and the corresponding eigenvectors simultaneously coalesce. In optics, the abrupt nature of the phase transitions that are encountered around exceptional points has been shown to lead to many intriguing phenomena, such as loss-induced transparency, unidirectional invisibility, band merging, topological chirality and laser mode selectivity. Recently, it has been shown that the bifurcation properties of second-order non-Hermitian degeneracies can provide a means of enhancing the sensitivity (frequency shifts) of resonant optical structures to external perturbations. Of particular interest is the use of even higher-order exceptional points (greater than second order), which in principle could further amplify the effect of perturbations, leading to even greater sensitivity. Although a growing number of theoretical studies have been devoted to such higher-order degeneracies, their experimental demonstration in the optical domain has so far remained elusive. Here we report the observation of higher-order exceptional points in a coupled cavity arrangement-specifically, a ternary, parity-time-symmetric photonic laser molecule-with a carefully tailored gain-loss distribution. We study the system in the spectral domain and find that the frequency response associated with this system follows a cube-root dependence on induced perturbations in the refractive index. Our work paves the way for utilizing non-Hermitian degeneracies in fields including photonics, optomechanics, microwaves and atomic physics.

Erratum: Enhanced sensitivity at higher-order exceptional points.

This corrects the article DOI: 10.1038/nature23280.

Direct modulation of electrically pumped coupled microring lasers.

We demonstrate how the presence of gain-loss contrast between two coupled identical resonators can be used as a new degree of freedom to enhance the modulation frequency response of laser diodes. An electrically pumped microring laser system with a bending radius of 50 µm is fabricated on an InAlGaAs/InP MQW p-i-n structure. The room temperature continuous wave (CW) laser threshold current of the device is 27 mA. By adjusting the ratio between the injection current levels in the two coupled microrings, our experimental results clearly show a bandwidth improvement by up to 1.63 times the fundamental resonant frequency of the individual device. This matches well with our rate equation simulation model.

Multimode nonlinear dynamics in spatiotemporal mode-locked anomalous-dispersion lasers.

Spatiotemporal mode-locking in a laser with anomalous dispersion is investigated. Mode-locked states with varying modal content can be observed, but we find it difficult to observe highly-multimode states. We describe the properties of these mode-locked states and compare them to the results of numerical simulations. Prospects for the generation of highly-multimode states and lasers based on multimode soliton formation are discussed.

Thermalization Dynamics of Nonlinear Non-Hermitian Optical Lattices.

We develop a rigorous theoretical framework based on principles from statistical mechanics that allows one to predict the equilibrium response of classical non-Hermitian arrangements in the weakly nonlinear regime. In this respect, we demonstrate that a pseudo-Hermitian configuration can always be driven into thermal equilibrium when a proper nonlinear operator is paired with the linear Hamiltonian of the system. We show that, in this case, the system will thermodynamically settle into an irregular pattern that does not resemble any known statistical distribution. Interestingly, this stable equilibrium response is associated with a Rayleigh-Jeans law when viewed within an appropriately transformed space that displays unitary dynamics. By considering a non-Hermitian Su-Schrieffer-Heeger chain, our results indicate that the thermodynamic equilibrium will always favor the edge modes instead of the ground state, in stark contrast to conventional nonlinear Hermitian configurations. Moreover, non-Hermitian lattices are shown to exhibit unusually high heat capacities, potentially acting as optical heat reservoirs to other Hermitian systems, by employing only a small number of sites and low power levels.

Thermalization of Light's Orbital Angular Momentum in Nonlinear Multimode Waveguide Systems.

We show that the orbital angular momentum (OAM) of a light field can be thermalized in a nonlinear cylindrical multimode optical waveguide. We find that upon thermal equilibrium, the maximization of the optical entropy leads to a generalized Rayleigh-Jeans distribution that governs the power modal occupancies with respect to the discrete OAM charge numbers. This distribution is characterized by a temperature that is by nature different from that associated with the longitudinal electromagnetic momentum flow of the optical field. Counterintuitively and in contrast to previous results, we demonstrate that even under positive temperatures, the ground state of the fiber is not always the most populated in terms of power. Instead, because of OAM, the thermalization processes may favor higher-order modes. A new equation of state is derived along with an extended Euler equation resulting from the extensivity of the entropy itself. By monitoring the nonlinear interaction between two multimode optical wave fronts with opposite spins, we show that the exchange of angular momentum is dictated by the difference in OAM temperatures, in full accord with the second law of thermodynamics. The theoretical analysis presented here is corroborated by numerical simulations that take into account the complex nonlinear dynamics of hundreds of modes. Our results may pave the way toward high-power optical sources with controllable orbital angular momenta, and at a more fundamental level, they may open up opportunities in drawing parallels with other complex multimode nonlinear systems like rotating atomic clouds.

Realizing spin Hamiltonians in nanoscale active photonic lattices.

Spin models arise in the microscopic description of magnetic materials and have been recently used to map certain classes of optimization problems involving large degrees of freedom. In this regard, various optical implementations of such Hamiltonians have been demonstrated to quickly converge to the global minimum in the energy landscape. Yet, so far, an integrated nanophotonic platform capable of emulating complex magnetic materials is still missing. Here, we show that the cooperative interplay among vectorial electromagnetic modes in coupled metallic nanolasers can be utilized to implement certain types of spin Hamiltonians. Depending on the topology/geometry of the arrays, these structures can be governed by a classical XY Hamiltonian that exhibits ferromagnetic and antiferromagnetic couplings, as well as geometrical frustration. Our results pave the way towards a scalable nanophotonic platform to study spin exchange interactions and could address a variety of optimization problems.

Scalar and vector supermode solitons owing to competing nonlocal nonlinearities.

We investigate scalar and vector multi-hump spatial solitons resulting from competing Kerr-like nonlinear responses excited in a nonlocal medium by either one or two (mutually incoherent) light beams. Two-color vector supermode solitons are more amenable to control but exhibit an intriguing form of spontaneous symmetry breaking in propagation.

Weak beam self-cleaning of femtosecond pulses in the anomalous dispersion regime.

Kerr beam cleaning in graded-index multimode fiber has been investigated in experiments with sub-nanosecond pulses and in experiments with femtosecond pulses at wavelengths where the dispersion is normal. We report a theoretical and experimental study of this effect with femtosecond pulses and anomalous dispersion. In this regime, only weak beam cleaning is observed experimentally, along with strong temporal evolution of the pulse. Numerical simulations exhibit the qualitative trends of the experiments.

Formation and stability of vortex solitons in nematic liquid crystals.

We study the propagation dynamics of bright optical vortex solitons in nematic liquid crystals with a nonlocal reorientational nonlinear response. We investigate the role of optical birefringence on the stability of these solitons. In agreement with recent experimental observations, we show that the birefringence-induced astigmatism can eventually destabilize these vortex solitons. However, for low and moderate birefringence, vortex solitons can propagate stably over experimentally relevant distances.