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1.
Phys Rev Lett ; 110(13): 137404, 2013 Mar 29.
Artigo em Inglês | MEDLINE | ID: mdl-23581371

RESUMO

We use terahertz pulses to induce resonant transitions between the eigenstates of optically generated exciton populations in a high-quality semiconductor quantum well sample. Monitoring the excitonic photoluminescence, we observe transient quenching of the 1s exciton emission, which we attribute to the terahertz-induced 1s-to-2p excitation. Simultaneously, a pronounced enhancement of the 2s exciton emission is observed, despite the 1s-to-2s transition being dipole forbidden. A microscopic many-body theory explains the experimental observations as a Coulomb-scattering mixing of the 2s and 2p states, yielding an effective terahertz transition between the 1s and 2s populations.

2.
Phys Rev Lett ; 108(26): 267402, 2012 Jun 29.
Artigo em Inglês | MEDLINE | ID: mdl-23005012

RESUMO

Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique Λ-type three-level system. Pronounced nonlinearities are observed via time-resolved strong-terahertz and weak-optical excitation spectroscopy and explained with a fully microscopic theory. The results show that the terahertz pulses strongly couple the exciton-polariton states to the 2p-exciton state while no resonant transition between the two polariton levels is observed.

3.
Opt Express ; 18(20): 20558-64, 2010 Sep 27.
Artigo em Inglês | MEDLINE | ID: mdl-20940950

RESUMO

We investigate high-Q, small mode volume photonic crystal nanobeam cavities using a curved, tapered optical microfiber loop. The strength of the coupling between the cavity and the microfiber loop is shown to depend on the contact position on the nanobeam, angle between the nanobeam and the microfiber, and polarization of the light in the fiber. The results are compared to a resonant scattering measurement.

4.
Nanotechnology ; 21(6): 065202, 2010 Feb 10.
Artigo em Inglês | MEDLINE | ID: mdl-20057040

RESUMO

In this paper, we present recent progress in the growth, modelling, fabrication and characterization of gallium arsenide (GaAs) two-dimensional (2D) photonic-crystal slab cavities with embedded indium arsenide (InAs) quantum dots (QDs) that are designed for cavity quantum electrodynamics (cQED) experiments. Photonic-crystal modelling and device fabrication are discussed, followed by a detailed discussion of different failure modes that lead to photon loss. It is found that, along with errors introduced during fabrication, other significant factors such as the presence of a bottom substrate and cavity axis orientation with respect to the crystal axis, can influence the cavity quality factor (Q). A useful diagnostic tool in the form of contour finite-difference time domain (FDTD) is employed to analyse device performance.

5.
Nature ; 432(7014): 200-3, 2004 Nov 11.
Artigo em Inglês | MEDLINE | ID: mdl-15538363

RESUMO

Cavity quantum electrodynamics (QED) systems allow the study of a variety of fundamental quantum-optics phenomena, such as entanglement, quantum decoherence and the quantum-classical boundary. Such systems also provide test beds for quantum information science. Nearly all strongly coupled cavity QED experiments have used a single atom in a high-quality-factor (high-Q) cavity. Here we report the experimental realization of a strongly coupled system in the solid state: a single quantum dot embedded in the spacer of a nanocavity, showing vacuum-field Rabi splitting exceeding the decoherence linewidths of both the nanocavity and the quantum dot. This requires a small-volume cavity and an atomic-like two-level system. The photonic crystal slab nanocavity--which traps photons when a defect is introduced inside the two-dimensional photonic bandgap by leaving out one or more holes--has both high Q and small modal volume V, as required for strong light-matter interactions. The quantum dot has two discrete energy levels with a transition dipole moment much larger than that of an atom, and it is fixed in the nanocavity during growth.

6.
Opt Express ; 17(8): 6813-28, 2009 Apr 13.
Artigo em Inglês | MEDLINE | ID: mdl-19365510

RESUMO

A detailed experimental and theoretical study of the linear and nonlinear optical properties of different Fibonacci-spaced multiple-quantum-well structures is presented. Systematic numerical studies are performed for different average spacing and geometrical arrangement of the quantum wells. Measurements of the linear and nonlinear (carrier density dependent) reflectivity are shown to be in good agreement with the computational results. As the pump pulse energy increases, the excitation-induced dephasing broadens the exciton resonances resulting in a disappearance of sharp features and reduction in peak reflectivity.


Assuntos
Cristalização , Manufaturas , Modelos Teóricos , Pontos Quânticos , Refratometria/métodos , Simulação por Computador , Luz , Dinâmica não Linear , Espalhamento de Radiação
7.
Nature ; 451(7176): 256, 2008 Jan 17.
Artigo em Inglês | MEDLINE | ID: mdl-18202634
8.
Opt Express ; 16(20): 15382-7, 2008 Sep 29.
Artigo em Inglês | MEDLINE | ID: mdl-18825174

RESUMO

The fabrication and characterization of light-emitting one-dimensional photonic quasicrystals based on excitonic resonances is reported. The structures consist of high-quality GaAs/AlGaAs quantum wells grown by molecular-beam epitaxy with wavelength-scale spacings satisfying a Fibonacci sequence. The polaritonic (resonant light-matter coupling) effects and light emission originate from the quantum well excitonic resonances. Measured reflectivity spectra as a function of detuning between emission and Bragg wavelength are in good agreement with excitonic polariton theory. Photoluminescence experiments show that active photonic quasicrystals, unlike photonic crystals, can be good light emitters: While their long-range order results in a stopband similar to that of photonic crystals, the lack of periodicity results in strong emission.


Assuntos
Cristalização/métodos , Óptica e Fotônica , Arsenicais/química , Desenho de Equipamento , Gálio/química , Luz , Fótons , Teoria Quântica
9.
Opt Express ; 16(26): 21512-21, 2008 Dec 22.
Artigo em Inglês | MEDLINE | ID: mdl-19104581

RESUMO

An instability in the growth of nonperiodic InGaAs/GaAs multiple quantum well samples, ordinarily of high-quality when grown with equal periods of order of half the wavelength of light in the material, leads to a dramatic microscopic, self-organized surface grating. This effect was discovered while growing quantum wells with two unequal barrier lengths arranged in a Fibonacci sequence to form an optical quasicrystal. A laser beam incident normal to the surface of the sample is diffracted into a propeller-shaped pattern. The sample surface has a distinctly cloudy appearance when viewed along one crystal axis but is mirror-like when the sample is rotated 90 degrees. The instability results in a five-fold increase in the absorption linewidth of the heavy-hole exciton transition. Atomic force microscopy, transmission electron microscopy, and scanning electron microscopy were used to study the samples.

10.
Opt Express ; 14(6): 2289-99, 2006 Mar 20.
Artigo em Inglês | MEDLINE | ID: mdl-19503566

RESUMO

We report a novel hemispherical micro-cavity that is comprised of a planar integrated semiconductor distributed Bragg reflector (DBR) mirror, and an external, concave micro-mirror having a radius of curvature 50 microm. The integrated DBR mirror containing quantum dots (QD), is designed to locate the QDs at an antinode of the field in order to maximize the interaction between the QD and cavity. The concave micro-mirror, with high-reflectivity over a large solid-angle, creates a diffraction-limited (sub-micron) mode-waist at the planar mirror, leading to a large coupling constant between the cavity mode and QD. The half-monolithic design gives more spatial and spectral tuning abilities, relatively to fully monolithic structures. This unique micro-cavity design will potentially enable us to both reach the cavity quantum electrodynamics (QED) strong coupling regime and realize the deterministic generation of single photons on demand.

11.
Nat Mater ; 5(7): 523-31, 2006 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-16819475

RESUMO

Excitons are quasi-particles that form when Coulomb-interacting electrons and holes in semiconductors are bound into pair states. They have many features analogous to those of atomic hydrogen. Because of this, researchers are interested in exploring excitonic phenomena, from optical, quantum-optical and thermodynamic transitions to the possible condensation of excitons into a quantum-degenerate state. Excitonic signatures commonly appear in the optical absorption and emission of direct-gap semiconductor systems. However, the precise properties of incoherent exciton populations in such systems are difficult to determine and are the subject of intense debate. We review recent contributions to this discussion, and argue that to obtain detailed information about exciton populations, conventional experimental techniques should be supplemented by direct quasi-particle spectroscopy using the relatively newly available terahertz light sources. Finally, we propose a scheme of quantum-optical excitation to generate quantum-degenerate exciton states directly.

12.
Opt Lett ; 10(5): 220-2, 1985 May 01.
Artigo em Inglês | MEDLINE | ID: mdl-19724400

RESUMO

We report the first observation to our knowledge of mirrorless optical bistability based on a dispersive effect, namely, cross-trapping optical bistability due to the mutual interaction of two counterpropagating beams. The phase conjugation of a probe beam generated by four-wave mixing in such a system is sensitive to the intensities of the counterpropagating beams and has been used to monitor the bistability.

13.
Opt Lett ; 7(9): 429-31, 1982 Sep 01.
Artigo em Inglês | MEDLINE | ID: mdl-19714045

RESUMO

This Letter is concerned with the parallel operation of optical bistable devices. The two-beam side-by-side case has been simulated numerically. Diffraction coupling from one device operating in the upper branch can cause the other one, operating in the lower branch, to switch to the upper branch if the separation of the two beams is too small. The separation required for independent operation is usually a few beamwidths. The results give promise for performing parallel operations with optical bistable devices on the same étalon.

14.
Opt Lett ; 18(7): 494-6, 1993 Apr 01.
Artigo em Inglês | MEDLINE | ID: mdl-19802178

RESUMO

We show that bright optical pulses can be compressed in the wavelength region of normal group-velocity dispersion by using dark optical solitons. Various cases of the pulse compression are studied numerically for dark soliton pulses with a background of finite temporal duration.

15.
Opt Lett ; 14(14): 740-2, 1989 Jul 15.
Artigo em Inglês | MEDLINE | ID: mdl-19752953

RESUMO

Optical-activity-supported energy transfer is explained, and a transfer of 4% is observed in bismuth silicon oxide with same-frequency equal-intensity beams having the same circular polarization. The direction of energy exchange can be controlled by the sign of the electric field or the sense of the circularity. In general, energy exchange occurs by destructive and constructive interference between diffracted and transmitted beams; here, with the induced grating vector along the [110] direction, interference cannot occur unless optical activity and an external electric field are present.

16.
Phys Rev Lett ; 92(21): 217403, 2004 May 28.
Artigo em Inglês | MEDLINE | ID: mdl-15245317

RESUMO

We observe a triplet around the third harmonic of the semiconductor band gap when exciting 50-100 nm thin GaAs films with 5 fs pulses at 3 x 10(12) W/cm(2). The comparison with solutions of the semiconductor Bloch equations allows us to interpret the observed peak structure as being due to a two-band Mollow triplet. This triplet in the optical spectrum is a result of light-induced gaps in the band structure, which arise from coherent band mixing. The theory is formulated for full tight-binding bands and uses no rotating-wave approximation.

17.
Phys Rev Lett ; 85(14): 3041-4, 2000 Oct 02.
Artigo em Inglês | MEDLINE | ID: mdl-11005998

RESUMO

Resonance Rayleigh scattering by periodic semiconductor multiple quantum-well structures is studied experimentally and theoretically. Polaritonic effects are found to dominate disorder in the secondary emission dynamics. The coexistence of several radiant polaritonic modes with different radiative decay times leads to polarization beating between modes, strongly influences the rise times, and determines the fast decay times of the resonance Rayleigh scattered signals.

18.
Opt Lett ; 21(13): 994-6, 1996 Jul 01.
Artigo em Inglês | MEDLINE | ID: mdl-19876229

RESUMO

GaAs/AlAs microcavities containing two different quantum wells have been grown and their normal mode coupling studied. We present experimental results that exhibit three-dip reflectivity spectra characteristic of three coupled oscillators. A theoretical model based on a nonlocal dielectric response and a transfer matrix method is used to model the microcavities and yields good agreement with experiment.

19.
Phys Rev Lett ; 92(6): 067402, 2004 Feb 13.
Artigo em Inglês | MEDLINE | ID: mdl-14995274

RESUMO

Time-resolved photoluminescence spectra after nonresonant excitation show a distinct 1s resonance, independent of the existence of bound excitons. A microscopic analysis identifies exciton and electron-hole plasma contributions. For low temperatures and low densities, the excitonic emission is extremely sensitive to details of the electron-hole-pair population making it possible to identify even minute fractions of optically active excitons.

20.
Phys Rev Lett ; 93(6): 067401, 2004 Aug 06.
Artigo em Inglês | MEDLINE | ID: mdl-15323660

RESUMO

The lack of translational invariance perpendicular to the plane of a single quantum well causes equal probability for spontaneous emission to the left or right. Combining one emission path from the left and one from the right into a common detector leads to interference fringes for fundamentally indistinguishable paths corresponding to geometries where the same in-plane momentum is transferred to the quantum well. For all other paths, no interference is observed because of the entanglement between the photon and extended Bloch states of the many-body system. In multiple-quantum-well structures the interference can be controlled via the spacing between the wells.

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