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1.
Phys Rev Lett ; 127(19): 192501, 2021 Nov 05.
Artigo em Inglês | MEDLINE | ID: mdl-34797155

RESUMO

The changes in the mean-square charge radius (relative to ^{209}Bi), magnetic dipole, and electric quadrupole moments of ^{187,188,189,191}Bi were measured using the in-source resonance-ionization spectroscopy technique at ISOLDE (CERN). A large staggering in radii was found in ^{187,188,189}Bi^{g}, manifested by a sharp radius increase for the ground state of ^{188}Bi relative to the neighboring ^{187,189}Bi^{g}. A large isomer shift was also observed for ^{188}Bi^{m}. Both effects happen at the same neutron number, N=105, where the shape staggering and a similar isomer shift were observed in the mercury isotopes. Experimental results are reproduced by mean-field calculations where the ground or isomeric states were identified by the blocked quasiparticle configuration compatible with the observed spin, parity, and magnetic moment.

2.
J Chem Phys ; 154(22): 224303, 2021 Jun 14.
Artigo em Inglês | MEDLINE | ID: mdl-34241194

RESUMO

The YbOH triatomic molecule can be efficiently used to measure the electron electric dipole moment, which violates time-reversal (T) and spatial parity (P) symmetries of fundamental interactions [Kozyryev and Hutzler, Phys. Rev. Lett. 119, 133002 (2017)]. We study another mechanism of the T, P-violation in the YbOH molecule-the electron-electron interaction mediated by the low-mass axionlike particle. For this, we calculate the molecular constant that characterizes this interaction and use it to estimate the expected magnitude of the effect to be measured. It is shown that this molecular constant has the same order of magnitude as the corresponding molecular constant corresponding to the axion-mediated electron-nucleus interaction. According to our estimation, an experiment on YbOH will allow one to set updated laboratory constraints on the CP-violating electron-axion coupling constants.

3.
J Chem Phys ; 153(22): 224302, 2020 Dec 14.
Artigo em Inglês | MEDLINE | ID: mdl-33317302

RESUMO

The time-reversal and spatial parity violating interaction of the nuclear magnetic quadrupole moment (MQM) of the 175Lu and 176Lu nuclei with electrons in the molecular cation LuOH+ is studied. The resulting effect is expressed in terms of fundamental parameters, such as quantum chromodynamics angle θ¯, quark electric dipole moment (EDM), and chromo-EDM. For this, we have estimated the magnetic quadrupole moments of 175Lu and 176Lu nuclei and calculated the molecular constant that characterizes the interaction of the MQM with electrons in the considered molecules. Additionally, we predict the hyperfine structure constants for the ground electronic state of LuOH+. In the molecular calculations, both the correlation and relativistic effects including the Gaunt interaction have been considered. According to the calculated expressions in terms of the fundamental constants, we conclude that LuOH+ can be a promising system to measure the nuclear MQM.

4.
J Chem Phys ; 152(4): 044301, 2020 Jan 31.
Artigo em Inglês | MEDLINE | ID: mdl-32007077

RESUMO

The influence of the nuclear magnetization distribution effects on the hyperfine structure of electronic states of thallium atom is studied within the relativistic coupled cluster theory. Relative significance of these effects is demonstrated for the first excited electronic state 6P3/2 of neutral Tl. Based on the obtained theoretical and available experimental data, the nuclear magnetic moments of short-lived 191Tlm and 193Tlm isotopes are predicted: µ191 = 3.79(2) µN and µ193 = 3.84(3) µN, respectively. Using theoretical and experimental data for the neutral Tl, the magnetic anomalies 205Δ203 for the 7S1/2 state of the neutral Tl atom and the 1S1/2 state of the hydrogen-like ion are also predicted.

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