Near-infrared imaging via upconversion in Er3+:CaF2 crystal with dual wavelength excitation.

We propose a system for imaging 1510 nm near-infrared (NIR) wavelength via upconversion (UC) luminescence in an Er3+-doped CaF2 crystal. Er3+ ions are excited from the ground to the excited state levels by an 800-nm pre-excitation wavelength, followed by the promotion of these ions to a higher energy level by the NIR excitation wavelength. Relaxation of these excited ions gives rise to 540 nm UC luminescence in the visible region, enabling the detection of the 1510 nm NIR wavelength. Using this UC scheme, 1510 nm was successfully imaged. Our system enables imaging of NIR wavelengths using low-cost optics and readily available Si-based detectors that are sensitive only to visible wavelengths, opening new possibilities for detection and imaging of NIR wavelengths.

Mid-infrared imaging through up-conversion luminescence in trivalent lanthanide ion-doped self-organizing optical fiber array crystal.

We propose a scheme for imaging mid-infrared (MIR) wavelengths via pre-excitation-assisted up-conversion luminescence in lanthanide ion (Ln3+)-doped Self-organizing Optical FIber Array (SOFIA) crystal. First, near-infrared pre-excitation wavelength excites an electron from the ground state to an excited state of Ln3+. Next, the MIR wavelength to be imaged promotes this excited electron to a higher-lying energy state. Finally, relaxation of the electron from the higher-lying energy state to the ground state emits the up-conversion luminescence in the visible region, completing the MIR-to-visible wavelength conversion. An analysis of the 4f to 4f intra-configurational energy level transitions in Ln3+, together with an appropriate selection of the pre-excitation wavelength and the visible luminescence constrained within the 500-700 nm wavelength range, reveals that trivalent erbium (Er3+), thulium (Tm3+), holmium (Ho3+), and neodymium (Nd3+) can be used to image MIR wavelengths. Our proposed scheme, called MIR imAging through up-Conversion LuminEscence in a SOFIA crystal, will enable the imaging of MIR wavelengths using low-cost optics and readily available silicon-based detectors in the visible spectral region and will open up new possibilities for MIR wavelength detection and imaging.

Tunable vacuum ultraviolet cross-luminescence from KMgF under high pressure as potential fast-response scintillator.

We report on the potential of the potassium magnesium fluoride (KMgF) crystal as a fast-response scintillator with tunable cross-luminescence (CL) emission wavelength through high-pressure applications. By performing first-principles density functional theory calculations using the Perdew-Burke-Ernzerhof (PBE) hybrid functional including exact exchange (PBE0) and Green's function and screened Coulomb interaction approximation as implemented in the Vienna Ab initio Simulation Package using plane-wave basis sets within the projector-augmented wave method, we identify the specific valence-to-core band transition that results in the experimentally observed CL emission at 148 nm (8.38 eV) and 170 nm (7.29 eV) wavelengths with intrinsically fast decay times of 290 ps and 210 ps, respectively. Uniform volume compression through hydrostatic high-pressure applications could decrease the energy gap between the valence and core bands, potentially shifting the CL emission wavelength to the ultraviolet (UV) region from 200 nm (6.2 eV) to 300 nm (4.1 eV). The ability to tune and shift the CL emission to UV wavelengths allows for the detection of the CL emission using UV-sensitive photodetectors in ambient atmosphere instead of highly specialized vacuum UV detectors operating in vacuum while maintaining the intrinsically fast CL decay times, thereby opening up new possibilities for KMgF as a fast-response scintillator.

Enhancing terahertz magnetic near field induced by a micro-split-ring resonator with a tapered waveguide.

Substantial enhancement of terahertz magnetic near field achieved by the combination of a tapered metallic waveguide and a micro-split-ring resonator is demonstrated. The magnetic near field is probed directly via the magneto-optic sampling with a Tb3Ga5O12 crystal. The incident terahertz wave with a half-cycle waveform is generated by using the pulse-front tilting method. The magnetic near field at the resonant frequency is enhanced by more than 30 times through the combination of the waveguide and the resonator. The peak amplitude of the magnetic field with a damped oscillation waveform in the time domain is up to 0.4 T. The resonant frequency can be tuned by adopting different resonator designs. The mechanism of the enhancement is analyzed by performing calculations based on the finite element method. The strong terahertz magnetic near field enables the excitation of large-amplitude spin dynamics and can be utilized for an ultrafast spin control.

Metastable atomic-ordered configurations for Al1/2Ga1/2N predicted by Monte-Carlo method based on first-principles calculations.

Metastability of Aln/12Ga1-n/12N (n= 2-10: integer) with the 1-2 monolayer (ML) in-plane configuration towards thec[0001] direction has been demonstrated recently. To theoretically explain the existence of these metastable structures, relatively large calculation cells are needed. However, previous calculations were limited to the use of small calculation cell sizes to estimate the local potential depth (Δσ) of ordered Al1/2Ga1/2N models. In this work, we were able to evaluate large calculation cells based on the interaction energies between proximate Al atoms (δEAl-Al) in AlGaN alloys. To do this,δEAl-Alvalues were estimated by first-principles calculations (FPCs) using a (5a1× 5a2× 5c) cell. Next, a survey of the possible ordered configurations using various large calculation cell models was performed using the estimatedδEAl-Alvalues and the Monte-Carlo method. Then, various Δσvalues were estimated by FPCs and compared with the configurations previously reported by other research groups. We found that the ordered configuration obtained from the (4a1× 2a2× 1c) calculation cell (C42) has the lowest Δσof -9.3 meV/cation and exhibited an in-plane configuration at thec(0001) plane having (-Al-Al-Ga-Ga-) and (-Al-Ga-) sequence arrangements observed along them11-00planes. Hence, we found consistencies between the morphology obtained from experiment and the shape of the primitive cell based on our numerical calculations.

Response-time improved hydrothermal-method-grown ZnO scintillator for soft x-ray free-electron laser timing-observation.

For pump and probe experiments in x-ray free-electron laser (XFEL) facilities, accurate timing synchronization between short-wavelength femtosecond pulses from XFELs and short optical pulses from other light sources is required. For this purpose, the response time of a hydrothermal-method-grown ZnO is improved by over one order of magnitude via intentional iron ion doping. The fluorescence rise- and decay-time constants are measured to be less than 10 and 100 ps, respectively. Owing to its intense fluorescence even for single pulse XFEL excitation, the timing jitter of the soft x-ray pulse and timing electronics are evaluated to be less than 70 ps.

Note: Light output enhanced fast response and low afterglow 6Li glass scintillator as potential down-scattered neutron diagnostics for inertial confinement fusion.

The characteristics of an APLF80+3Ce scintillator are presented. Its sufficiently fast decay profile, low afterglow, and an improved light output compared to the recently developed APLF80+3Pr, were experimentally demonstrated. This scintillator material holds promise for applications in neutron imaging diagnostics at the energy regions of 0.27 MeV of DD fusion down-scattered neutron peak at the world's largest inertial confinement fusion facilities such as the National Ignition Facility and the Laser Mégajoule.

Pr3+-doped fluoro-oxide lithium glass as scintillator for nuclear fusion diagnostics.

Experimental results are presented on the neutron scintillating properties of a custom-designed Pr3+ (praseodymium)-doped lithium (Li) glass. Luminescence was observed at 278 nm wavelength, originating from the 5d-4f transition. Time-resolved measurements yielded about 20 ns decay times for ultraviolet and x-ray excitation while much faster decay times of about 6 ns were observed for alpha particle and neutron excitation. Actual time-of-flight data in laser fusion experiments at the GEKKO XII facility of the Institute of Laser Engineering, Osaka University reveal that it can clearly discriminate fusion neutrons from the much stronger x-rays signals. This material can promise improved accuracy in future scattered neutron diagnostics.

Transmission of terahertz radiation using a microstructured polymer optical fiber.

A hollow-core microstructured polymer optical fiber was analyzed in the terahertz (THz) region. Spectral analysis of time domain data shows propagation of THz waves in both the hollow-core and the microstructured cladding with a time delay of approximately 20 ps. The frequency range and shift of the transmission bands between different sized waveguides suggested photonic bandgap or resonant guidance. Finite-difference time domain calculations agree relatively well to the experimental transmission results. Propagation losses were estimated to be as low as 0.9 dB/cm.

Terahertz time-domain spectroscopy of amino acids and polypeptides.

Frequency-dependent absorption coefficients and refractive indices of amino acids (glycine and l-alanine) and polypeptides (polyglycine and poly-l-alanine) in the wavenumber region from 7 to 55 cm(-1) were measured by terahertz time-domain spectroscopy. A vibrational band was observed at 45.5 cm(-1) for polyglycine, which was assigned as an interchain mode. The reduced absorption cross sections of the amino acids and polypeptides show power-law behavior. The exponents are different between the monomers and polymers, and those of the two polypeptides suggest that the time dependences of the total dipole moments are similar in the timescale of subpico- to picoseconds.

High-energy, all-solid-state, ultraviolet laser power-amplifier module design and its output-energy scaling principle.

We demonstrate that a coaxially pumped, large-aperture ultraviolet power-amplifier module with solid-state tunable laser medium Ce(3+):LiCaAlF6 has 98-mJ, 290-nm, and 3-ns output pulses with a sufficient extraction efficiency of 25%. The detailed information of design parameters, including the gain-coefficient dependence on pump condition, is successfully accumulated for further energy scaling for a terawatt-class ultraviolet chirped pulse amplification laser system or a high-pulse-energy laser system.