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1.
Proc Natl Acad Sci U S A ; 116(52): 26382-26388, 2019 Dec 26.
Artigo em Inglês | MEDLINE | ID: mdl-31818944

RESUMO

The glaciers near Puncak Jaya in Papua, Indonesia, the highest peak between the Himalayas and the Andes, are the last remaining tropical glaciers in the West Pacific Warm Pool (WPWP). Here, we report the recent, rapid retreat of the glaciers near Puncak Jaya by quantifying the loss of ice coverage and reduction of ice thickness over the last 8 y. Photographs and measurements of a 30-m accumulation stake anchored to bedrock on the summit of one of these glaciers document a rapid pace in the loss of ice cover and a ∼5.4-fold increase in the thinning rate, which was augmented by the strong 2015-2016 El Niño. At the current rate of ice loss, these glaciers will likely disappear within the next decade. To further understand the mechanisms driving the observed retreat of these glaciers, 2 ∼32-m-long ice cores to bedrock recovered in mid-2010 are used to reconstruct the tropical Pacific climate variability over approximately the past half-century on a quasi-interannual timescale. The ice core oxygen isotopic ratios show a significant positive linear trend since 1964 CE (0.018 ± 0.008‰ per year; P < 0.03) and also suggest that the glaciers' retreat is augmented by El Niño-Southern Oscillation processes, such as convection and warming of the atmosphere and sea surface. These Papua glaciers provide the only tropical records of ice core-derived climate variability for the WPWP.

2.
Environ Sci Technol ; 38(24): 6507-12, 2004 Dec 15.
Artigo em Inglês | MEDLINE | ID: mdl-15669306

RESUMO

Ice cores from glaciers situated near anthropogenic sources of air pollution provide important archives of the emissions of species with short atmospheric lifetimes. Here we present the history of atmospheric Pu fallout reconstructed from an ice core from the Belukha glacier in the Siberian Altai. Fourteen ice core samples covering the time period 1941-1986 were selected for Pu analysis, chemically processed, and measured using accelerator mass spectrometry. The Pu concentration peaks in 1963, coinciding with the maximum of the nuclear weapons tests and in concordance with the 3H activity concentration peak. The shapes of the 239Pu and 3H profiles reflect two main periods of atmospheric nuclear test activity: premoratorium testing before 1958 and postmoratorium testing in 1961 and 1962. Premoratorium tests contribute about 45% of the integrated Pu inventory. The average 240Pu/239Pu isotopic ratio is 0.18 +/- 0.05, indicating that a large majority of the Pu in the Belukha glacier originates from global stratospheric fallout rather than from direct tropospheric input.


Assuntos
Poluentes Radioativos do Ar/análise , Plutônio/análise , Cinza Radioativa/análise , Monitoramento Ambiental , História do Século XX , Humanos , Gelo , Guerra Nuclear/história , Sibéria
3.
Environ Sci Technol ; 38(15): 4085-90, 2004 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-15352445

RESUMO

Cr, Cu, Zn, Co, Ni, Mo, Rh, Pd, Ag, Cd, Sb, Pt, Au, and U have been determined in clean room conditions by inductively coupled plasma sector field mass spectrometry and other analytical techniques, in various sections of two dated snow/ice cores from the high-altitude (4450 m asl) glacier saddle Colle Gnifetti, Monte Rosa massif, located in the Swiss-Italian Alps. These cores cover a 350-year time period, from 1650 to 1994. The results show highly enhanced concentrations for most metals in snow/ice dated from the second half of the 20th century, compared with concentrations in ancient ice dated from the 17th and 18th centuries. The highest increase factors from the pre-1700 period to the post-1970 period are observed for Cd (36), Zn (19), Bi (15), Cu (11), and Ni (9), confirming the importance of atmospheric pollution by heavy metals in Europe. Metal concentrations observed in Colle Gnifetti snow around 1980 appear to be quantitatively related to metal emissions from Italy, Switzerland, Germany, France, Belgium, and Austria at that time, making it possible to reconstruct past changes in metal emission in these countries during the last centuries.


Assuntos
Poluentes Atmosféricos/análise , Poluentes Atmosféricos/história , Gelo , Metais Pesados/análise , Metais Pesados/história , Neve/química , Monitoramento Ambiental , Europa (Continente) , História do Século XVII , História do Século XVIII , História do Século XIX , História do Século XX , Itália , Suíça
4.
Environ Sci Technol ; 38(4): 957-64, 2004 Feb 15.
Artigo em Inglês | MEDLINE | ID: mdl-14998005

RESUMO

Lead concentrations and lead isotope ratios were analyzed in two firn/ice cores covering the period from 1650 to 1994, which were obtained from the 4450 m high glacier saddle Colle Gnifetti located in the Monte Rosa massif at the Swiss-Italian border. This study presents the first glaciochemical time series with annual resolution, spanning several centuries of lead concentrations and lead isotopic compositions in precipitation in Europe. Lead concentrations in firn dated from the 1970s are approximately 25 times higher than in ice dated from the 17th century, confirming the massive rise in lead pollution in Europe during the last few centuries. A decline of the lead concentration is then observed during the last two decades, i.e., from 1975 to 1994. The lead isotope ratio 206Pb/207Pb decreased from about 1.18 in the 17th and 18th centuries to about 1.12 in the 1970s. These variations are in good agreement with available information on variations in anthropogenic lead emissions from West European countries, especially from the use of lead additives in gasoline.


Assuntos
Poluentes Atmosféricos/análise , Poluentes Atmosféricos/história , Chumbo/análise , Chumbo/história , Altitude , Monitoramento Ambiental , Europa (Continente) , História do Século XVII , História do Século XVIII , História do Século XIX , História do Século XX , Humanos , Gelo , Indústrias , Isótopos , Neve , Emissões de Veículos
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