Time-Resolved Measurement of Interatomic Coulombic Decay Induced by Two-Photon Double Excitation of Ne_{2}.

The hitherto unexplored two-photon doubly excited states [Ne^{*}(2p^{-1}3s)]_{2} were experimentally identified using the seeded, fully coherent, intense extreme ultraviolet free-electron laser FERMI. These states undergo ultrafast interatomic Coulombic decay (ICD), which predominantly produces singly ionized dimers. In order to obtain the rate of ICD, the resulting yield of Ne_{2}^{+} ions was recorded as a function of delay between the extreme ultraviolet pump and UV probe laser pulses. The extracted lifetimes of the long-lived doubly excited states, 390(-130/+450) fs, and of the short-lived ones, less than 150 fs, are in good agreement with ab initio quantum mechanical calculations.

Slow Interatomic Coulombic Decay of Multiply Excited Neon Clusters.

Ne clusters (∼5000 atoms) were resonantly excited (2p→3s) by intense free electron laser (FEL) radiation at FERMI. Such multiply excited clusters can decay nonradiatively via energy exchange between at least two neighboring excited atoms. Benefiting from the precise tunability and narrow bandwidth of seeded FEL radiation, specific sites of the Ne clusters were probed. We found that the relaxation of cluster surface atoms proceeds via a sequence of interatomic or intermolecular Coulombic decay (ICD) processes while ICD of bulk atoms is additionally affected by the surrounding excited medium via inelastic electron scattering. For both cases, cluster excitations relax to atomic states prior to ICD, showing that this kind of ICD is rather slow (picosecond range). Controlling the average number of excitations per cluster via the FEL intensity allows a coarse tuning of the ICD rate.

The FERMI free-electron lasers.

FERMI is a seeded free-electron laser (FEL) facility located at the Elettra laboratory in Trieste, Italy, and is now in user operation with its first FEL line, FEL-1, covering the wavelength range between 100 and 20 nm. The second FEL line, FEL-2, a high-gain harmonic generation double-stage cascade covering the wavelength range 20-4 nm, has also completed commissioning and the first user call has been recently opened. An overview of the typical operating modes of the facility is presented.

Probabilistic aspects of magnetization relaxation in single-domain nanomagnets.

A single-domain nanomagnet is a basic example of a system where relaxation from high to low energy is probabilistic in nature even when thermal fluctuations are neglected. The reason is the presence of multiple stable states combined with extreme sensitivity to initial conditions. It is demonstrated that for this system the probability of relaxing from high energies to one of the stable magnetization orientations can be tuned to any desired value between 0 and 1 by applying a small transverse magnetic field of appropriate amplitude. In particular, exact analytical predictions are derived for the conditions under which the probability of reaching one of the stable states becomes exactly 0 or 1. Under these conditions, magnetization relaxation is totally insensitive to initial conditions, and the final state can be predicted with certainty, a feature that could be exploited to devise novel magnetization switching strategies or novel methods for the measurement of the magnetization damping constant.

Large Hysteresis effect in Synchronization of Nanocontact Vortex Oscillators by Microwave Fields.

Current-induced vortex oscillations in an extended thin-film with point-contact geometry are considered. The synchronization of these oscillations with a microwave external magnetic field is investigated by a reduced order model that takes into account the dynamical effects associated with the significant deformation of the vortex structure produced by the current, which cannot be taken care of by using the standard rigid vortex theory. The complete phase diagram of the vortex oscillation dynamics is derived and it is shown that strong hysteretic behavior occurs in the synchronization with the external field. The complex nonlinear nature of the synchronization manifests itself also through the appearance of asymmetry in the locking frequency bands for moderate microwave field amplitudes. Predictions from the reduced order model are confirmed by full micromagnetic simulations.

Two-colour pump-probe experiments with a twin-pulse-seed extreme ultraviolet free-electron laser.

Exploring the dynamics of matter driven to extreme non-equilibrium states by an intense ultrashort X-ray pulse is becoming reality, thanks to the advent of free-electron laser technology that allows development of different schemes for probing the response at variable time delay with a second pulse. Here we report the generation of two-colour extreme ultraviolet pulses of controlled wavelengths, intensity and timing by seeding of high-gain harmonic generation free-electron laser with multiple independent laser pulses. The potential of this new scheme is demonstrated by the time evolution of a titanium-grating diffraction pattern, tuning the two coherent pulses to the titanium M-resonance and varying their intensities. This reveals that an intense pulse induces abrupt pattern changes on a time scale shorter than hydrodynamic expansion and ablation. This result exemplifies the essential capabilities of the jitter-free multiple-colour free-electron laser pulse sequences to study evolving states of matter with element sensitivity.

Magnetization switching and microwave oscillations in nanomagnets driven by spin-polarized currents.

A novel theoretical approach to magnetization dynamics driven by spin-polarized currents is presented. Complete stability diagrams are obtained for the case where spin torques and external magnetic fields are simultaneously present. Quantitative predictions are made for the critical currents and fields inducing magnetization switching, for the amplitude and frequency of magnetization self-oscillations, and for the conditions leading to hysteretic transitions between self-oscillations and stationary states.

Nonlinear magnetization dynamics under circularly polarized field.

Exact analytical results are presented for the nonlinear large motion of the magnetization vector in a body with uniaxial symmetry subject to a circularly polarized field. The absence of chaos, the existence of pure time-harmonic magnetization modes with no generation of higher-order harmonics, and the existence of quasiperiodic magnetization modes with spontaneous breaking of the rotational symmetry are proven. Application to ferromagnetic resonance and connection with the Stoner-Wohlfarth model are discussed.

Spin-wave instabilities in large-scale nonlinear magnetization dynamics.

The stability of large magnetization motions in systems with uniaxial symmetry subject to a circularly polarized radio-frequency field is analytically studied. Instability conditions valid for arbitrary values of the amplitude and frequency of the driving field are derived. In the limit of small motions, these conditions yield Suhl's theory of spin-wave instabilities for the case of ferromagnetic resonance. It is shown that the input powers capable of inducing spin-wave instabilities are bounded from both below and above, so that large enough motions are always stable. In addition, it is demonstrated that stability of uniform motions depends on their preparation history.