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1.
Environ Geochem Health ; 36(5): 935-51, 2014 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-24760620

RESUMO

This work presents a modeling approach to simulate spatial distribution of metal contamination in aerosols with evaluation of health hazard. This approach offers the advantage to be non-intrusive, less expensive than sampling and laboratory analyses. It was applied to assess the impact of metal-bearing dust from mining wastes on air quality for a nearby community and agricultural lands in Jebel Ressas (Tunisia) locality. Dust emission rates were calculated using existing parameterization adapted to the contamination source composed of mining wastes. Metal concentrations were predicted using a Gaussian model (fugitive dust model) with, as input: emission rates, dump physical parameters and meteorological data measured in situ for 30 days in summertime. Metal concentration maps were built from calculated PM10 particle concentrations. They evidence the areas where Pb and Cd concentrations exceeded WHO guidelines (0.5 and 0.005 µg/m(3), respectively). Maximum concentrations of Pb and Cd in PM10 are, respectively, of 5.74 and 0.0768 µg/m(3) for measured wind speed values up to 22 m/s. Preferential areas of contamination were determined in agricultural lands to the NW from the source dump where Pb and Cd exceeded guidelines up to a distance of 1,200 m. The secondary spreading directions were SW and E, toward the village. Health hazard prospecting shown that a major part of the village was exposed to contaminated dust and that daily hazard quotient (HQ) values reached locally 118 and 158, respectively, for Pb and Cd during the study period. However, HQ variations in the village are high, both temporally and geographically.


Assuntos
Poluentes Atmosféricos/análise , Poeira/análise , Metais/análise , Mineração , Modelos Químicos , Vento , Cádmio/análise , Monitoramento Ambiental , Avaliação do Impacto na Saúde , Humanos , Chumbo/análise , Distribuição Normal , Tunísia
2.
Sci Total Environ ; 695: 133880, 2019 Dec 10.
Artigo em Inglês | MEDLINE | ID: mdl-31425992

RESUMO

The long-term variations of ozone are the combined results of climate change and air quality management. As Guangzhou is under the influence of both subtropical monsoon climate and rapid economic development, the ozone trend in recent years is uncertain. This paper presents the trend analysis of maximum daily average 8 h (MDA8) ozone and daily meteorological observations in Guangzhou from 2008 to 2018, using the Kolmogorov-Zurbenko (KZ) filter method. The observations were conducted at two sites in suburban Guangzhou, thus the datasets were processed in two periods. The first period (P1) is from 2008 to 2013, and the second period (P2) is from 2014 to 2018. Results show that the KZ filter method separates the short-term, seasonal, and long-term components efficiently, leaving a covariance term of 7.3% (5.4%) for P1 (P2). Through linear regression of long-term components, the trends were inferred as -0.06 ±â€¯0.04 ppb year-1 (R2 = 0.00, p < 0.05) for P1, and 0.51 ±â€¯0.08 ppb year-1 (R2 = 0.11, p < 0.05) for P2. It is found that the solar radiation has the strongest impact on ozone. With inclusion of temperature, relative humidity, and wind speed, these four meteorological factors held 71% (76%) variability in baseline ozone (sum of seasonal and long-term ozone) for P1 (P2). After applying the KZ filter method, the results reveal that the variance contribution of emission to long-term ozone variation is larger than that of meteorology in P1, while smaller in P2. Furthermore, 59% of the emission-induced ozone change in P2 could be explained by nitrogen dioxide variation, and their inverse correlation suggests that Guangzhou is mainly under volatile organic compounds-limited regime, despite continuous nitrogen oxides reduction.

4.
Environ Health Perspect ; 125(3): 385-391, 2017 03.
Artigo em Inglês | MEDLINE | ID: mdl-27557093

RESUMO

BACKGROUND: Globally, pollen allergy is a major public health problem, but a fundamental unknown is the likely impact of climate change. To our knowledge, this is the first study to quantify the consequences of climate change upon pollen allergy in humans. OBJECTIVES: We produced quantitative estimates of the potential impact of climate change upon pollen allergy in humans, focusing upon common ragweed (Ambrosia artemisiifolia) in Europe. METHODS: A process-based model estimated the change in ragweed's range under climate change. A second model simulated current and future ragweed pollen levels. These findings were translated into health burdens using a dose-response curve generated from a systematic review and from current and future population data. Models considered two different suites of regional climate/pollen models, two greenhouse gas emissions scenarios [Representative Concentration Pathways (RCPs) 4.5 and 8.5], and three different plant invasion scenarios. RESULTS: Our primary estimates indicated that sensitization to ragweed will more than double in Europe, from 33 to 77 million people, by 2041-2060. According to our projections, sensitization will increase in countries with an existing ragweed problem (e.g., Hungary, the Balkans), but the greatest proportional increases will occur where sensitization is uncommon (e.g., Germany, Poland, France). Higher pollen concentrations and a longer pollen season may also increase the severity of symptoms. Our model projections were driven predominantly by changes in climate (66%) but were also influenced by current trends in the spread of this invasive plant species. Assumptions about the rate at which ragweed spreads throughout Europe had a large influence upon the results. CONCLUSIONS: Our quantitative estimates indicate that ragweed pollen allergy will become a common health problem across Europe, expanding into areas where it is currently uncommon. Control of ragweed spread may be an important adaptation strategy in response to climate change. Citation: Lake IR, Jones NR, Agnew M, Goodess CM, Giorgi F, Hamaoui-Laguel L, Semenov MA, Solomon F, Storkey J, Vautard R, Epstein MM. 2017. Climate change and future pollen allergy in Europe. Environ Health Perspect 125:385-391; http://dx.doi.org/10.1289/EHP173.


Assuntos
Alérgenos/análise , Mudança Climática/estatística & dados numéricos , Exposição Ambiental/estatística & dados numéricos , Pólen , Rinite Alérgica Sazonal/epidemiologia , Europa (Continente)/epidemiologia , Hipersensibilidade
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