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Yield-stress transition in suspensions of deformable droplets.
Negro, Giuseppe; Carenza, Livio Nicola; Gonnella, Giuseppe; Mackay, Fraser; Morozov, Alexander; Marenduzzo, Davide.
Afiliação
  • Negro G; Dipartimento di Fisica, Universitá degli Studi di Bari and INFN, Sezione di Bari, via Amendola 173, Bari I-70126, Italy.
  • Carenza LN; School of Physics and Astronomy (SUPA), University of Edinburgh, Peter Guthrie Tait Road, Edinburgh EH9 3FD, UK.
  • Gonnella G; Instituut-Lorentz, Universiteit Leiden, P.O. Box 9506, 2300 RA Leiden, Netherlands.
  • Mackay F; Dipartimento di Fisica, Universitá degli Studi di Bari and INFN, Sezione di Bari, via Amendola 173, Bari I-70126, Italy.
  • Morozov A; School of Physics and Astronomy (SUPA), University of Edinburgh, Peter Guthrie Tait Road, Edinburgh EH9 3FD, UK.
  • Marenduzzo D; School of Physics and Astronomy (SUPA), University of Edinburgh, Peter Guthrie Tait Road, Edinburgh EH9 3FD, UK.
Sci Adv ; 9(22): eadf8106, 2023 Jun 02.
Article em En | MEDLINE | ID: mdl-37256946
Yield-stress materials, which require a sufficiently large forcing to flow, are currently ill-understood theoretically. To gain insight into their yielding transition, we study numerically the rheology of a suspension of deformable droplets in 2D. We show that the suspension displays yield-stress behavior, with droplets remaining motionless below a critical body-force. In this phase, droplets jam to form an amorphous structure, whereas they order in the flowing phase. Yielding is linked to a percolation transition in the contacts of droplet-droplet overlaps and requires strict conservation of the droplet area to exist. Close to the transition, we find strong oscillations in the droplet motion that resemble those found experimentally in confined colloidal glasses. We show that even when droplets are static, the underlying solvent moves by permeation so that the viscosity of the composite system is never truly infinite, and its value ceases to be a bulk material property of the system.

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2023 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2023 Tipo de documento: Article