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A Universal Approach for Sustainable Urea Synthesis via Intermediate Assembly at the Electrode/Electrolyte Interface.
Tu, Xiaojin; Zhu, Xiaorong; Bo, Shuowen; Zhang, Xiaoran; Miao, Ruping; Wen, Guobin; Chen, Chen; Li, Jing; Zhou, Yangyang; Liu, Qinghua; Chen, Dawei; Shao, Huaiyu; Yan, Dafeng; Li, Yafei; Jia, Jianfeng; Wang, Shuangyin.
Afiliação
  • Tu X; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Zhu X; School of Chemistry and Chemical Engineering, Nantong University, Nantong, Jiangsu, P. R. China.
  • Bo S; National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui, P. R. China.
  • Zhang X; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Miao R; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Wen G; College of Material Science and Engineering, Qingdao University of Science and Technology, Qingdao, Shandong, P. R. China.
  • Chen C; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Li J; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Zhou Y; Guangdong-Hong Kong-Macau Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau SAR, 999078, P. R. China.
  • Liu Q; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Chen D; National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui, P. R. China.
  • Shao H; State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, Hunan, China.
  • Yan D; College of Material Science and Engineering, Qingdao University of Science and Technology, Qingdao, Shandong, P. R. China.
  • Li Y; Guangdong-Hong Kong-Macau Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau SAR, 999078, P. R. China.
  • Jia J; College of Chemistry and Chemical Engineering, Hubei University, Wuhan, Hubei, P. R. China.
  • Wang S; College of Chemistry and Materials Science, Nanjing Normal University, Nanjing, Jiangsu, P. R. China.
Angew Chem Int Ed Engl ; 63(3): e202317087, 2024 Jan 15.
Article em En | MEDLINE | ID: mdl-38055225
Electrocatalytic C-N coupling process is indeed a sustainable alternative for direct urea synthesis and co-upgrading of carbon dioxide and nitrate wastes. However, the main challenge lies in the unactivated C-N coupling process. Here, we proposed a strategy of intermediate assembly with alkali metal cations to activate C-N coupling at the electrode/electrolyte interface. Urea synthesis activity follows the trend of Li+
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Ano de publicação: 2024 Tipo de documento: Article