Spin-Selective Angular Dispersion Control in Dielectric Metasurfaces for Multichannel Meta-Holographic Displays.

Angle-dependent next-generation displays have potential applications in 3D stereoscopic and head-mounted displays, image combiners, and encryption for augmented reality (AR) and security. Metasurfaces enable such exceptional functionalities with groundbreaking achievements in efficient displays over the past decades. However, limitations in angular dispersion control make them unfit for numerous nanophotonic applications. Here, we propose a spin-selective angle-dependent all-dielectric metasurface with a unique design strategy to manifest distinct phase information at different incident angles of light. As a proof of concept, the phase masks of two images are encoded into the metasurface and projected at the desired focal plane under different angles of left circularly polarized (LCP) light. Specifically, the proposed multifunctional metasurface generates two distinct holographic images under LCP illumination at angles of +35 and -35°. The presented holographic displays may provide a feasible route toward multifunctional meta-devices for potential AR displays, encrypted imaging, and information storage applications.

Single-layered meta-reflectarray for polarization retention and spin-encrypted phase-encoding.

Broadband communication with high data rates is a dire need for state-of-the-art wireless technologies. For achieving efficient wireless communication (particularly in an indoor environment), the electromagnetic (EM) waves should maintain their state of polarization despite encountering multiple reflections. Metasurfaces provide a unique platform to design subwavelength-featured meta-reflectarrays which enable the desired retention of the polarization state of an EM wave upon reflection. We present a single-layered broadband meta-reflectarray, simultaneously breaking n-fold (n > 2) rotational and mirror symmetry, which exhibits an unprecedented control over the phase, amplitude, and polarization of a reflected EM wave. This unique control enables the retention of polarization state and recording of spin-encrypted information for the reflected EM waves. Such novel multifunctional meta-reflectarray can be crucial to building an indoor setup for high data rate wireless communications. Meanwhile, the meta-array's ability to encode phase information provides an extra degree of freedom to structure and control (via incident spin) the reflected EM beam in the desired way. For the proof of concept, we have experimentally demonstrated a spin-encrypted holographic display which reconstructs the recorded holographic image at an image plane for the left circularly polarized (LCP) illumination and exhibits circular dichroism for the right circularly polarized (RCP) incident waves. The proposed meta-array can find applications in 5G indoor wireless communication, chiral sensing, spin-selective imaging, holography, and encryption.

Metasurface for Engineering Superimposed Ince-Gaussian Beams.

Ince-Gaussian beams (IGBs) are the third complete family of exact and orthogonal solutions of the paraxial wave equation and have been applied in many fields ranging from particle trapping to quantum optics. IGBs play a very important role in optics as they represent the exact and continuous transition modes connecting Laguerre-Gaussian and Hermite-Gaussian beams. The method currently in use suffers from the high cost, complexity, and large volume of the optical system. The superposition of IGBs can generate complicated structured beams with multiple phase and polarization singularities. A metasurface approach is proposed to realizing various superpositions of IGBs without relying on a complicated optical setup. By superimposing IGBs with even and odd modes, multiple phase, and polarization singularities are observed in the resultant beams. The phase and polarization singularities are modulated by setting the initial phase in the design and controlling the incident linear polarization. The compactness of the developed metasurface devices and the unique properties of the generated beams have the potential to impact many practical applications such as particle manipulation, orbital angular momentum spectrum manipulation, and optical communications.

Multifaceted control of focal points along an arbitrary 3D curved trajectory.

Metalenses can integrate the functionalities of multiple optical components thanks to the unprecedented capability of optical metasurfaces in light control. With the rapid development of optical metasurfaces, metalenses continue to evolve. Polarization and color play a very important role in understanding optics and serve as valuable tools for gaining insights into our world. Benefiting from the design flexibility of metasurfaces, we propose and experimentally demonstrate a super metalens that can realize multifaceted control of focal points along any 3D curved trajectory. The wavelengths and polarization states of all focal points are engineered in a desirable manner. The super metalens can simultaneously realize customized 3D positioning, polarization states, and wavelengths of focal points, which are experimentally demonstrated with incident wavelengths ranging from 501 to 700 nm. We further showcase the application of the developed super metalenses in 3D optical distance measurement. The compact nature of metasurfaces and unique properties of the proposed super metalenses hold promise to dramatically miniaturize and simplify the optical architecture for applications in optical metrology, imaging, detection, and security.

Multiple Multicolored 3D Polarization Knots Arranged along Light Propagation.

Polarization and color play essential roles in understanding optical phenomena and practical applications. Customized three-dimensional (3D) light fields, characterized by specific polarization and color distributions, have garnered growing interest owing to their unique optical attributes and expanded capacity for information encoding. To align with the ongoing trend of compactness and integration, it is desirable to develop lightweight optical elements that can simultaneously control polarization and color in 3D space. Although engineering longitudinally variable 3D optical structures with predesigned color and polarization information can add more degrees of freedom and additional capacity for information encoding, it has not been reported. We propose a metasurface approach to generating multiple 3D polarization knots along the light propagation direction. Each knot features two colors and an engineered 3D polarization profile. Different multicolored 3D polarization knots are obtained by controlling the observation region along the light propagation. Our approach simultaneously combines polarization, color, and longitudinal control in 3D environment, offering extra degrees of freedom for engineering complex vector beams. The unique properties of the developed metadevices, together with the design flexibility and compactness of metasurface, pave the way for polarization systems with small volumes applicable to some areas such as complex structured beams and encryption.

Dynamic control of hybrid grafted perfect vector vortex beams.

Perfect vector vortex beams (PVVBs) have attracted considerable interest due to their peculiar optical features. PVVBs are typically generated through the superposition of perfect vortex beams, which suffer from the limited number of topological charges (TCs). Furthermore, dynamic control of PVVBs is desirable and has not been reported. We propose and experimentally demonstrate hybrid grafted perfect vector vortex beams (GPVVBs) and their dynamic control. Hybrid GPVVBs are generated through the superposition of grafted perfect vortex beams with a multifunctional metasurface. The generated hybrid GPVVBs possess spatially variant rates of polarization change due to the involvement of more TCs. Each hybrid GPVVB includes different GPVVBs in the same beam, adding more design flexibility. Moreover, these beams are dynamically controlled with a rotating half waveplate. The generated dynamic GPVVBs may find applications in the fields where dynamic control is in high demand, including optical encryption, dense data communication, and multiple particle manipulation.

Metasurface-Enabled 3-in-1 Microscopy.

Edge enhancement and polarization detection are critical to image transparent or low-contrast samples. However, currently available systems are limited to performing only a single functionality. To meet the requirement of system integration, there is a pressing need for a microscope with multiple functionalities. Here, we propose and develop a microscope with three different functionalities based on spatial multiplexing and polarization splitting. A novel geometric metasurface (MS) is used to realize a spiral phase profile and two phase gradient profiles along two vertical directions, which can perform such an extremely challenging optical task. This is the first demonstration of a 3-in-1 microscope that can simultaneously obtain five images with different optical properties in an imaging plane for the same sample. Imaging experiments with different samples verify its capability to simultaneously perform edge imaging, polarimetric imaging, and conventional microscope imaging. Benefiting from the compactness and multifunctionality of the optical MS device, the integration does not increase the volume of the microscope. This approach can enable users to visualize the multiple facets of samples in real-time.

Design Strategies and Applications of Dimensional Optical Field Manipulation Based on Metasurfaces.

Recent rapid progress in metasurfaces is underpinned by the physics of local and nonlocal resonances and the modes coupling among them, leading to tremendous applications such as optical switching, information transmission, and sensing. In this review paper, an overview of the recent advances in a broad range of dimensional optical field manipulation based on metasurfaces categorized into different classes based on design strategies is provided. This review starts from the near-field optical resonances of artificial nanostructures and discusses the far-field optical wave manipulation based on fundamental mechanisms such as mode generation and mode coupling. The recent advances in optical field manipulation based on metasurfaces in different optical dimensions such as phase and polarization are summarized, and newly-developed dimensions such as the orbital angular momentum and the coherence dimensions resulting from phase modulation are discussed. Then, the recent achievements of multiplexing and multifunctional metasurfaces empowered by multidimensional optical field manipulation for optical information transmission and integrated applications are reviewed. Finally, the paper concludes with a few perspectives on emerging trends, possible directions, and existing challenges in this fast-developing field.

Longitudinally variable 3D optical polarization structures.

Generation and manipulation of three-dimensional (3D) optical polarization structures have received considerable interest because of their distinctive optical features and potential applications. However, the realization of multiple 3D polarization structures in a queue along the light propagation direction has not yet been reported. We propose and experimentally demonstrate a metalens to create longitudinally variable 3D polarization knots. A single metalens can simultaneously generate three distinct 3D polarization knots, which are indirectly validated with a rotating polarizer. The 3D polarization profiles are dynamically modulated by manipulating the linear polarization direction of the incident light. We further showcase the 3D image steganography with the generated 3D polarization structures. The ultrathin nature of metasurfaces and unique properties of the developed metalenses hold promise for lightweight polarization systems applicable to areas such as 3D image steganography and virtual reality.

Compact multi-foci metalens spectrometer.

A lightweight and portable spectrometer is desirable for miniaturization and integration. The unprecedented capability of optical metasurfaces has shown much promise to perform such a task. We propose and experimentally demonstrate a compact high-resolution spectrometer with a multi-foci metalens. The novel metalens is designed based on wavelength and phase multiplexing, which can accurately map the wavelength information into its focal points located on the same plane. The measured wavelengths in the light spectra agree with simulation results upon the illumination of various incident light spectra. The uniqueness of this technique lies in the novel metalens that can simultaneously realize wavelength splitting and light focusing. The compactness and ultrathin nature of the metalens spectrometer render this technology have potential applications in on-chip integrated photonics where spectral analysis and information processing can be performed in a compact platform.

Multichannel Superposition of Grafted Perfect Vortex Beams.

Inspired by plant grafting, grafted vortex beams can be formed through grafting two or more helical phase profiles of optical vortex beams. Recently, grafted perfect vortex beams (GPVBs) have attracted much attention due to their unique optical properties and potential applications. However, the current method to generate and manipulate GPVBs requires a complex and bulky optical system, hindering further investigation and limiting its practical applications. Here, a compact metasurface approach for generating and manipulating GPVBs in multiple channels is proposed and demonstrated, which eliminates the need for such a complex optical setup. A single metasurface is utilized to realize various superpositions of GPVBs with different combinations of topological charges in four channels, leading to asymmetric singularity distributions. The positions of singularities in the superimposed beam can be further modulated by introducing an initial phase difference in the metasurface design. The work demonstrates a compact metasurface platform that performs a sophisticated optical task that is very challenging with conventional optics, opening opportunities for the investigation and applications of GPVBs in a wide range of emerging application areas, such as singular optics and quantum science.

Single-Step Fabricable Flexible Metadisplays for Sensitive Chemical/Biomedical Packaging Security and Beyond.

Secure packaging and transportation of light-sensitive chemical and biomedical test tubes are crucial for environmental protection and public health. Benefiting from the compact form factor and high efficiency of optical metasurfaces, we propose a broad-band polarization-insensitive flexible metasurface for the security of sensitive packages in the transport industry. We employ both the propagation and the geometric phase of novel TiO2 resin-based anisotropic nanoresonators to demonstrate a flexible and broad-band polarization-insensitive metasurface in the visible domain. The ultraviolet nanoimprint lithographic technique (UV-NIL) is used to fabricate high-index TiO2 nanoparticle-embedded-resin (nano-PER) structures that are patterned on a flexible substrate. This novel approach provides swift single-step fabrication without secondary fabrication steps such as deposition and etching. Moreover, replicating and transforming patterns over flexible substrates make the proposed technique highly suitable for large-throughput commercial manufacturing. As the proposed metahologram manifests high transmission efficiency in the visible domain, such flexible metaholographic platforms could find several exciting applications in bendable/curved displays, wearable devices, and holographic labeling for interactive displays.

Holographic metasurface gas sensors for instantaneous visual alarms.

The rapid detection of biological and chemical substances in real time is particularly important for public health and environmental monitoring and in the military sector. If the process of substance detection to visual reporting can be implemented into a single miniaturized sensor, there could be a profound impact on practical applications. Here, we propose a compact sensor platform that integrates liquid crystals (LCs) and holographic metasurfaces to autonomously sense the existence of a volatile gas and provide an immediate visual holographic alarm. By combining the advantage of the rapid responses to gases realized by LCs with the compactness of holographic metasurfaces, we develop ultracompact gas sensors without additional complex instruments or machinery to report the visual information of gas detection. To prove the applicability of the compact sensors, we demonstrate a metasurface-integrated gas sensor on safety goggles via a one-step nanocasting process that is attachable to flat, curved, and flexible surfaces.

Optical spin-symmetry breaking for high-efficiency directional helicity-multiplexed metaholograms.

Helicity-multiplexed metasurfaces based on symmetric spin-orbit interactions (SOIs) have practical limits because they cannot provide central-symmetric holographic imaging. Asymmetric SOIs can effectively address such limitations, with several exciting applications in various fields ranging from asymmetric data inscription in communications to dual side displays in smart mobile devices. Low-loss dielectric materials provide an excellent platform for realizing such exotic phenomena efficiently. In this paper, we demonstrate an asymmetric SOI-dependent transmission-type metasurface in the visible domain using hydrogenated amorphous silicon (a-Si:H) nanoresonators. The proposed design approach is equipped with an additional degree of freedom in designing bi-directional helicity-multiplexed metasurfaces by breaking the conventional limit imposed by the symmetric SOI in half employment of metasurfaces for one circular handedness. Two on-axis, distinct wavefronts are produced with high transmission efficiencies, demonstrating the concept of asymmetric wavefront generation in two antiparallel directions. Additionally, the CMOS compatibility of a-Si:H makes it a cost-effective alternative to gallium nitride (GaN) and titanium dioxide (TiO2) for visible light. The cost-effective fabrication and simplicity of the proposed design technique provide an excellent candidate for high-efficiency, multifunctional, and chip-integrated demonstration of various phenomena.

Stimuli-Responsive Dynamic Metaholographic Displays with Designer Liquid Crystal Modulators.

Flat optics, realized by the artificially created 2D material platform called optical metasurfaces, is currently undergoing a science-to-technology transition. However, "real-time" active operations of such flat optical devices remain yet unresolved. Here, liquid crystals (LCs)-integrated metaholograms for ultracompact dynamic holographic displays are proposed. The anisotropic nature of the LCs allows facile and repeatable manipulation of the polarization of light. Specifically designed ("designer") LCs and efficient helicity-encoded metaholograms are combined to realize stimuli-responsive dynamic displays. The designer LC modulators are used as switches that enable a variety of external stimuli (e.g., electric field, heat, surface pressure) to operate holographic images in real-time. Such a dynamic metaholographic platform will provide a path to external stimuli-driven "smart" sensing and display applications such as hologram labels for temperature/pressure/touch monitoring and interactive holographic displays with haptic motion recognition.

Planar Achiral Metasurfaces-Induced Anomalous Chiroptical Effect of Optical Spin Isolation.

Planar chiral structures respond differently for oppositely handed incident light, and thus can produce extraordinary chiroptical effects such as circular conversion dichroism (CCD) and asymmetric transmission (AT). Such chiroptical effects are powerful tools to realize the fundamental principle of optical spin isolation, which leads to a plethora of applications such as optical conversion diodes, chiral imaging, and sensing. Here, we demonstrate the chiroptical effects of simultaneous CCD and AT through meticulously designed single-layered achiral nanofins. Our metamolecule consists of four achiral hydrogenated amorphous silicon (a-Si:H) nanofins that are carefully oriented and optimized to exhibit considerable CCD and AT. The device demonstrates a circular conversion dichroism of 55% and an asymmetric transmission of 58% at a wavelength of 633 nm. Right-hand circularly polarized light (RHCP) is completely absorbed, while left-hand circularly polarized light (LHCP) is transmitted with a polarization conversion, making it a perfect circular polarization wave isolator with negligible backscattering (due to low reflectance). This unique design and its underlying working mechanism are described comprehensively with three different techniques. These methods validate the proposed design and its methodology. For practical applications such as imaging, the proposed design realizes the Pancharatnam-Berry (PB) phase, achieving a 0-2π phase coverage for transmitted circular polarization. For the proof of concept, a metahologram is designed and demonstrated by employing the achieved full-phase control. The measured response of the fabricated metadevice not only validates the CCD and AT but also exhibits a simulated polarization conversion efficiency of up to 71% and measured efficiency up to 52%, comparable to state-of-the-art metahologram demonstrations.