RESUMEN
The scattering of electromagnetic waves by resonant systems is determined by the excitation of the quasinormal modes (QNMs), i.e. the eigenmodes, of the system. This Review addresses three fundamental concepts in relation to the representation of the scattered field as a superposition of the excited QNMs: normalization, orthogonality, and completeness. Orthogonality and normalization enable a straightforward assessment of the QNM excitation strength for any incident wave. Completeness guarantees that the scattered field can be faithfully expanded into the complete QNM basis. These concepts are not trivial for non-conservative (non-Hermitian) systems and have driven many theoretical developments since initial studies in the 70's. Yet, they are not easy to grasp from the extensive and scattered literature, especially for newcomers in the field. After recalling fundamental results obtained in initial studies on the completeness of the QNM basis for simple resonant systems, we review recent achievements and the debate on the normalization, clarify under which circumstances the QNM basis is complete, and highlight the concept of QNM regularization with complex coordinate transforms.
RESUMEN
We develop an exact analytical approach to the optical response of a two-level system coupled to a microcavity for arbitrary excitation strengths. The response is determined in terms of the complex amplitudes of transitions between the rungs of the Jaynes-Cummings ladder, explicitly isolating nonlinearities of different orders. Increasing the pulse area of the excitation field, we demonstrate the formation of a quantum Mollow quadruplet (QMQ), quantizing the semiclassical Mollow triplet into a coherent superposition of a large number of transitions between rungs of the ladder, with inner and outer doublets of the QMQ formed by densely lying inner and outer quantum transitions between the split rungs. Remarkably, a closed-form analytic approximation for the QMQ of any order of nonlinearity is found in the high-field low-damping limit.
RESUMEN
Nanophotonic chiral sensing has recently attracted a lot of attention. The idea is to exploit the strong light-matter interaction in nanophotonic resonators to determine the concentration of chiral molecules at ultralow thresholds, which is highly attractive for numerous applications in life science and chemistry. However, a thorough understanding of the underlying interactions is still missing. The theoretical description relies on either simple approximations or on purely numerical approaches. We close this gap and present a general theory of chiral light-matter interactions in arbitrary resonators. Our theory describes the chiral interaction as a perturbation of the resonator modes, also known as resonant states or quasi-normal modes. We observe two dominant contributions: A chirality-induced resonance shift and changes in the modes' excitation and emission efficiencies. Our theory brings deep insights for tailoring and enhancing chiral light-matter interactions. Furthermore, it allows us to predict spectra much more efficiently in comparison to conventional approaches. This is particularly true, as chiral interactions are inherently weak and therefore perturbation theory fits extremely well for this problem.