ROLE OF METEOROLOGY AND LITHOLOGY IN THE TEMPORAL VARIATION OF THE OUTDOOR RADON LEVEL.

The outdoor radon concentration was monitored together with the meteorological parameters at two contrasting complex topographies: sub-Alpine basin (SA) and sub-Mediterranean valley (SM) in winter (December 2017-February 2018) and summer (June-August 2018). The time series for each site and each season are evaluated in three different ways: (i) clear-sky and cloudy condition together, (ii) clear-sky conditions only (cloud cover <20%) and (iii) cloudy condition only (cloud cover >20%), and compared to the expected atmospheric boundary layer (ABL) 'mixing volume' caused by meteorological changes. The results have confirmed the sensitivity of diurnal and seasonal radon concentration to the expected ABL 'mixing volume' at the two selected sites. The relationship is more pronounced in calm clear-sky conditions. Cloudy conditions are associated with fast weather changes, when the ABL is well mixed and hourly mean radon concentrations do not follow the typical diurnal trend.

Exposure to radon in the Gadime Cave, Kosovo.

Air radon concentration was measured in summer and winter at 11 points along the tourist guided route in the Gadime Cave in Kosovo using alpha scintillation cells and etched track detectors. At two points in summer, values higher than 1700Bqm(-3) were observed; they otherwise were in the range 400-1000Bqm(-3). Values were lower in winter. The effective dose received by a person during a 90min visit is 3.7microSv in summer and 2.5microSv in winter. For a tourist guide the annual effective dose is less than 3.5mSv.

Exposure to radon in dwellings in the Sharri community, Kosovo.

Indoor air radon concentration was measured by exposing etched track detectors in the sleeping and living rooms of 18 houses in 6 villages of the Sharri community in Kosovo. Values ranged from 24 to 209 Bq m(-3), with only one exceeding 200 Bq m(-3), with a geometric mean and geometric standard deviation of 95.4 Bq m(-3) and 1.6, respectively. On the basis of the assumption that the spring radon concentrations obtained in this survey represent the yearly average, annual effective doses of residents were calculated; they range from 0.89 to 4.7 mSv y(-1), with the geometric mean and geometric standard deviation of 1.5 mSv y(-1) and 2.2, respectively. No mitigation measures are planned to be undertaken.

Radon in a thermal spring: identification of anomalies related to seismic activity.

Anomalies have been observed in the radon content of thermal spring water at the Italian-Slovenian border. To distinguish the anomalies caused by environmental parameters (air and water temperature, barometric and hydrostatic pressure, rainfall) from those ascribed solely to earthquakes with M(L) from 1.2 to 2.5 and epicentres, R(E), within 2R(D) (R(D)--Dobrovolsky's radius), two approaches have been used: (i) correlation between time gradients of radon concentration and hydrostatic pressure, and (ii) regression trees within machine learning programs. The regression trees approach has been improved by introducing additional environmental parameters and prolonging the measuring period.

High natural radiation exposure in radon spa areas: a detailed field investigation in Niska Banja (Balkan region).

The measurement campaigns have been done in the rural community of Niska Banja, a spa town located in southern Serbia, to evaluate population exposure to natural radioactivity. After a screening survey in 200 houses, annual radon and thoron concentrations were measured in 34 houses, and in 2004 a detailed investigation was carried out at six houses with elevated indoor radon concentrations. The paper presents the results of these detailed measurements. The complementary techniques were applied to determine radon and thoron concentrations in indoor air, in soil gas, radon exhalation from soil, soil permeability, and indoor and outdoor gamma doses. Soil and water samples were collected and analysed in the laboratory. Indoor radon and thoron concentrations were found to be more than 1kBqm(-3) and 200Bqm(-3), respectively. Extremely high concentrations of soil-gas radon (>2000kBqm(-3)) and radon exhalation rates (1.5mBqm(-2)s(-1)) were observed. These results will be utilised to set up the methodology for a more systematic investigation.

Long-term measurements of radon, thoron and their airborne progeny in 25 schools in Republic of Srpska.

This article reports results of the first investigations on indoor radon, thoron and their decay products concentration in 25 primary schools of Banja Luka, capital city of Republic Srpska. The measurements have been carried out in the period from May 2011 to April 2012 using 3 types of commercially available nuclear track detectors, named: long-term radon monitor (GAMMA 1)- for radon concentration measurements (C(Rn)); radon-thoron discriminative monitor (RADUET) for thoron concentration measurements (C(Tn)); while equilibrium equivalent radon concentration (EERC) and equilibrium equivalent thoron concentrations (EETC) measured by Direct Radon Progeny Sensors/Direct Thoron Progeny Sensors (DRPS/DTPS) were exposed in the period November 2011 to April 2012. In each school the detectors were deployed at 10 cm distance from the wall. The obtained geometric mean concentrations were C(Rn) = 99 Bq m(-3) and C(Tn) = 51 Bq m(-3) for radon and thoron gases respectively. Those for equilibrium equivalent radon concentration (EERC) and equilibrium equivalent thoron concentrations (EETC) were 11.2 Bq m(-3) and 0.4 Bq m(-3), respectively. The correlation analyses showed weak relation only between C(Rn) and C(Tn) as well as between C(Tn) and EETC. The influence of the school geographical locations and factors linked to buildings characteristic in relation to measured concentrations were tested. The geographical location and floor level significantly influence C(Rn) while C(Tn) depend only from building materials (ANOVA, p ≤ 0.05). The obtained geometric mean values of the equilibrium factors were 0.123 for radon and 0.008 for thoron.

Correlation between short-term and long-term radon measurements.

In selected kindergartens and schools, long-term average indoor air radon concentrations were measured by two-month exposure of etched track detectors. Short-term average concentrations were obtained from 7-10 day continuous radon recordings during the exposure of etched track detectors. Only in about 1/3 of cases both averages did agree within +/- 20%; otherwise they differ considerably. The assumption that short-term results can substitute for long-term data, which is sometimes made to correct radon exposure estimated on the basis of concentrations obtained by etched track detectors, should therefore be treated with caution.

Systematic indoor radon and gamma-ray measurements in Slovenian schools.

During the winter months of 1992/93 and 1993/94, instantaneous indoor radon concentrations and gamma dose rates were measured in 890 schools in Slovenia attended in total by about 280,000 pupils. Under "closed conditions," the room to be surveyed was closed for more than 12 h prior to sampling, the air was sampled into alpha scintillation cells with a volume of 700 cm3, and alpha activity was measured. An arithmetic mean of 168 Bq m(-3) and a geometric mean of 82 Bq m(-3) were obtained. In 67% of schools, indoor radon concentrations were below 100 Bq m(-3), and in 8.7% (77 schools with about 16,000 pupils) they exceeded 400 Bq m(-3), which is the proposed Slovene action level. In the majority of cases, radon concentrations were high due to the geological characteristics of the ground. Approximately 70% of schools with high radon levels were found in the Karst region. Gamma dose rates were measured using a portable scintillation counter. An arithmetic mean of 102 nGy h(-1) and a geometric mean of 95 nGy h(-1) were obtained. No extraordinarily high values were recorded.

Radon level reduction in two kindergartens in Slovenia.

Remedial actions were carried out in two kindergartens with average heating season radon concentrations of about 2,000 Bq m-3. The first kindergarten is built on sedimentary gravel and the second one on fly ash and cinder fill. In both cases, radon accumulated in a sub-floor channel (service tunnel). The channels were opened at both ends. Natural ventilation of the tunnels did not produce a sufficient reduction in radon concentration. A fan was mounted in one kindergarten to ventilate the channel for 20 min three times each day, thus reducing radon levels to an acceptable value.

Preliminary indoor radon investigations in Lublin region, Poland.

Indoor air radon concentrations in all kindergartens and play schools in Lublin, Poland, were determined in grab samples by using alpha scintillation cells. In addition, some public buildings and homes in Lublin and several places in Eastern Poland were surveyed for radon. For kindergartens and play schools, the geometric mean was 23 Bq m-3 with a standard deviation of 1.4 Bq m-3, while in public buildings and homes, these values were 26 and 1.6 Bq m-3, respectively.

Systematic indoor radon and gamma measurements in kindergartens and play schools in Slovenia.

Systematic measurements of indoor radon concentrations and gamma dose rates were carried out in the 730 kindergartens and play schools in Slovenia that, together, care for 65,600 children. The main method for indoor radon measurement was direct sampling in alpha scintillation cells, but in cases with an increased instantaneous radon concentration, the additional methods of track-etch detectors and alpha spectroscopy were applied. In 528 kindergartens and play schools (72%), radon concentrations were below 100 Bq m-3, with a geometric mean of 58 Bq m-3. In 16 kindergartens and play schools (2.2%), radon concentrations exceeded 800 Bq m-3. In all cases, the main reason for a high indoor radon concentration was the geological structure of the soil. Gamma dose rates were measured with a portable scintillation counter, but in the Ljubljana region thermoluminescence dosimeters were also exposed. The results ranged from 30 to 295 nGy h-1, with a geometric mean of 88 nGy h-1.

Search for radon sources in buildings--kindergartens.

In ten high radon level kindergartens, radon sources were sought by applying a combination of several radon measuring techniques: etched track detectors to obtain average indoor air radon concentration, continuous devices to record radon concentration and see its diurnal variation, and alpha scintillation cells to determine radon concentration in the air entering a room from cracks, holes and sinks in the floor and from under-floor channels. In three cases, a strong local radon source was identified while, in the others, the bad quality of the basic concrete slab was responsible for the high indoor radon concentration.

Application of decision trees to the analysis of soil radon data for earthquake prediction.

Different regression methods have been used to predict radon concentration in soil gas on the basis of environmental data, i.e. barometric pressure, soil temperature, air temperature and rainfall. Analyses of the radon data from three stations in the Krsko basin, Slovenia, have shown that model trees outperform other regression methods. A model has been built which predicts radon concentration with a correlation of 0.8, provided it is influenced only by the environmental parameters. In periods with seismic activity this correlation is much lower. This decrease in predictive accuracy appears 1-7 days before earthquakes with local magnitude 0.8-3.3.

Geochemical monitoring of thermal waters in Slovenia: relationships to seismic activity.

Thermally anomalous fluids released in seismic areas in Slovenia were the subjects of geochemical monitoring. Thermal waters were surveyed from the seismically active area of Posocje (Bled and Zatolmin; NW Slovenia) and from Rogaska Slatina in eastern Slovenia. Continuous monitoring of geochemical parameters (radon concentration, electrical conductivity, and water temperature) was performed with discrete gas sampling for their (3)He/(4)He ratio. The observed values were correlated with meteorological parameters (rainfall, barometric pressure and air temperature) and with seismic activity. Only a few earthquakes occurred in the vicinity of the measuring sites during the monitoring period. Nevertheless, changes in radon concentration, water temperature, electrical conductivity and helium isotopic ratio were detected at the three thermal springs in the periods preceding the earthquakes. A close correlation was also observed of both water temperature and electrical conductivity with the Earth tide, making the observations in the selected sites a promising tool for addressing the widely debated question of earthquake prediction.

Soil radon monitoring in the Krsko Basin, Slovenia.

In order to support the safe operation of the Krsko Nuclear Power Plant (Westinghouse, 676 MWe PWR), the seismotectonic structure of the Krsko basin has been thoroughly investigated. As part of a wider study, a study on radon in soil gas was started in April 1999. Combined barasol detectors buried in six boreholes, two along the Orlica fault and four on either side of it, measure and record radon activity, temperature and pressure every 60 min. The results have been evaluated and the possibility of a correlation with seismic activity is discussed. Correlation between radon concentration and barometric pressure has been observed for all barasols. Preliminary results show that, at one location, the correlation coefficient between radon and barometric pressure changed sign before earthquakes.

Identification of sources of high radon levels in Slovenian schools.

The sources of radon were investigated in twenty selected schools with high room levels of radiation. A combination of radon measuring techniques was applied: etched track and electret detectors to obtain average indoor air radon concentration. devices to record radon concentration continuously and thus characterise its diurnal variation, and alpha scintillation cells to analyse air from potential sources of radon entry. In some cases, a single strong source was identified (e.g. sinks, sub-floor channels), while in others the poor quality of the basic concrete slab was responsible for high indoor radon concentrations. The combination of etched track and electret detectors and alpha scintillation cells was essential for locating these sources.

Radon exposure in Slovenian spas.

Radon and gamma dose rates were surveyed in five Slovenian spas, at Rogaska Slatina, Radenci, Moravci, Podcetrtek, and Catez. Due to effective ventilation systems, the indoor air radon concentration rarely exceeds 200 Bq x m(-3) and is usually lower. Uncer the present operationsal conditions and working regimes of the spas, there is no basis for concern about elevated exposure of personnel to radon.

Radon exposure in slovene kindergartens based on continuous radon measurements.

Contiunuous measurements of concentration of radon and radon decay products, and equilibrium factor were carried out in the indoor air of 13 kindergartens at the beginning of 2000. Average values of the parameters measured during working time only and during the whole period, were compared and applied to estimate effective doses to the personnel. Results of short-term continuous measurements were used to correct the exposure, based generally on the radon concentration.

Radon levels and doses in dwellings in two villages in Kosovo, affected by depleted uranium.

The radon ((222)Rn) activity concentration in 15 dwellings in the Planej village and 10 dwellings in the Gorozhup village has been measured with the aim to complement the national radon survey and to compare the results of two different measurement techniques. The radon concentration has been measured in winter and spring using alpha scintillation cells and in winter, spring and summer by exposing solid-state nuclear track detectors. Both methods gave similar results. Radon concentrations in both villages were similar, ranging from 82 to 432 Bq m(-3); the value of 400 Bq m(-3) was exceeded only in two dwellings. The resulting annual effective doses ranged from 1.78 to 6.40 mSv, with the average values of 3.28 mSv in the Planej village and 3.87 mSv in the Gorozhup village.

Geographical distribution of the annual mean radon concentrations in primary schools of Southern Serbia - application of geostatistical methods.

Between 2008 and 2011 a survey of radon ((222)Rn) was performed in schools of several districts of Southern Serbia. Some results have been published previously (Zunic et al., 2010; Carpentieri et al., 2011; Zunic et al., 2013). This article concentrates on the geographical distribution of the measured Rn concentrations. Applying geostatistical methods we generate "school radon maps" of expected concentrations and of estimated probabilities that a concentration threshold is exceeded. The resulting maps show a clearly structured spatial pattern which appears related to the geological background. In particular in areas with vulcanite and granitoid rocks, elevated radon (Rn) concentrations can be expected. The "school radon map" can therefore be considered as proxy to a map of the geogenic radon potential, and allows identification of radon-prone areas, i.e. areas in which higher Rn radon concentrations can be expected for natural reasons. It must be stressed that the "radon hazard", or potential risk, estimated this way, has to be distinguished from the actual radon risk, which is a function of exposure. This in turn may require (depending on the target variable which is supposed to measure risk) considering demographic and sociological reality, i.e. population density, distribution of building styles and living habits.