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1.
Proc Natl Acad Sci U S A ; 120(48): e2305541120, 2023 Nov 28.
Artículo en Inglés | MEDLINE | ID: mdl-37983495

RESUMEN

The interplay between chirality and topology nurtures many exotic electronic properties. For instance, topological chiral semimetals display multifold chiral fermions that manifest nontrivial topological charge and spin texture. They are an ideal playground for exploring chirality-driven exotic physical phenomena. In this work, we reveal a monopole-like orbital-momentum locking texture on the three-dimensional Fermi surfaces of topological chiral semimetals with B20 structures (e.g., RhSi and PdGa). This orbital texture enables a large orbital Hall effect (OHE) and a giant orbital magnetoelectric (OME) effect in the presence of current flow. Different enantiomers exhibit the same OHE which can be converted to the spin Hall effect by spin-orbit coupling in materials. In contrast, the OME effect is chirality-dependent and much larger than its spin counterpart. Our work reveals the crucial role of orbital texture for understanding OHE and OME effects in topological chiral semimetals and paves the path for applications in orbitronics, spintronics, and enantiomer recognition.

2.
J Synchrotron Radiat ; 31(Pt 5): 1058-1066, 2024 Sep 01.
Artículo en Inglés | MEDLINE | ID: mdl-39150680

RESUMEN

Advances in physics have been significantly driven by state-of-the-art technology, and in photonics and X-ray science this calls for the ability to manipulate the characteristics of optical beams. Orbital angular momentum (OAM) beams hold substantial promise in various domains such as ultra-high-capacity optical communication, rotating body detection, optical tweezers, laser processing, super-resolution imaging etc. Hence, the advancement of OAM beam-generation technology and the enhancement of its technical proficiency and characterization capabilities are of paramount importance. These endeavours will not only facilitate the use of OAM beams in the aforementioned sectors but also extend the scope of applications in diverse fields related to OAM beams. At the FERMI Free-Electron Laser (Trieste, Italy), OAM beams are generated either by tailoring the emission process on the undulator side or, in most cases, by coupling a spiral zone plate (SZP) in tandem with the refocusing Kirkpatrick-Baez active optic system (KAOS). To provide a robust and reproducible workflow to users, a Hartmann wavefront sensor (WFS) is used for both optics tuning and beam characterization. KAOS is capable of delivering both tightly focused and broad spots, with independent control over vertical and horizontal magnification. This study explores a novel non-conventional `near collimation' operational mode aimed at generating beams with OAM that employs the use of a lithographically manufactured SZP to achieve this goal. The article evaluates the mirror's performance through Hartmann wavefront sensing, offers a discussion of data analysis methodologies, and provides a quantitative analysis of these results with ptychographic reconstructions.

3.
Chirality ; 36(2): e23648, 2024 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-38384149

RESUMEN

Magnetic circular dichroism (MCD) spectroscopy is a powerful method for evaluating the electronic structure and magnetic and optical properties of molecules. In particular, MCD measurements have been performed on phthalocyanines and porphyrins with various central metal ions, axial ligands, and substituents to elucidate their properties. It is essential to develop a robust high-throughput technique to perform these measurements comprehensively and efficiently. However, MCD spectroscopy requires very high optical quality for each component of the instrument, and even slight cell distortions can impair the baseline flatness. Consequently, when versatility and data quality are important, an optical system designed for a microplate reader is not suitable for the MCD spectrometer. Therefore, in this study, we develop a new magnetic flow-through cell and combine it with an existing CD spectrometer and autosampler to construct a high-throughput system. The effectiveness and performance of this new system are then evaluated. In addition, based on the MCD and absorption spectra of various phthalocyanine complexes, the effects of substituents and solvents on their magnetic and optical properties and the causes of these effects are discussed. The results demonstrate that this system is effective for the evaluation of the physicochemical properties of various phthalocyanine complexes.

4.
Proc Natl Acad Sci U S A ; 118(2)2021 01 12.
Artículo en Inglés | MEDLINE | ID: mdl-33372145

RESUMEN

Spin angular momentum of light is vital to investigate enantiomers characterized by circular dichroism (CD), widely adopted in biology, chemistry, and material science. However, to discriminate chiral materials with multiscale features, CD spectroscopy normally requires wavelength-swept laser sources as well as wavelength-specific optical accessories. Here, we experimentally demonstrate an orbital-angular-momentum-assisted approach to yield chiroptical signals with monochromatic light. The gigantic vortical differential scattering (VDS) of ∼120% is achieved on intrinsically chiral microstructures fabricated by femtosecond laser. The VDS measurements can robustly generate chiroptical properties on microstructures with varying geometric features (e.g., diameters and helical pitches) and detect chiral molecules with high sensitivity. This VDS scheme lays a paradigm-shift pavement toward efficiently chiroptical discrimination of multiscale chiral structures with photonic orbital angular momentum. It simplifies and complements the conventional CD spectroscopy, opening possibilities for measuring weak optical chirality, especially on mesoscale chiral architectures and macromolecules.

5.
Sensors (Basel) ; 24(3)2024 Feb 01.
Artículo en Inglés | MEDLINE | ID: mdl-38339661

RESUMEN

Vortex beams carrying orbital angular momentum (OAM) provide a new degree of freedom for light waves in addition to the traditional degrees of freedom, such as intensity, phase, frequency, time, and polarization. Due to the theoretically unlimited orthogonal states, the physical dimension of OAM is capable of addressing the problem of low information capacity. With the advancement of the OAM optical communication technology, OAM router devices (OAM-RDs) have played a key role in significantly improving the flexibility and practicability of communication systems. In this review, major breakthroughs in the OAM-RDs are summarized, and the latest technological standing is examined. Additionally, a detailed account of the recent works published on techniques related to the OAM-RDs has been categorized into five areas: channel multicasting, channel switching, channel filtering, channel hopping, and channel adding/extracting. Meanwhile, the principles, research methods, advantages, and disadvantages are discussed and summarized in depth while analyzing the future development trends and prospects of the OAM-RDs.

6.
Sensors (Basel) ; 24(9)2024 Apr 29.
Artículo en Inglés | MEDLINE | ID: mdl-38732932

RESUMEN

In this paper, a 3D conformal meta-lens designed for manipulating electromagnetic beams via height-to-phase control is proposed. The structure consists of a 40 × 20 array of tunable unit cells fabricated using 3D printing, enabling full 360° phase compensation. A novel automatic synthesizing method (ASM) with an integrated optimization process based on genetic algorithm (GA) is adopted here to create the meta-lens. Simulation using CST Microwave Studio and MATLAB reveals the antenna's beam deflection capability by adjusting phase compensations for each unit cell. Various beam scanning techniques are demonstrated, including single-beam, dual-beam generation, and orbital angular momentum (OAM) beam deflection at different angles of 0°, 10°, 15°, 25°, 30°, and 45°. A 3D-printed prototype of the dual-beam feature has been fabricated and measured for validation purposes, with good agreement between both simulation and measurement results, with small discrepancies due to 3D printing's low resolution and fabrication errors. This meta-lens shows promise for low-cost, high-gain beam deflection in mm-wave wireless communication systems, especially for sensing applications, with potential for wider 2D beam scanning and independent beam deflection enhancements.

7.
Nano Lett ; 23(6): 2436-2441, 2023 Mar 22.
Artículo en Inglés | MEDLINE | ID: mdl-36723626

RESUMEN

The electron vortex beam (EVB)-carrying quantized orbital angular momentum (OAM) plays an essential role in a series of fundamental research. However, the radius of the transverse intensity profile of a doughnut-shaped EVB strongly depends on the topological charge of the OAM, impeding its wide applications in electron microscopy. Inspired by the perfect vortex in optics, herein, we demonstrate a perfect electron vortex beam (PEVB), which completely unlocks the constraint between the beam size and the beam's OAM. We design nanoscale holograms to generate PEVBs carrying different quanta of OAM but exhibiting almost the same beam size. Furthermore, we show that the beam size of the PEVB can be readily controlled by only modifying the design parameters of the hologram. The generation of PEVB with a customized beam size independent of the OAM can promote various in situ applications of free electrons carrying OAM in electron microscopy.

8.
Nano Lett ; 23(7): 2991-2997, 2023 Apr 12.
Artículo en Inglés | MEDLINE | ID: mdl-36971648

RESUMEN

Spiral phase contrast imaging and bright-field imaging are two widely used modes in microscopy, providing distinct morphological information about objects. However, conventional microscopes are always unable to operate with these two modes at the same time and need additional optical elements to switch between them. Here, we present a microscopy setup that incorporates a dielectric metasurface capable of achieving spiral phase contrast imaging and bright-field imaging synchronously. The metasurface not only can focus the light for diffraction-limited imaging but also can perform a two-dimensional spatial differentiation operation by imparting an orbital angular momentum to the incident light field. This allows two spatially separated images to be simultaneously obtained, one containing high-frequency edge information and the other showing the entirety of the object. Combined with the advantages of planar architecture and ultrathin thickness of the metasurface, this approach is expected to provide support in the fields of microscopy, biomedicine, and materials science.

9.
Nano Lett ; 23(9): 3921-3928, 2023 May 10.
Artículo en Inglés | MEDLINE | ID: mdl-37102437

RESUMEN

Twisted photons can in principle carry a discrete unbounded amount of orbital angular momentum (OAM), which are of great significance for quantum communication and fundamental tests of quantum theory. However, the methods for characterization of the OAM quantum states present a fundamental limit for miniaturization. Metasurfaces can exploit new degrees of freedom to manipulate optical fields beyond the capabilities of bulk optics, opening a broad range of novel and superior applications in quantum photonics. Here we present a scheme to reconstruct the density matrix of the OAM quantum states of single photons with all-dielectric metasurfaces composed of birefringent meta-atoms. We have also measured the Schmidt number of the OAM entanglement by the multiplexing of multiple degrees of freedom. Our work represents a step toward the practical application of quantum metadevices for the measurement of OAM quantum states in free-space quantum imaging and communications.

10.
Nano Lett ; 23(6): 2304-2311, 2023 Mar 22.
Artículo en Inglés | MEDLINE | ID: mdl-36880306

RESUMEN

Vortex beams, which intrinsically possess optical orbital angular momentum (OAM), are considered as one of the promising chiral light waves for classical optical communications and quantum information processing. For a long time, it has been an expectation to utilize artificial three-dimensional (3D) chiral metamaterials to manipulate the transmission of vortex beams for practical optical display applications. Here, we demonstrate the concept of selective transmission management of vortex beams with opposite OAM modes assisted by the designed 3D chiral metahelices. Utilizing the integrated array of the metahelices, a series of optical operations, including display, hiding, and even encryption, can be realized by the parallel processing of multiple vortex beams. The results open up an intriguing route for metamaterial-dominated optical OAM processing, which fosters the development of photonic angular momentum engineering and high-security optical encryption.

11.
Nano Lett ; 23(4): 1195-1201, 2023 Feb 22.
Artículo en Inglés | MEDLINE | ID: mdl-36622968

RESUMEN

Metasurfaces have shown remarkable potential to manipulate many of light's intrinsic properties, such as phase, amplitude, and polarization. Recent advancements in nanofabrication technologies and persistent efforts from the research community result in the realization of highly efficient, broadband, and multifunctional metasurfaces. Simultaneous control of these characteristics in a single-layered metasurface will be an apparent technological extension. Here, we demonstrate a broadband multifunctional metasurface platform with the unprecedented ability to independently control the phase profile for two orthogonal polarization states of incident light over dual-wavelength spectra (ultraviolet to visible). In this work, multiple single-layered metasurfaces composed of bandgap-engineered silicon nitride nanoantennas are designed, fabricated, and optically characterized to demonstrate broadband multifunctional light manipulation ability, including structured beam generation and meta-interferometer implementation. We envision the presented metasurface platform opening new avenues for broadband multifunctional applications including ultraviolet-visible spectroscopy, spatially modulated illumination microscopy, optical data storage, and information encoding.

12.
Nano Lett ; 23(19): 9096-9104, 2023 Oct 11.
Artículo en Inglés | MEDLINE | ID: mdl-37748028

RESUMEN

Vertical-cavity surface-emitting lasers (VCSELs) represent an attractive light source to integrate with OAM structures to realize chip-scale vortex lasers. Although pioneering endeavors of VCSEL-based vortex lasers have been reported, they cannot achieve large topological charges (less than l = 5) due to the insufficient space-bandwidth product (SBP) caused by the inherent limited device size. Here, by integrating a nanoprinted OAM phase structure on the VCSELs, we demonstrate a vortex microlaser with a low threshold and simple structure. A monolithic microlaser array with addressable control of vortex beams with different topological charges (l = 1 to l = 5) was achieved. Nanoprinting offers high degrees of freedom for the manipulation of spatial structures. To address the challenge of insufficient SBP, two-layer cascaded spiral phase plates were designed. Thereby, a vortex beam with l = 15 and mode purity of 83.7% was obtained. Our work paves the way for future chip-scale OAM-based information multiplexing with more channels.

13.
Entropy (Basel) ; 26(8)2024 Jul 27.
Artículo en Inglés | MEDLINE | ID: mdl-39202105

RESUMEN

The integration of terrestrial- and satellite-based quantum key distribution (QKD) experiments has markedly advanced global-scale quantum networks, showcasing the growing maturity of quantum technologies. Notably, the use of unmanned aerial vehicles (UAVs) as relay nodes has emerged as a promising method to overcome the inherent limitations of fiber-based and low-Earth orbit (LEO) satellite connections. This paper introduces a protocol for measurement-device-independent QKD (MDI-QKD) using photon orbital angular momentum (OAM) encoding, with UAVs as relay platforms. Leveraging UAV mobility, the protocol establishes a secure and efficient link, mitigating threats from untrusted UAVs. Photon OAM encoding addresses reference frame alignment issues exacerbated by UAV jitter. A comprehensive analysis of atmospheric turbulence, state-dependent diffraction (SDD), weather visibility, and pointing errors on free-space OAM-state transmission systems was conducted. This analysis elucidates the relationship between the key generation rate and propagation distance for the proposed protocol. Results indicate that considering SDD significantly decreases the key rate, halving previous data results. Furthermore, the study identifies a maximum channel loss capacity of 26 dB for the UAV relay platform. This result is pivotal in setting realistic parameters for the deployment of UAV-based quantum communications and lays the foundation for practical implementation strategies in the field.

14.
Proc Natl Acad Sci U S A ; 117(26): 14682-14687, 2020 06 30.
Artículo en Inglés | MEDLINE | ID: mdl-32546523

RESUMEN

We predict and experimentally verify an entoptic phenomenon through which humans are able to perceive and discriminate optical spin-orbit states. Direct perception and discrimination of these particular states of light with polarization-coupled spatial modes is possible through the observation of distinct profiles induced by the interaction between polarization topologies and the radially symmetric dichroic elements that are centered on the foveola in the macula of the human eye. A psychophysical study was conducted where optical states with a superposition of right and left circular polarization coupled to two different orbital angular momentum (OAM) values ([Formula: see text] and [Formula: see text]) were directed onto the retina of participants. The number of azimuthal fringes that a human sees when viewing the spin-orbit states is shown to be equal to the number (N) of radial lines in the corresponding polarization profile of the beam, where [Formula: see text] The participants were able to correctly discriminate between two states carrying OAM [Formula: see text] and differentiated by [Formula: see text] and [Formula: see text], with an average success probability of 77.6% (average sensitivity [Formula: see text], [Formula: see text], [Formula: see text]). These results enable methods of robustly characterizing the structure of the macula, probing retina signaling pathways, and conducting experiments with human detectors and optical states with nonseparable modes.


Asunto(s)
Fenómenos Fisiológicos Oculares , Retina/fisiología , Percepción Visual/fisiología , Humanos , Luz , Estimulación Luminosa , Teoría Cuántica
15.
Proc Natl Acad Sci U S A ; 117(42): 26118-26122, 2020 Oct 20.
Artículo en Inglés | MEDLINE | ID: mdl-33004628

RESUMEN

We present an experimental demonstration of a general entanglement-generation framework, where the form of the entangled state is independent of the physical process used to produce the particles. It is the indistinguishability of multiple generation processes and the geometry of the setup that give rise to the entanglement. Such a framework, termed entanglement by path identity, exhibits a high degree of customizability. We employ one class of such geometries to build a modular source of photon pairs that are high-dimensionally entangled in their orbital angular momentum. We demonstrate the creation of three-dimensionally entangled states and show how to incrementally increase the dimensionality of entanglement. The generated states retain their quality even in higher dimensions. In addition, the design of our source allows for its generalization to various degrees of freedom and even for the implementation in integrated compact devices. The concept of entanglement by path identity itself is a general scheme and allows for construction of sources producing also customized states of multiple photons. We therefore expect that future quantum technologies and fundamental tests of nature in higher dimensions will benefit from this approach.

16.
Sensors (Basel) ; 23(2)2023 Jan 14.
Artículo en Inglés | MEDLINE | ID: mdl-36679765

RESUMEN

In underwater wireless optical communication (UWOC), a vortex beam carrying orbital angular momentum has a spatial spiral phase distribution, which provides spatial freedom for UWOC and, as a new information modulation dimension resource, it can greatly improve channel capacity and spectral efficiency. In a case of the disturbance of a vortex beam by ocean turbulence, where a Laguerre-Gaussian (LG) beam carrying orbital angular momentum (OAM) is damaged by turbulence and distortion, which affects OAM pattern recognition, and the phase feature of the phase map not only has spiral wavefront but also phase singularity feature, the convolutional neural network (CNN) model can effectively extract the information of the distorted OAM phase map to realize the recognition of dual-mode OAM and single-mode OAM. The phase map of the Laguerre-Gaussian beam passing through ocean turbulence was used as a dataset to simulate and analyze the OAM recognition effect during turbulence caused by different temperature ratios and salinity. The results showed that, during strong turbulence Cn2=1.0×10-13K2m-2/3, when different ω = -1.75, the recognition rate of dual-mode OAM (ℓ = ±1~±5, ±1~±6, ±1~±7, ±1~±8, ±1~±9, ±1~±10) had higher recognition rates of 100%, 100%, 100%, 100%, 98.89%, and 98.67% and single-mode OAM (ℓ = 1~5, 1~6, 1~7, 1~8, 1~9, 1~10) had higher recognition rates of 93.33%, 92.77%, 92.33%, 90%, 87.78%, and 84%, respectively. With the increase in ω, the recognition accuracy of the CNN model will gradually decrease, and in a fixed case, the dual-mode OAM has stronger anti-interference ability than single-mode OAM. These results may provide a reference for optical communication technologies that implement high-capacity OAM.


Asunto(s)
Redes Neurales de la Computación , Reconocimiento en Psicología , Humanos , Movimiento (Física) , Distribución Normal , Tecnología
17.
Sensors (Basel) ; 23(16)2023 Aug 11.
Artículo en Inglés | MEDLINE | ID: mdl-37631657

RESUMEN

In laser active detection, detection performance is affected by optical noise, laser interference, and environmental background interference. Conventional methods to filter optical noise take advantage of the differences between signal and noise in wavelength and polarization. Due to the limitations of traditional methods in the physical dimension, noise cannot be completely filtered out. In this manuscript, a new method of noise filtering based on the spatial distribution difference between the quantum orbital angular momentum beam and the background noise is proposed. The use of beams containing quantum orbital angular momentum can make the signal light have a new physical dimension and enrich the information of emitted light. We conduct a complete theoretical analysis and provide a proof-of-principle experiment. The experimental results are in good agreement with the theoretical analysis results, and there is a signal-to-noise ratio improvement of more than five times in laser active detection. Our method meets the urgent needs of laser active detection and can be applied in the field of high-quality target detection.

18.
Sensors (Basel) ; 23(5)2023 Feb 26.
Artículo en Inglés | MEDLINE | ID: mdl-36904796

RESUMEN

Antennas that generate orbital angular momentum (OAM) have the potential to significantly enhance the channel capacity of upcoming wireless systems. This is because different OAM modes that are excited from a shared aperture are orthogonal, which means that each mode can carry a distinct stream of data. As a result, it is possible to transmit multiple data streams at the same time and frequency using a single OAM antenna system. To achieve this, there is a need to develop antennas that can create several OAM modes. This study employs an ultrathin dual-polarized Huygens' metasurface to design a transmit array (TA) that can generate mixed-OAM modes. Two concentrically-embedded TAs are used to excite the desired modes by achieving the required phase difference according to the coordinate position of each unit cell. The prototype of the TA, which operates at 28 GHz and has a size of 11 × 11 cm 2, generates mixed OAM modes of -1 and -2 using dual-band Huygens' metasurfaces. To the best of the authors' knowledge, this is the first time that such a low-profile and dual-polarized OAM carrying mixed vortex beams has been designed using TAs. The maximum gain of the structure is 16 dBi.

19.
Sensors (Basel) ; 23(21)2023 Oct 26.
Artículo en Inglés | MEDLINE | ID: mdl-37960437

RESUMEN

For orbital angular momentum (OAM) recognition in atmosphere turbulence, how to design a self-adapted model is a challenging problem. To address this issue, an efficient deep learning framework that uses a derived extreme learning machine (ELM) has been put forward. Different from typical neural network methods, the provided analytical machine learning model can match the different OAM modes automatically. In the model selection phase, a multilayer ELM is adopted to quantify the laser spot characteristics. In the parameter optimization phase, a fast iterative shrinkage-thresholding algorithm makes the model present the analytic expression. After the feature extraction of the received intensity distributions, the proposed method develops a relationship between laser spot and OAM mode, thus building the steady neural network architecture for the new received vortex beam. The whole recognition process avoids the trial and error caused by user intervention, which makes the model suitable for a time-varying atmospheric environment. Numerical simulations are conducted on different experimental datasets. The results demonstrate that the proposed method has a better capacity for OAM recognition.

20.
Sensors (Basel) ; 23(23)2023 Nov 30.
Artículo en Inglés | MEDLINE | ID: mdl-38067905

RESUMEN

Vortex beams carrying orbital angular momentum (OAM) have gained much interest in optical communications because they can be used to expand the number of multiplexing channels and greatly improve the transmission capacity. However, the number of states used for OAM-based communication is generally limited by the imperfect OAM generation, transmission, and demultiplexing methods. In this work, we proposed a dense space-division multiplexing (DSDM) scheme to further increase the transmission capacity and transmission capacity density of free space optical communications with a small range of OAM modes exploiting a multi-ring perfect vortex (MRPV). The proposed MRPV is generated using a pixel checkerboard complex amplitude modulation method that simultaneously encodes amplitude and phase information in a phase-only hologram. The four rings of the MRPV are mutually independent channels that transmit OAM beams under the condition of occupying only one spatial position, and the OAM mode transmitted in these spatial channels can be efficiently demodulated using a multilayer annular aperture. The effect of atmospheric turbulence on the MRPV was also analyzed, and the results showed that the four channels of the MRPV can be effectively separated under weak turbulence conditions. Under the condition of limited available space and OAM states, the proposed DSDM strategy exploiting MRPV might inspire wide optical communication applications exploiting the space dimension of light beams.

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