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1.
Angew Chem Int Ed Engl ; 61(37): e202208587, 2022 Sep 12.
Artículo en Inglés | MEDLINE | ID: mdl-35791044

RESUMEN

Interfacial photo-vapor conversion has been suggested as a cost-effective and sustainable technology for seawater desalination. However, the conversion performance was still limited by some drawbacks, like salt accumulation and poor mechanical stability. Herein, a scalable MoS2 -based porous hydrogel (SMoS2 -PH) with good mechanical stability and salt resistance was successfully constructed through a crosslinking foaming polymerization method. With the high porosity (92.63 %), the SMoS2 -PH performed an impressive evaporation rate of 3.297 kg m-2 h-1 and photothermal conversion efficiency of 93.4 % under 1-sun illumination. Most importantly, the SMoS2 -PH could maintain high and stable photothermal properties for 15 days on the surface of seawater. We believe that the excellent salt resistance, the high photothermal conversion efficiency, the ease of scale preparation method and the available commercial MoS2 make the SMoS2 -PH a promising device for full-scale seawater desalination.

2.
ChemSusChem ; 16(15): e202300611, 2023 Aug 07.
Artículo en Inglés | MEDLINE | ID: mdl-37271731

RESUMEN

Solar steam generation technology (SSGT) using unlimited solar energy is regarded as one of the most promising sustainable technologies to produce clean water. However, most of studies on SSGT simply focus on how to improve salt resistance as well as exclude inorganic and organic pollutants in targeted water, and only very limited studies pay attention to the micro-organisms in the collected water. Herein, one porous Cu2 ZnSnS4 -based photothermal hydrogel (CZTS-PH) with antibacterial properties as well as good salt resistance was successfully prepared. The CZTS-PH was measured with the water evaporation rate as high as 3.249 kg m-2 h-1 and photothermal conversion efficiency of 96.3 % under one sun irradiation. Impressively, owing to the amino groups in the skeleton, CZTS-PH can significantly deteriorate the cell membrane and lead to the death of the Escherichia coli (E. coli) and Staphylococcus aureus (S. aureus), which ensures its long-term stability photothermal conversion and the safety of clean water. Overall, the admired photothermal conversion efficiency, and the excellent salt resistance and antibacterial performance suggest that CZTS-PH could be a promising full-scale device applied in seawater desalination and water purification.


Asunto(s)
Hidrogeles , Aguas del Alcantarillado , Destilación , Escherichia coli , Staphylococcus aureus , Cloruro de Sodio , Agua de Mar , Agua , Antibacterianos/farmacología
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